Abstract
We report the results of specific-heat measurements of (x=0, 0.01, 0.02) single crystals in magnetic fields up to 15 T. For x=0.02, a sharp transition was observed at the Néel temperature =4.8 K, which is almost constant up to 15 T. For x=0.01, two broad transitions were observed at the spin-Peierls transition temperature =10.8 K and =2.5 K in zero magnetic field. The antiferromagnetic state is changed drastically by the magnetic field and the magnetic-field-induced magnetic state was observed by specific-heat measurements. The magnetic phase diagram of was determined from specific-heat, thermal-expansion, and magnetization measurements.
DOI:https://doi.org/10.1103/PhysRevB.55.R6125
©1997 American Physical Society