Fission product yield measurements using monoenergetic photon beams

Krishichayan, Megha Bhike, C. R. Howell, A. P. Tonchev, and W. Tornow
Phys. Rev. C 100, 014608 – Published 19 July 2019

Abstract

Background: High-accuracy and self-consistent fission product yield (FPY) data are needed to advance microscopic/macroscopic descriptions of the nuclear fission process, to improve the predictive power of phenomenological models, and for applications in nuclear energy, nuclear forensics, and homeland security.

Purpose: In a collaboration between the Triangle Universities Nuclear Laboratory (TUNL), Los Alamos National Laboratory (LANL), and Lawrence Livermore National Laboratory (LLNL), the dependence of a number of cumulative FPYs on the incoming neutron energy has been measured and unexpected energy dependencies of certain fission products have been reported [M. E. Gooden, Nucl. Data Sheets 131, 319 (2016)]. To investigate whether this observation is unique to neutron-induced fission, a program has been initiated to measure FPYs in photon-induced fission.

Method: The photon-induced FPYs were measured by a combination of fission counting using a specially designed dual-fission chamber and γ-ray counting. The measurements were carried out with a monoenergetic photon beam at the HIγS facility. Gamma-ray counting of the activated targets was performed with well-shielded high-purity germanium (HPGe) detectors over a period of two months after irradiation to properly identify the decay history of fission products.

Results: We report on our photofission product yield measurements on U235, U238, and Pu239 using a monoenergetic photon beam of Eγ=13MeV. More than 40 fission products were uniquely identified, and their yield values were computed. The use of the fission chamber with post-activation measurements has provided absolute fission product yield data with minimal uncertainties.

Conclusion: The photon-induced cumulative fission product yields of U235, U238, and Pu239 are compared with previous photon- and neutron-induced fission measurements. In the near future data will be obtained at lower and higher photon energies.

  • Figure
  • Figure
  • Figure
  • Figure
  • Figure
  • Figure
  • Figure
13 More
  • Received 1 March 2019
  • Corrected 19 March 2020

DOI:https://doi.org/10.1103/PhysRevC.100.014608

©2019 American Physical Society

Physics Subject Headings (PhySH)

Nuclear Physics

Corrections

19 March 2020

Correction: A numerical entry in the last column of Table 3 contained a typo and has been fixed.

Authors & Affiliations

Krishichayan1,*, Megha Bhike1, C. R. Howell1, A. P. Tonchev2, and W. Tornow1

  • 1Department of Physics, Duke University, and Triangle Universities Nuclear Laboratory, Durham, North Carolina 27708, USA
  • 2Nuclear and Chemical Sciences Division, Lawrence Livermore National Laboratory, Livermore, California 94550, USA

  • *krishi@tunl.duke.edu; krishichayan@gmail.com

Article Text (Subscription Required)

Click to Expand

References (Subscription Required)

Click to Expand
Issue

Vol. 100, Iss. 1 — July 2019

Reuse & Permissions
Access Options
CHORUS

Article Available via CHORUS

Download Accepted Manuscript
Author publication services for translation and copyediting assistance advertisement

Authorization Required


×
×

Images

×

Sign up to receive regular email alerts from Physical Review C

Log In

Cancel
×

Search


Article Lookup

Paste a citation or DOI

Enter a citation
×