Abstract
By solving the time-dependent Schrödinger equation nonperturbatively by the state-specific expansion approach, we have obtained reliable results showing the dependence of the formation of the excitation profile of the autoionizing state He for Gaussian pulses of intensities in the range to , and of duration 100–2 fs. Conclusions are drawn as regards the breakdown of first-order time-dependent perturbation theory.
- Received 2 December 2010
DOI:https://doi.org/10.1103/PhysRevA.83.015403
© 2011 American Physical Society