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  • Elsevier  (171,811)
  • 2010-2014  (129,654)
  • 1980-1984  (42,157)
  • 2014  (129,654)
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  • 11
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    South Pacific dissolved Nd isotope compositions and rare earth element distributions: Water mass mixing versus biogeochemical cycling (2014)
    Elsevier
    Details
    Publication Date: 2023-01-23
    Description: Despite its enormous extent and importance for global climate, the South Pacific has been poorly investigated in comparison to other regions with respect to chemical oceanography. Here we present the first detailed analysis of dissolved radiogenic Nd isotopes (εNd) and rare earth elements (REEs) in intermediate and deep waters of the mid-latitude (∼40°S) South Pacific along a meridional transect between South America and New Zealand. The goal of our study is to gain better insight into the distribution and mixing of water masses in the South Pacific and to evaluate the validity of Nd isotopes as a water mass tracer in this remote region of the ocean. The results demonstrate that biogeochemical cycling (scavenging processes in the Eastern Equatorial Pacific) and release of LREEs from the sediment clearly influence the distribution of the dissolved REE concentrations at certain locations. Nevertheless, the Nd isotope signatures clearly trace water masses including AAIW (Antarctic Intermediate Water) (average εNd = −8.2 ± 0.3), LCDW (Lower Circumpolar Deep Water) (average εNd = −8.3 ± 0.3), NPDW (North Pacific Deep Water) (average εNd = −5.9 ± 0.3), and the remnants of NADW (North Atlantic Deep Water) (average εNd = −9.7 ± 0.3). Filtered water samples taken from the sediment–water interface under the deep western boundary current off New Zealand suggest that boundary exchange processes are limited at this location and highlight the spatial and temporal variability of this process. These data will serve as a basis for the paleoceanographic application of Nd isotopes in the South Pacific.
    Type: Article , PeerReviewed
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  • 12
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    Distinguishing seawater from geologic brine in saline coastal groundwater using radium-226; an example from the Sabkha of the UAE (2014)
    Elsevier
    Details
    Publication Date: 2022-05-26
    Description: This paper is not subject to U.S. copyright. The definitive version was published in Chemical Geology 371 (2014): 1-8, doi:10.1016/j.chemgeo.2014.01.018.
    Description: Sabkhat (Salt flats) are common geographic features of low-lying marine coastal areas that develop under hyper-arid climatic conditions. They are characterized by the presence of highly concentrated saline solutions and evaporitic minerals, and have been cited in the geologic literature as present-day representations of hyper-arid regional paleohydrogeology, paleoclimatology, coastal processes, and sedimentation in the geologic record. It is therefore important that a correct understanding of the origin and development of these features be achieved. Knowledge of the source of solutes is an important first step in understanding these features. Historically, two theories have been advanced as to the main source of solutes in sabkha brines: an early concept entailing seawater as the obvious source, and a more recent and dynamic theory involving ascending geologic brine forced upward into the base of the sabkha by a regional hydraulic gradient in the underlying formations. Ra-226 could uniquely distinguish between these sources under certain circumstances, as it is typically present at elevated activity of hundreds to thousands of Bq/m3 (Becquerels per cubic meter) in subsurface formation brines; at exceedingly low activities in open ocean and coastal water; and not significantly supplied to water from recently formed marine sedimentary framework material. The coastal marine sabkha of the Emirate of Abu Dhabi was used to test this hypothesis. The distribution of Ra-226 in 70 samples of sabkha brine (mean: 700 Bq/m3), 7 samples of underlying deeper formation brine (mean: 3416 Bq/m3), the estimated value of seawater (〈 16 Bq/m3) and an estimate of supply from sabkha sedimentary framework grains (〈~6 Bq/m3) provide the first direct evidence that ascending geologic brine contributes significantly to the solutes of this sabkha system.
    Keywords: Sabkhat ; Radium-226 ; Geologic brine ; Seawater
    Repository Name: Woods Hole Open Access Server
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  • 13
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    Multiple sulfur isotope constraints on the modern sulfur cycle (2014)
    Elsevier
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    Publication Date: 2022-05-26
    Description: © The Author(s), 2014. This article is distributed under the terms of the Creative Commons Attribution License. The definitive version was published in Earth and Planetary Science Letters 396 (2014): 14-21, doi:10.1016/j.epsl.2014.03.057.
    Description: We present 28 multiple sulfur isotope measurements of seawater sulfate (δ34SSO4δ34SSO4 and Δ33SSO4Δ33SSO4) from the modern ocean over a range of water depths and sites along the eastern margin of the Pacific Ocean. The average measured δ34SSO4δ34SSO4 is 21.24‰ (±0.88‰,2σ±0.88‰,2σ) with a calculated Δ33SSO4Δ33SSO4 of +0.050‰+0.050‰ (±0.014‰,2σ±0.014‰,2σ). With these values, we use a box-model to place constraints on the gross fraction of pyrite burial in modern sediments. This model presents an improvement on previous estimates of the global pyrite burial flux because it does not rely on the assumed value of δ34Spyriteδ34Spyrite, which is poorly constrained, but instead uses new information about the relationship between δ34Sδ34S and δ33Sδ33S in global marine sulfate. Our calculations indicate that the pyrite burial flux from the modern ocean is between 10% and 45% of the total sulfur lost from the oceans, with a more probable range between 20% and 35%.
    Description: RT acknowledges financial support from NERC Grant NE/I00596X/1. Support was provided through NERC grant NE/H011595/1 to AVT. AVT acknowledges financial support from the ERC Starting Investigator Grant 307582. JF acknowledges support from the NASA Astrobiology Institute.
    Keywords: Sulfur isotopes ; Multiple sulfur isotopes ; Pyrite flux ; Sulfur cycle ; Sulfate reduction ; Biogeochemical cycles
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  • 14
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    Assessment of tsunami hazard to the U.S. Atlantic margin (2014)
    Elsevier
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    Publication Date: 2022-05-26
    Description: This paper is not subject to U.S. copyright. The definitive version was published in Marine Geology 353 (2014): 31-54, doi:10.1016/j.margeo.2014.02.011.
    Description: Tsunami hazard is a very low-probability, but potentially high-risk natural hazard, posing unique challenges to scientists and policy makers trying to mitigate its impacts. These challenges are illustrated in this assessment of tsunami hazard to the U.S. Atlantic margin. Seismic activity along the U.S. Atlantic margin in general is low, and confirmed paleo-tsunami deposits have not yet been found, suggesting a very low rate of hazard. However, the devastating 1929 Grand Banks tsunami along the Atlantic margin of Canada shows that these events continue to occur. Densely populated areas, extensive industrial and port facilities, and the presence of ten nuclear power plants along the coast, make this region highly vulnerable to flooding by tsunamis and therefore even low-probability events need to be evaluated. We can presently draw several tentative conclusions regarding tsunami hazard to the U.S. Atlantic coast. Landslide tsunamis likely constitute the biggest tsunami hazard to the coast. Only a small number of landslides have so far been dated and they are generally older than 10,000 years. The geographical distribution of landslides along the margin is expected to be uneven and to depend on the distribution of seismic activity along the margin and on the geographical distribution of Pleistocene sediment. We do not see evidence that gas hydrate dissociation contributes to the generation of landslides along the U.S. Atlantic margin. Analysis of landslide statistics along the fluvial and glacial portions of the margin indicate that most of the landslides are translational, were probably initiated by seismic acceleration, and failed as aggregate slope failures. How tsunamis are generated from aggregate landslides remains however, unclear. Estimates of the recurrence interval of earthquakes along the continental slope may provide maximum estimates for the recurrence interval of landslide along the margin. Tsunamis caused by atmospheric disturbances and by coastal earthquakes may be more frequent than those generated by landslides, but their amplitudes are probably smaller. Among the possible far-field earthquake sources, only earthquakes located within the Gulf of Cadiz or west of the Tore-Madeira Rise are likely to affect the U.S. coast. It is questionable whether earthquakes on the Puerto Rico Trench are capable of producing a large enough tsunami that will affect the U.S. Atlantic coast. More information is needed to evaluate the seismic potential of the northern Cuba fold-and-thrust belt. The hazard from a volcano flank collapse in the Canary Islands is likely smaller than originally stated, and there is not enough information to evaluate the magnitude and frequency of flank collapse from the Azores Islands. Both deterministic and probabilistic methods to evaluate the tsunami hazard from the margin are available for application to the Atlantic margin, but their implementation requires more information than is currently available.
    Description: The work was funded by the U.S.-NRC Job Code V6166: Tsunami Landslide Source Probability and Potential Impact on New and Existing Power Plants.
    Keywords: Submarine landslides ; Meteo-tsunami ; Earthquakes and landslides ; Probabilistic hazard assessment
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  • 15
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    Composition of hydrothermal fluids and mineralogy of associated chimney material on the East Scotia Ridge back-arc spreading centre (2014)
    Elsevier
    Details
    Publication Date: 2022-05-26
    Description: © The Author(s), 2014. This article is distributed under the terms of the Creative Commons Attribution License. The definitive version was published in Geochimica et Cosmochimica Acta 139 (2014): 47-71, doi:10.1016/j.gca.2014.04.024.
    Description: The East Scotia Ridge is an active back-arc spreading centre located to the west of the South Sandwich island arc in the Southern Ocean. Initial exploration of the ridge by deep-tow surveys provided the first evidence for hydrothermal activity in a back-arc setting outside of the western Pacific, and we returned in 2010 with a remotely operated vehicle to precisely locate and sample hydrothermal sites along ridge segments E2 and E9. Here we report the chemical and isotopic composition of high- and low-temperature vent fluids, and the mineralogy of associated high-temperature chimney material, for two sites at E2 (Dog’s Head and Sepia), and four sites at E9 (Black & White, Ivory Tower, Pagoda and Launch Pad). The chemistry of the fluids is highly variable between the ridge segments. Fluid temperatures were ∼350 °C at all vent sites except Black & White, which was significantly hotter (383 °C). End-member chloride concentrations in E2 fluids (532–536 mM) were close to background seawater (540 mM), whereas Cl in E9 fluids was much lower (98–220 mM) indicating that these fluids are affected by phase separation. Concentrations of the alkali elements (Na, Li, K and Cs) and the alkaline earth elements (Ca, Sr and Ba) co-vary with Cl, due to charge balance constraints. Similarly, concentrations of Mn and Zn are highest in the high Cl fluids but, by contrast, Fe/Cl ratios are higher in E9 fluids (3.8–8.1 × 10−3) than they are in E2 fluids (1.5–2.4 × 10−3) and fluids with lowest Cl have highest Cu. Although both ridge segments are magmatically inflated, there is no compelling evidence for input of magmatic gases to the vent fluids. Fluid δD values range from 0.2‰ to 1.5‰, pH values (3.02–3.42) are not especially low, and F concentrations (34.6–54.4 μM) are lower than bottom seawater (62.8 μM). The uppermost sections of conjugate chimney material from E2, and from Ivory Tower and Pagoda at E9, typically exhibit inner zones of massive chalcopyrite enclosed within an outer zone of disseminated sulphide, principally sphalerite and pyrite, in an anhydrite matrix. By contrast, the innermost part of the chimneys that currently vent fluids with lowest Cl (Black & White and Launch Pad), is dominated by anhydrite. By defining and assessing the controls on the chemical composition of these vent fluids, and associated mineralisation, this study provides new information for evaluating the significance of hydrothermal processes at back-arc basins for ocean chemistry and the formation of seafloor mineral deposits.
    Description: This work was funded by the Natural Environment Research Council consortium grant NE/D01249X/1. C.R.G. acknowledges further support from the National Science Foundation’s Office of Polar Programs grant ANT-0739675. N.R.B. acknowledges funding from the National Sciences and Engineering Research Council of Canada, Ontario Ministry of Research and Innovation, and the Academic Development Fund at Western University.
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  • 16
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    A fossil winonaite-like meteorite in Ordovician limestone : a piece of the impactor that broke up the L-chondrite parent body? (2014)
    Elsevier
    Details
    Publication Date: 2022-05-26
    Description: © The Author(s), 2014. This article is distributed under the terms of the Creative Commons Attribution License. The definitive version was published in Earth and Planetary Science Letters 400 (2014): 145-152, doi:10.1016/j.epsl.2014.05.034.
    Description: About a quarter of all meteorites falling on Earth today originate from the breakup of the L-chondrite parent body ∼470 Ma∼470 Ma ago, the largest documented breakup in the asteroid belt in the past ∼3 Ga∼3 Ga. A window into the flux of meteorites to Earth shortly after this event comes from the recovery of about 100 fossil L chondrites (1–21 cm in diameter) in a quarry of mid-Ordovician limestone in southern Sweden. Here we report on the first non-L-chondritic meteorite from the quarry, an 8 cm large winonaite-related meteorite of a type not known among present-day meteorite falls and finds. The noble gas data for relict spinels recovered from the meteorite show that it may be a remnant of the body that hit and broke up the L-chondrite parent body, creating one of the major asteroid families in the asteroid belt. After two decades of systematic recovery of fossil meteorites and relict extraterrestrial spinel grains from marine limestone, it appears that the meteorite flux to Earth in the mid-Ordovician was very different from that of today.
    Description: This study was supported by an European Research Council Advanced Grant to B.S., in part by NASA grant NNX08AE08G to K.K., and a grant to M.M. from the Swiss National Science Foundation.
    Keywords: Fossil meteorite ; Asteroid breakup ; Winonaite ; Ordinary chondrite ; Asteroid family ; Meteorite flux
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  • 17
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    Anthropogenic nutrients and harmful algae in coastal waters (2014)
    Elsevier
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    Publication Date: 2022-05-26
    Description: © The Author(s), 2014. This article is distributed under the terms of the Creative Commons Attribution License. The definitive version was published in Journal of Environmental Management 146 (2014): 206-216, doi:10.1016/j.jenvman.2014.07.002.
    Description: Harmful algal blooms (HABs) are thought to be increasing in coastal waters worldwide. Anthropogenic nutrient enrichment has been proposed as a principal causative factor of this increase through elevated inorganic and/or organic nutrient concentrations and modified nutrient ratios. We assess: 1) the level of understanding of the link between the amount, form and ratio of anthropogenic nutrients and HABs; 2) the evidence for a link between anthropogenically generated HABs and negative impacts on human health; and 3) the economic implications of anthropogenic nutrient/HAB interactions. We demonstrate that an anthropogenic nutrient-HAB link is far from universal, and where it has been demonstrated, it is most frequently associated with high biomass rather than low biomass (biotoxin producing) HABs. While organic nutrients have been shown to support the growth of a range of HAB species, insufficient evidence exists to clearly establish if these nutrients specifically promote the growth of harmful species in preference to benign ones, or if/how they influence toxicity of harmful species. We conclude that the role of anthropogenic nutrients in promoting HABs is site-specific, with hydrodynamic processes often determining whether blooms occur. We also find a lack of evidence of widespread significant adverse health impacts from anthropogenic nutrient-generated HABs, although this may be partly due to a lack of human/animal health and HAB monitoring. Detailed economic evaluation and cost/benefit analysis of the impact of anthropogenically generated HABs, or nutrient reduction schemes to alleviate them, is also frequently lacking.
    Description: The work described here is based in part on a project ‘Harmful Algae, Nuisance Blooms and Anthropogenic Nutrient Enrichment’ funded by the UK Department for Environment, Food and Rural Affairs (contract ME2208). In addition KD was supported by the FP7 project Asimuth and funding from the NERC Shelf Seas Biogeochemistry and PURE Associates programmes. PJH was supported by University Grants Council of Hong Kong AoE project (AoE/P-04/0401). PH and LEF were funded by the US National Science Foundation (NSF) Award 1009106; LEF was funded in part by the European Regional Development Fund and European Social Fund (University of Exeter, Truro, Cornwall, UK). GM was supported by a NERC PhD studentship.
    Keywords: Harmful algal blooms ; HABs ; Anthropogenic nutrients ; Human health ; Economic impact
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  • 18
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    PSP toxin levels and plankton community composition and abundance in size-fractionated vertical profiles during spring/summer blooms of the toxic dinoflagellate Alexandrium fundyense in the Gulf of Maine and on Georges Bank, 2007, 2008, and 2010 : 1. Toxin levels (2014)
    Elsevier
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    Publication Date: 2022-05-26
    Description: This paper is not subject to U.S. copyright. The definitive version was published in Deep Sea Research Part II: Topical Studies in Oceanography 103 (2014): 329–349, doi:10.1016/j.dsr2.2013.04.013.
    Description: As part of the NOAA ECOHAB funded Gulf of Maine Toxicity (GOMTOX)1 project, we determined Alexandrium fundyense abundance, paralytic shellfish poisoning (PSP) toxin composition, and concentration in quantitatively-sampled size-fractionated (20–64, 64–100, 100–200, 200–500, and 〉500 μm) particulate water samples, and the community composition of potential grazers of A. fundyense in these size fractions, at multiple depths (typically 1, 10, 20 m, and near-bottom) during 10 large-scale sampling cruises during the A. fundyense bloom season (May–August) in the coastal Gulf of Maine and on Georges Bank in 2007, 2008, and 2010. Our findings were as follows: (1) when all sampling stations and all depths were summed by year, the majority (94%±4%) of total PSP toxicity was contained in the 20–64 μm size fraction; (2) when further analyzed by depth, the 20–64 μm size fraction was the primary source of toxin for 97% of the stations and depths samples over three years; (3) overall PSP toxin profiles were fairly consistent during the three seasons of sampling with gonyautoxins (1, 2, 3, and 4) dominating (90.7%±5.5%), followed by the carbamate toxins saxitoxin (STX) and neosaxitoxin (NEO) (7.7%±4.5%), followed by n-sulfocarbamoyl toxins (C1 and 2, GTX5) (1.3%±0.6%), followed by all decarbamoyl toxins (dcSTX, dcNEO, dcGTX2&3) (〈1%), although differences were noted between PSP toxin compositions for nearshore coastal Gulf of Maine sampling stations compared to offshore Georges Bank sampling stations for 2 out of 3 years; (4) surface cell counts of A. fundyense were a fairly reliable predictor of the presence of toxins throughout the water column; and (5) nearshore surface cell counts of A. fundyense in the coastal Gulf of Maine were not a reliable predictor of A. fundyense populations offshore on Georges Bank for 2 out of the 3 years sampled.
    Description: Vangie Shue was supported through the FDA and also through the Thomas Jefferson High School for Science and Technology Mentorship Program. Research support was provided by National Oceanic and Atmospheric Administration Grant NA06NOS4780245 for the Gulf of Maine Toxicity (GOMTOX) program. BAK, DJM, and DMA were partially supported by the Woods Hole Center for Oceans and Human Health through National Science Foundation Grants OCE-0430724 and OCE-0911031 and National Institute of Environmental Health Sciences Grant 1P50-ES01274201.
    Keywords: Harmful algal bloom ; PSP toxins ; Alexandrium sp. ; Vectorial intoxication ; Gulf of Maine ; Georges Bank
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  • 19
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    Near-bottom circulation and dispersion of sediment containing Alexandrium fundyense cysts in the Gulf of Maine during 2010–2011 (2014)
    Elsevier
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    Publication Date: 2022-05-26
    Description: © The Author(s), 2013. This article is distributed under the terms of the Creative Commons Attribution License. The definitive version was published in Deep Sea Research Part II: Topical Studies in Oceanography 103 (2014): 96–111, doi:10.1016/j.dsr2.2013.11.003.
    Description: The life cycle of Alexandrium fundyense in the Gulf of Maine includes a dormant cyst stage that spends the winter predominantly in the bottom sediment. Wave-current bottom stress caused by storms and tides induces resuspension of cyst-containing sediment during winter and spring. Resuspended sediment could be transported by water flow to different locations in the Gulf and the redistribution of sediment containing A. fundyense cysts could alter the spatial and temporal manifestation of its spring bloom. The present study evaluates model near-bottom flow during storms, when sediment resuspension and redistribution are most likely to occur, between October and May when A. fundyense cells are predominantly in cyst form. Simulated water column sediment (mud) concentrations from representative locations of the Gulf are used to initialize particle tracking simulations for the period October 2010–May 2011. Particles are tracked in full three-dimensional model solutions including a sinking velocity characteristic of cyst and aggregated mud settling (0.1 mm s−1). Although most of the material was redeposited near the source areas, small percentages of total resuspended sediment from some locations in the western (~4%) and eastern (2%) Maine shelf and the Bay of Fundy (1%) traveled distances longer than 100 km before resettling. The redistribution changed seasonally and was sensitive to the prescribed sinking rate. Estimates of the amount of cysts redistributed with the sediment were small compared to the inventory of cysts in the upper few centimeters of sediment but could potentially have more relevance immediately after deposition.
    Description: Research support to all authors, except DJM and VAS, was provided by U.S. Geological Survey. DJM gratefully acknowledges financial support of the National Oceanic and Atmospheric Administration (Grant NA06NOS4780245 for the Gulf of Maine Toxicity (GOMTOX) program) and the Woods Hole Center for Oceans and Human Health through National Science Foundation Grant OCE-1314642 and National Institute of Environmental Health Sciences Grant 1P01ES021923-01. VAS was supported by the North East Consortium Grant NA05NMF4721057.
    Keywords: Sediment connectivity ; Near-bottom circulation ; Harmful Algal Bloom cysts ; Gulf of Maine ; Alexandrium fundyense ; Particle tracking
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  • 20
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    Investigating the importance of sediment resuspension in Alexandrium fundyense cyst population dynamics in the Gulf of Maine (2014)
    Elsevier
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    Publication Date: 2022-05-26
    Description: © The Author(s), 2013. This article is distributed under the terms of the Creative Commons Attribution License. The definitive version was published in Deep Sea Research Part II: Topical Studies in Oceanography 103 (2014): 79–95, doi:10.1016/j.dsr2.2013.10.011.
    Description: Cysts of Alexandrium fundyense, a dinoflagellate that causes toxic algal blooms in the Gulf of Maine, spend the winter as dormant cells in the upper layer of bottom sediment or the bottom nepheloid layer and germinate in spring to initiate new blooms. Erosion measurements were made on sediment cores collected at seven stations in the Gulf of Maine in the autumn of 2011 to explore if resuspension (by waves and currents) could change the distribution of over-wintering cysts from patterns observed in the previous autumn; or if resuspension could contribute cysts to the water column during spring when cysts are viable. The mass of sediment eroded from the core surface at 0.4 Pa ranged from 0.05 kg m−2 near Grand Manan Island, to 0.35 kg m−2 in northern Wilkinson Basin. The depth of sediment eroded ranged from about 0.05 mm at a station with sandy sediment at 70 m water depth on the western Maine shelf, to about 1.2 mm in clayey–silt sediment at 250 m water depth in northern Wilkinson Basin. The sediment erodibility measurements were used in a sediment-transport model forced with modeled waves and currents for the period October 1, 2010 to May 31, 2011 to predict resuspension and bed erosion. The simulated spatial distribution and variation of bottom shear stress was controlled by the strength of the semi-diurnal tidal currents, which decrease from east to west along the Maine coast, and oscillatory wave-induced currents, which are strongest in shallow water. Simulations showed occasional sediment resuspension along the central and western Maine coast associated with storms, steady resuspension on the eastern Maine shelf and in the Bay of Fundy associated with tidal currents, no resuspension in northern Wilkinson Basin, and very small resuspension in western Jordan Basin. The sediment response in the model depended primarily on the profile of sediment erodibility, strength and time history of bottom stress, consolidation time scale, and the current in the water column. Based on analysis of wave data from offshore buoys from 1996 to 2012, the number of wave events inducing a bottom shear stress large enough to resuspend sediment at 80 m ranged from 0 to 2 in spring (April and May) and 0 to 10 in winter (October through March). Wave-induced resuspension is unlikely in water greater than about 100 m deep. The observations and model results suggest that a millimeter or so of sediment and associated cysts may be mobilized in both winter and spring, and that the frequency of resuspension will vary interannually. Depending on cyst concentration in the sediment and the vertical distribution in the water column, these events could result in a concentration in the water column of at least 104 cysts m−3. In some years, resuspension events could episodically introduce cysts into the water column in spring, where germination is likely to be facilitated at the time of bloom formation. An assessment of the quantitative effects of cyst resuspension on bloom dynamics in any particular year requires more detailed investigation.
    Description: Research support to Donald M. Anderson and Bruce A. Keafer provided through the Woods Hole Center for Oceans and Human Health; National Science Foundation Grants OCE-0430724 and OCE-0911031; and National Institute of Environmental Health Sciences Grant 1-P50-ES012742-01; the ECOHAB Grant program through NOAA Grants NA06NOS4780245 and A09NOS4780193; the MERHAB Grant program through NOAA Grant NA11NOS4780025; and the PCMHAB Grant program through NOAA Grant NA11NOS4780023. Research support to all other authors was provided by U.S. Geological Survey.
    Keywords: Sediment transport ; Bottom stress ; Sediment resuspension ; Harmful algal blooms ; Gulf of Maine ; Alexandrium fundyense ; HAB
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