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Diluting a salty soup: Impact of long-lasting salt pollution on a deep Alpine lake (Traunsee, Austria) and the downside of recent recovery from salinization

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Abstract

Saline emissions can elevate water densities and have the potential to alter stratification and mixing dynamics in lakes. In the light of rising anthropogenic salinization of temperate freshwater lakes, it is highly relevant to understand how saline emissions, as well as the rehabilitation from salt pollution might affect lake circulation patterns. In this study, we present the impact of industrial pollution with chloride salts on the deep Alpine lake Traunsee in Austria from 1930 to 2005 and the observed limnological changes during the recovery from salinization in the following 12 years. We assembled and analysed a unique dataset of monthly sampling profiles covering chloride, conductivity, temperature and dissolved oxygen over a 87-year period. We quantified the impact of saline emissions on the lake’s total chloride content, water densities, stability indices and deepwater oxygen concentrations. Time-series of water density profiles and stability indices revealed a significant impact of salinization on seasonal stratification and mixing. Higher dilution and shallower release of saline wastes and the short water retention in Traunsee helped to prevent a long-lasting density stratification. Nevertheless, two periods of salt-induced meromixis occurred in the lake. The first was caused directly by the disposal of saline wastes into the deepwater in the 1930s and 1940s, whereas the second was induced by the recovery from salinization in recent years. The naturally faster wash-out of salts from shallower water layers reinforced the density gradient and impeded vertical water circulation after salt pollution ceased. The rehabilitation from salinization had a stronger effect on stratification intensity and deepwater oxygen concentration than the continuous salt pollution over the last century.

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References

  • Adrian R, O’Reilly CM, Zagarese H, Baines SB, Hessen DO, Keller W et al (2009) Lakes as sentinels of climate change. Limnol Oceanogr 54:2283–2297

    Article  Google Scholar 

  • Ambrosetti W, Barbanti L, Sala N (2003) Residence time and physical processes in lakes. J Limnol 62:1–15

    Article  Google Scholar 

  • Anderson GC (1958) Seasonal characteristics of two saline lakes in Washington. Limnol Oceanogr 3:51–68

    Article  Google Scholar 

  • Auer I, Böhm R, Jurkovic A, Lipa W, Orlik A, Potzmann R et al (2007) HISTALP—historical instrumental climatological surface time series of the greater Alpine region 1760–2003. Int J Climatol 27:17–46

    Article  Google Scholar 

  • Blöschl G, Nester T, Komma J, Parajka J, Perdigão RAP (2013) The June 2013 flood in the Upper Danube Basin, and comparisons with the 2002, 1954 and 1899 floods. Hydrol Earth Syst Sci 17:5197–5212

    Article  Google Scholar 

  • Boehrer B, von Rohden C, Schultze M (2017) Physical features of meromictic lakes: stratification and circulation. In: Gulati RD, Zadereev ES, Degermendzhi AG (eds) Ecology of meromictic lakes, vol 228. Springer, Berlin

    Chapter  Google Scholar 

  • CCME (2011) Canadian water quality guidelines for the protection of aquatic life: chloride. Canadian Council of Ministers of the Environment, Winnipeg

    Google Scholar 

  • Cole JJ, Pace ML (1998) Hydrologic variability of small, Northern Michigan Lakes measured by the addition of tracers. Ecosystems 1:310–320

    Article  Google Scholar 

  • Doerr SM, Effler SW, Whitehead KA, Auer MT, Perkins M, Heidtke TM (1994) Chloride model for polluted Onondaga Lake. Water Res 28:849–861

    Article  CAS  Google Scholar 

  • Dugan HA, Bartlett SL, Burke SM, Doubek JP, Krivak-Tetley FE, Skaff NK et al (2017a) Salting our freshwater lakes. Proc Natl Acad Sci 114:4453–4458

    Article  CAS  Google Scholar 

  • Dugan HA, Summers JC, Skaff NK, Krivak-Tetley FE, Doubek JP, Burke SM et al (2017b) Long-term chloride concentrations in North American and European freshwater lakes. Sci Data 4:170101. https://doi.org/10.1038/sdata.2017.101

    Article  CAS  PubMed  PubMed Central  Google Scholar 

  • Effler SW, Driscroll CT (1986) A chloride budget for Onondaga Lake, New York, U.S.A. Water Air Soil Pollut 27:29–44

    Article  CAS  Google Scholar 

  • Effler SW, Matthews DA (2003) Impacts of soda ash facility on Onondaga lake and the Seneca River, NY. Lake Reserv Manag 19:285–306

    Article  CAS  Google Scholar 

  • Effler SW, Owens EM (1996) Density stratification in Onondaga lake: 1968–1994. Lake Reserv Manag 12:25–33

    Article  CAS  Google Scholar 

  • Effler SW, Auer MT, Johnson N A (1989) Modeling Cl concentraion in Cayuga Lake, USA. Water Air Soil Pollut 44:347–362

    Article  CAS  Google Scholar 

  • EPA (1988) Ambient water quality criteria for chloride. United States Environmental Protection Agency, Washington, DC

    Google Scholar 

  • Evans M, Frick C (2001) The effects of road salts on aquatic ecosystems. National Water Research Institute, Environment Canada, Ottawa, Canada Contribution Series No. 02-308, August 2001

  • Ficker H, Gassner H, Achleitner D, Schabetsberger R (2011) Ectogenic meromixis of Lake Hallstättersee, Austria induced by waste water intrusions from salt mining. Water Air Soil Pollut 218:109–120

    Article  CAS  Google Scholar 

  • Ficker H, Luger M, Gassner H (2017) From dimictic to monomictic: empirical evidence of thermal regime transitions in three deep Alpine lakes in Austria induced by climate change. Freshw Biol 62:1335–1345

    Article  CAS  Google Scholar 

  • Griebler C, Sonntag B, Mindl B, Posch T, Klammer S, Psenner R (2002) Assessment of the ecological integrity of Traunsee (Austria) via analysis of sediments and benthic microbial communities. Water Air Soil Pollut Focus 2:33–62

    Article  CAS  Google Scholar 

  • Hakala A (2004) Meromixis as a part of lake evolution – observations and a revised classification of true meromictic lakes in Finland. Boreal Environ Res 9(1):37–53

    CAS  Google Scholar 

  • Imboden DM, Wüest A (1995) Mixing mechanisms in lakes. In: Lerman A, Imboden DM, Gat JR (eds) Physics and chemistry of lakes. Springer, Berlin

    Google Scholar 

  • ISO 7888:1985, Water quality—determination of electrical conductivity. International Organization for Standardization, Geneva, pp 1–6

    Google Scholar 

  • Jagsch A, Gassner H, Dokulil MT (2002) Long-term changes in environmental variables of Traunsee, an oligotrophic Austrian lake impacted by the salt industry, and two reference sites, Hallstättersee and Attersee. Water Air Soil Pollut Focus 2:9–20

    Article  CAS  Google Scholar 

  • Jones FE, Harris GL (1992) ITS-90 density of water formulation for volumetric standards calibration. J Res Natl Inst Stand Technol 97:335–340

    Article  CAS  Google Scholar 

  • Kaushal SS, Groffman PM, Likens GE, Belt KT, Stack WP, Kelly VR et al (2005) Increases salinization of fresh water in the northeastern United States. Proc Natl Acad Sci 102:13517–13520

    Article  CAS  Google Scholar 

  • Löffler H (1983) Changes of the benthic fauna of the profundal zone of Traunsee (Austria) due to salt mining activities. Hydrobiologia 103:135–139

    Article  Google Scholar 

  • Miller LG, Jellison R, Oremland RS, Culbertson CW (1993) Meromixis in hypersaline Mono Lake, California. 3. Biogeochemical response to stratification and overturn. Limnol Oceanogr 38:1040–1051

    Article  CAS  Google Scholar 

  • Moreira S, Schultze M, Rahn K, Boehrer B (2016) A practical approach to lake water density from electrical conductivity and temperature. Hydrol Earth Syst Sci 20:2975–2986

    Article  Google Scholar 

  • Müller B, Gächter R (2011) Increasing chloride concentrations in Lake Constance: characterization of sources and estimation of loads. Aquat Sci 74:101–112

    Article  Google Scholar 

  • North RP, Livingstone DM (2013) Comparison of linear and cubic spline methods of interpolating lake water column profiles. Limnol Oceanogr 11:213–224

    Article  Google Scholar 

  • North RP, North RL, Livingstone DM, Köster O, Kipfer R (2014) Long-term changes in hypoxia and soluble reactive phosphorus in the hypolimnion of a large temperate lake: consequences of a climate regime shift. Glob Change Biol 20:811–823

    Article  Google Scholar 

  • O’Reilly CM, Sharma S, Gray DK, Hampton SE, Read JS, Rowley RJ et al (2015) Rapid and highly variable warming of lake surface waters around the globe. Geophys Res Lett 42:10773–10781

    Article  Google Scholar 

  • Pechlaner R, Sossau C (1982) Die Ergebnisse der 5-jährigen Studie, Limnologische Untersuchung Traunsee-Traun. Zusammenfassender Bericht Nr 13, Oberösterreichische Landesregierung, Linz

  • Pilotti M, Sinoncelli S, Valerio G (2014) A simple approach to the evaluation of the actual water renewal time of natural stratified lakes. Water Resour Res 50:2830–2849

    Article  Google Scholar 

  • Read JS, Hamilton DP, Jonses ID, Muraoka K, Winslow L, Kroiss R et al (2011) Derivation of lake mixing and stratification indices from high-resolution lake buoy data. Environ Model Softw 26:1325–1336

    Article  Google Scholar 

  • Rimmer A, Aoata Y, Kumagai M, Eckert W (2005) Chemical stratification in thermally stratified lakes: a chloride mass balance model. Limnol Oceanogr 50:147–157

    Article  CAS  Google Scholar 

  • Rogora M, Mosello R, Kamburska L, Salmaso N, Cerasino L, Leoni B et al (2015) Recent trends in chloride and sodium concentrations in the deep subalpine lakes (Northern Italy). Environ Sci Pollut Res 22:19013–19026

    Article  CAS  Google Scholar 

  • Sahoo GB, Forrest AL, Schladow SG, Reuter JE, Coats R, Dettinger M (2015) Climate change impacts on lake thermal dynamics and ecosystem vulnerabilities. Limnol Oceanogr 61:496–507

    Article  Google Scholar 

  • Sanderson B, Perry K, Pedersen T (1986) Vertical diffusion in meromictic Powell lake, British Columbia. J Geophys Res 91:7647–7655

    Article  CAS  Google Scholar 

  • Schwefel R, Gaudard A, Wüest A, Bouffard D (2016) Effects of climate change on deepwater oxygen and winter mixing in a deep lake (Lake Geneva): comparing observational findings and modeling. Water Resour Res 52:8811–8826

    Article  CAS  Google Scholar 

  • Sonntag B, Posch T, Klammer S, Griebler C, Psenner R (2002) Protozooplankton in the deep oligotrophic Traunsee (Austria) influenced by discharges of soda and salt industries. Water Air Soil Pollut Focus 2:211–226

    Article  CAS  Google Scholar 

  • Sossau C (1982) Schichtungs- und Strömungsverhältnisse, Chlorid und Sauerstoff im Traunsee. Limnologische Untersuchung Traunsee-Traun. Bericht Nr 9, Oberösterreichische Landesregierung, Linz

  • Sossau C, Pechlaner R (1988) The regained, but hidden holomixis of the Austrian Lake Traunsee. Verh Internat Ver Limnol 23:74–79

    Google Scholar 

  • Steinhauser G (2008) Cleaner production in the Solvay Process: general strategies and recent developments. J Clean Prod 16:833–841

    Article  Google Scholar 

  • Thies H, Nickus U, Arnold C, Psennner R (2002) A hydrological tracer experiment with LiCl in a high mountain lake. Hydrol Process 16:2329–2337

    Article  Google Scholar 

  • Varekamp JC (2002) Lake contamination models for evolution towards steady state. Papers from Bolsena conference, residence time in lakes: science, management, education. J Limnol 62(Suppl. 1):67–72

    Google Scholar 

  • Wanzenböck J, Gassner H, Lahnsteiner B, Hassan Y, Hauseder G, Doblander C et al (2002) Ecological integrity assessment of lakes using fish communities: an example from Traunsee exposed to intensive fishing and to effluents from the soda industry. Water Air Soil Pollut Focus 2:227–248

    Article  Google Scholar 

  • Winkler LW (1889) Die Löslichkeit des Sauerstoffs in Wasser. Berichte der deutschen chemischen Gesellschaft 22:1764–1774

    Article  Google Scholar 

  • Wüest A, Sommer T, Schmid M, Carpenter JR (2012) Diffusive-type of double diffusion in lakes—a review. In: Environmental fluid mechanics: memorial volume in honour of Prof. Gerhar H. Jirka, IAHR monograph. CRC Press, Boca Raton, pp 271–284

    Google Scholar 

  • Zadereev ES, Gulati RD, Camacho A (2017) Biological and ecological features, trophic structure and energy flow in meromictic lakes. In: Gulati RD, Zadereev ES, Degermendzhi AG (eds) Ecology of meromictic lakes, vol 228. Springer, Berlin

    Google Scholar 

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Acknowledgements

We thank Solvay Österreich GmbH, Salinen Austria AG and the Landesregierung Oberösterreich for extensive long-term monitoring of Traunsee and data acquisition.

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Correspondence to Harald Ficker.

Appendix

Appendix

Temporal and spatial dimensions of sampling profiles

The temporal and spatial resolution of sampling increased steadily over the first ten years of the monitoring program conducted from 1930 to 2016. The long-term records of water temperature, conductivity and chloride concentration predominantly comprise monthly vertical sampling profiles in at least 17 depth layers between surface and lake bottom from the 1950s onwards.

See Figs. 10, 11, 12 and 13.

Fig. 10
figure 10

a Number of temperature profiles per year and b mean number of individual temperature samples per profile. Error bars indicate varying numbers of samples in the profiles during a year

Fig. 11
figure 11

a Number of conductivity profiles per year and b mean number of individual conductivity samples per profile. Error bars indicate varying numbers of samples in the profiles during a year

Fig. 12
figure 12

a Number of chloride profiles per year and b mean number of individual chloride samples per profile. Error bars indicate varying numbers of samples in the profiles during a year

Fig. 13
figure 13

a Number of oxygen profiles per year and b mean number of individual oxygen samples per profile. Error bars indicate varying numbers of samples in the profiles during a year

Linear regression of chloride vs. conductivity measurements

See Fig. 14.

Fig. 14
figure 14

Linear relationship between measured chloride concentrations and measured electrical conductivities in Traunsee between June 1930 and December 2016

Development of daily stability indices of Traunsee between 1930 and 2016

See Fig. 15.

Fig. 15
figure 15

Daily time-series of Schmidt stability indices calculated with temperature data (St) and temperature and conductivity data (Stk) from a June 1930 to December 1959, b January 1960 to December 1989 and c January 1990 to December 2016

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Ficker, H., Luger, M., Pamminger-Lahnsteiner, B. et al. Diluting a salty soup: Impact of long-lasting salt pollution on a deep Alpine lake (Traunsee, Austria) and the downside of recent recovery from salinization. Aquat Sci 81, 7 (2019). https://doi.org/10.1007/s00027-018-0602-3

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