Absence of half-metallicity in defect-free digital magnetic heterostructures δ-doped with Cr and Mn

F. Beiuşeanu, C. Horea, E.-V. Macocian, T. Jurcuţ, L. Vitos, and L. Chioncel
Phys. Rev. B 83, 125107 – Published 18 March 2011

Abstract

We present the results of combined density functional and many-body calculations of the electronic and magnetic properties of the defect-free digital ferromagnetic heterostructures obtained by doping GaAs with Cr and Mn. While the local-density approximation +U predicts half-metallicity in these defect-free delta-doped heterostructures, we demonstrate that local many-body correlations captured by dynamical mean-field theory induce within the minority-spin channel nonquasiparticle states just above EF. As a consequence of the existence of these many-body states the half-metallic gap is closed and the carriers’ spin polarization is significantly reduced. Below the Fermi level the minority-spin highest valence states are found to localize more on the GaAs layers, being independent of the type of electronic correlations considered. Thus, our results confirm the confinement of carriers in these delta-doped heterostructures, having a spin polarization that follows a different temperature dependence than the magnetization. We suggest that polarized hot-electron photoluminescence experiments might uncover evidence for the existence of many-body states within the minority-spin channel and elucidate their finite-temperature behavior.

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  • Received 1 October 2010

DOI:https://doi.org/10.1103/PhysRevB.83.125107

©2011 American Physical Society

Authors & Affiliations

F. Beiuşeanu1, C. Horea1, E.-V. Macocian1, T. Jurcuţ1, L. Vitos2,3,4, and L. Chioncel5,6

  • 1Department of Physics, University of Oradea, RO-410087 Oradea, Romania
  • 2Applied Materials Physics, Department of Materials Science and Engineering, Royal Institute of Technology, Stockholm SE-100 44, Sweden
  • 3Department of Physics and Materials Science, Uppsala University, PO Box 516, SE-75120 Uppsala, Sweden
  • 4Research Institute for Solid State Physics and Optics, Budapest H-1525, PO Box 49, Hungary
  • 5Augsburg Center for Innovative Technologies, University of Augsburg, D-86135 Augsburg, Germany
  • 6Theoretical Physics III, Center for Electronic Correlations and Magnetism, Institute of Physics, University of Augsburg, D-86135 Augsburg, Germany

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Vol. 83, Iss. 12 — 15 March 2011

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