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Unusual antiferromagnetic state in Si-doped CuGeO3ssingle crystals studied by specific-heat measurements in magnetic fields

M. Hiroi, T. Hamamoto, M. Sera, H. Nojiri, N. Kobayashi, M. Motokawa, O. Fujita, A. Ogiwara, and J. Akimitsu
Phys. Rev. B 55, R6125(R) – Published 1 March 1997
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Abstract

We report the results of specific-heat measurements of CuGe1xSixO3 (x=0, 0.01, 0.02) single crystals in magnetic fields up to 15 T. For x=0.02, a sharp transition was observed at the Néel temperature TN=4.8 K, which is almost constant up to 15 T. For x=0.01, two broad transitions were observed at the spin-Peierls transition temperature TSP=10.8 K and TN=2.5 K in zero magnetic field. The antiferromagnetic state is changed drastically by the magnetic field and the magnetic-field-induced magnetic state was observed by specific-heat measurements. The magnetic phase diagram of CuGe1xSixO3 was determined from specific-heat, thermal-expansion, and magnetization measurements.

    DOI:https://doi.org/10.1103/PhysRevB.55.R6125

    ©1997 American Physical Society

    Authors & Affiliations

    M. Hiroi, T. Hamamoto, M. Sera, H. Nojiri, N. Kobayashi, and M. Motokawa

    • Institute for Materials Research, Tohoku University, Katahira, Aoba-ku, Sendai 980-77, Japan

    O. Fujita, A. Ogiwara, and J. Akimitsu

    • Department of Physics, Aoyama Gakuin University, Chitosedai, Setagaya-ku, Tokyo 157, Japan

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    Vol. 55, Iss. 10 — 1 March 1997

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