Abstract
The (199Hg)+ ions were stored in an RF quadrupole electric field and their ground state hyperfine populations pumped optically using the ion resonance radiation at 1942 Å from a (202Hg) isotope enriched lamp. A microwave field at 40.5 GHz was phase-locked to the 1350th harmonic of the output of a frequency synthesizer, referenced to a Cs-beam frequency standard. Using a digital averager, a high background suppression optical system monitored the fluorescence light from the ions. Linewidths on the order of 3 Hz were observed for the “field-independent” 0-0 transition, and a value of 40, 507, 348, 051±50 Hz was deduced for the magnetic hyperfine interval, corrected to zero magnetic field.
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References
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The authors are indebted to V. Kaufman of the U.S. Nat. Bureau of Standards, Gaitherburg, for obtaining high resolution spectrograms on a 10 m vacuum spectrograph of our experimental lamps
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Preliminary attempts to observe transition frequency shifts induced by a He buffer gas revealed shifts far greater than theoretically expected, and further study is indicated
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Work done under NASA support, originally at Goddard Space Flight Center (1969–73), more recently under NSG-5107
Senior Research Associate, Catholic University of American, 1976-present