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Observed Trends in Total Vertical Column Abundances of Atmospheric Gases from IR Solar Spectra Recorded at the Jungfraujoch

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Abstract

Since 1984, about 15000 high quality infrared solar spectra have beenrecorded with state-of-the-art grating and Fourier transform spectrometersat the International Scientific Station of the Jungfraujoch, Switzerland.Nonlinear least squares spectral curve fitting of selected microwindowscontaining isolated and well characterized lines of 20 telluric gases haveallowed to retrieve their total vertical column abundances above thestation, leading to observational data bases essential to derive long- andshort-term changes experienced by these species during the last 12 years. Inthis paper, we focus on atmospheric gases of particular interest within thecontext of the EUROTRAC/TOR (Tropospheric Ozone Research) project; secularevolution as well as seasonal cycles of the minor constituentsCH4, CO and of the trace gasesC2H6, OCS, C2H2, HCNand H2CO are reported and discussed. The long-livedN2O is included as a tracer of the dynamic activity of theatmosphere.

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Authors and Affiliations

  1. Institute of Astrophysics and Geophysics, University of Liège, 4000, Liège, Belgium

    E. Mahieu, R. Zander, L. Delbouille, P. Demoulin, G. Roland & C. Servais

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  1. E. Mahieu
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  2. R. Zander
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  3. L. Delbouille
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  4. P. Demoulin
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  5. G. Roland
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  6. C. Servais
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Mahieu, E., Zander, R., Delbouille, L. et al. Observed Trends in Total Vertical Column Abundances of Atmospheric Gases from IR Solar Spectra Recorded at the Jungfraujoch. Journal of Atmospheric Chemistry 28, 227–243 (1997). https://doi.org/10.1023/A:1005854926740

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