Abstract
A single, fully wettable, neutrally buoyant, small radioactive particle and 16 scintillation detectors are utilized to monitor particle motion in gas-liquid bubble columns of different heights and diameters and at different gas superficial velocities. Instantaneous velocities, time-averaged velocities, Reynolds stresses and eddy diffusivities are computed from the particle position versus time data. Anisotropy, indicated by the data, was confirmed by Hurst's rescaled R/S analysis of the fluctuating velocities. For the radial direction, Hurst's exponent is about 0.5 in agreement with a random walk (diffusion)-type mechanism, while in the axial direction, Hurst's exponent of about 0.7 indicates the persistence of long-range effects.
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Abbreviations
- \(\vec a\) :
-
position vector
- D :
-
eddy dispersion coefficient, (cm2/s); also column diameter, (m)
- H :
-
Hurst's exponent
- N exp :
-
number of independent experiments
- R L :
-
autocorrelation coefficient
- R(t, s) :
-
accumulated range of fluctuation velocities, (m/s)
- rms:
-
root mean square
- S(t, s) :
-
sample normalized standard deviation
- s :
-
number of recorded (sampled) fluctuating velocities
- t :
-
time, (s); also number of sampled fluctuating velocities
- T L :
-
integral time scale of turbulence, (s)
- v∼ :
-
Lagrangian fluctuating velocity, (m/s)
- U G :
-
superficial gas velocity, (m/s)
- u :
-
index of summation
- X(t) :
-
random variable, i.e. fluctuating velocity component, (m/s)
- X * (t) :
-
record of random variables (i.e. fluctuating velocities) de fined by Eq. (5)
References
Baird, M. H. J.; Rice, R. G. 1975: Axial dispersion in large unbaffled columns. Chem. Eng. J., 9, 171–174
Beaton, W. I.; McDaniel, N. K.; McWhriter, W. E.; Petersen, R. D., Van Driesen, R. P. 1986: ‘Resid hydrocracker expands crude processing flexibility’, Oil Gas J. 7, 47–53
Deckwer, W. D.; Schumpe, A. 1987: Bubble columns — the state of the art and current trends. Int. Chem. Eng., 27, 405–422
Devanathan, N. 1991: Investigation of liquid hydrodynamics in bubble columns via computer automated radioactive particle tracking (CARPT). D.Sc. Thesis, Washington University, St. Louis
Devanathan, N.; Moslemian, D.; Duduković, M. P. 1990: Flow mapping in bubble columns using CARPT. Chem. Eng. Sci., 45, 2285–2291
Duduković, M. P.; Devanathan, N.; Holub, R. 1991: Multiphase reactors: models and experimental verification. Rev. Inst. Francais du Petrole, 46, 439–465
Fan, L. S. 1989: Gas-liquid-solid fluidization engineering. Butterworth, Boston, MA
Fan, L. T.; Neogi, T.; Yashima, M.; Nassar, R. 1990: Stochastic analysis of a three-phase fluidized bed: Fractal approach. AIChe J. 36, 1529–1536
Hurst, E. H., 1956: Methods of using long-term storage in reservoirs: I Proc. Inst. Civil. Eng. 5, 519–525
Lin, J. S.; Chen, M. M.; Chao, B. T. 1985: A Novel radioactive particle tracking facility for measurement of solids motion in gas fluidized beds. AIChE J. 31, 465–473
Lubbert, A.; Wan, L. W. 1990: Mixing mechanisms in column reactors, A Fractal Analysis, Personal communication
Mandelbrot. B. B.; Wallis, J. R. 1969: Robustness of the rescaled range R/S in the measurement of noncyclic long run statistical dependence. Water Resour. Res. 5, 967–988
Meek, C. C. 1972: Statistical characterization of dilute particulate suspensions in turbulent fluid fields, Ph.D. Thesis, University of Illinois, Urbana, Illinois
Menzel, T.; Inderweide, T.; Standacker, O.; Wein, O.; Onken, U. 1990: Reynolds shear stress for modeling of bubble column reactors. IEC Research 29, 988–994
Miyauchi, T.; Furwsaki, S.; Mooroka, S.; Ikdea, Y. 1981: Transport phenomena and reaction in fluidized catalyst beds. Adv. Chem. Eng. 11, 276–448
Moslemian, M.; Chen, M.; Chao, B. T. 1989: Experimental and numerical simulations of solids mixing in a gas solid fluidizedbed, Particulate Sci. Techn. 7, 335–355
Shah, Y. T.; Kelkar, B. G.; Godbole, S. P.; Deckwer, W. D. 1982: Design parameter estimations for bubble column reactors, AIChE J. 28, 353–379
Tarmy, B. L.; Chang, M.; Coulaloglou, C. A.; Ponzi, P. R. 1984: The three-phase hydrodynamic characteristics of the EDS coal liquefaction reactors: their development and scale-up, Proc. of the Eighth International Symposium on Chemical Reaction Engineering, Elsevier Scientific, New York, N. Y.
Torvik, R. 1990: Investigations of 2- and 3-phase bubble columns. Ph.D. Thesis, University of Trondheim, Norway
Yao, B. B.; Zheng, C.; Gasche, H. F.; Hofmann, H. 1990: Bubble behavior and flow structure of bubble columns. Chem. Eng. Process. 27, 101–105
Yang, Y. B. 1992: Imaging of multiphase reactors: tracer and hydrodynamic studies using CARPT-CAT. CREL Annual Report 1991/92, Washington University, St. Louis, pp. 23–28
Zlokarnik, M. 1982: Verfahrenstechnik der aeroben Abwasserreiningung. Chem. Ing. Tech. 54, 939–945
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Currently with Abbott Laboratories, Abbott Park, IL 60064
Currently with Amoco Oil Research Center, Naperville, IL 60566
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Yang, Y.B., Devanathan, N. & Duduković, M.P. Liquid backmixing in bubble columns via computer-automated radioactive particle tracking (CARPT). Experiments in Fluids 16, 1–9 (1993). https://doi.org/10.1007/BF00188499
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DOI: https://doi.org/10.1007/BF00188499