Nonperturbative computation of the time-resolved formation of the profile of autoionizing states as a function of the intensity and duration of ultrashort pulses

Th. Mercouris, Y. Komninos, and C. A. Nicolaides
Phys. Rev. A 83, 015403 – Published 24 January 2011

Abstract

By solving the time-dependent Schrödinger equation nonperturbatively by the state-specific expansion approach, we have obtained reliable results showing the dependence of the formation of the excitation profile of the autoionizing state He 2s2p1Po for Gaussian pulses of intensities in the range I1010W/cm2 to I1015W/cm2, and of duration 100–2 fs. Conclusions are drawn as regards the breakdown of first-order time-dependent perturbation theory.

  • Figure
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  • Received 2 December 2010

DOI:https://doi.org/10.1103/PhysRevA.83.015403

© 2011 American Physical Society

Authors & Affiliations

Th. Mercouris*, Y. Komninos, and C. A. Nicolaides

  • Theoretical and Physical Chemistry Institute, Hellenic Research Foundation, 48 Vasileos Constantinou Avenue, Athens, GR-11635 Greece

  • *thmerc@eie.gr
  • ykomn@eie.gr
  • caan@eie.gr

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Vol. 83, Iss. 1 — January 2011

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