Which Wave Numbers Determine the Thermodynamic Stability of Soft Matter Quasicrystals?

D. J. Ratliff, A. J. Archer, P. Subramanian, and A. M. Rucklidge
Phys. Rev. Lett. 123, 148004 – Published 1 October 2019

Abstract

For soft matter to form quasicrystals an important ingredient is to have two characteristic length scales in the interparticle interactions. To be more precise, for stable quasicrystals, periodic modulations of the local density distribution with two particular wave numbers should be favored, and the ratio of these wave numbers should be close to certain special values. So, for simple models, the answer to the title question is that only these two ingredients are needed. However, for more realistic models, where in principle all wave numbers can be involved, other wave numbers are also important, specifically those of the second and higher reciprocal lattice vectors. We identify features in the particle pair interaction potentials that can suppress or encourage density modes with wave numbers associated with one of the regular crystalline orderings that compete with quasicrystals, enabling either the enhancement or suppression of quasicrystals in a generic class of systems.

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  • Received 15 July 2019

DOI:https://doi.org/10.1103/PhysRevLett.123.148004

© 2019 American Physical Society

Physics Subject Headings (PhySH)

Polymers & Soft MatterNonlinear Dynamics

Authors & Affiliations

D. J. Ratliff1,*, A. J. Archer1,†, P. Subramanian2,3,‡, and A. M. Rucklidge2,§

  • 1Department of Mathematical Sciences and Interdisciplinary Centre for Mathematical Modelling, Loughborough University, Loughborough, Leicestershire LE11 3TU, United Kingdom
  • 2School of Mathematics, University of Leeds, Leeds LS2 9JT, United Kingdom
  • 3Mathematical Institute, University of Oxford, Oxford OX2 6GG, United Kingdom

  • *D.J.Ratliff@lboro.ac.uk
  • A.J.Archer@lboro.ac.uk
  • Priya.Subramanian@maths.ox.ac.uk
  • §A.M.Rucklidge@leeds.ac.uk

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Issue

Vol. 123, Iss. 14 — 4 October 2019

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