Abstract
The stochastic variational method is applied to excitonic formations within semiconducting transition metal dichalcogenides using a correlated Gaussian basis. The energy and structure of two- to six-particle systems are investigated along with their dependence on the effective screening length of the two-dimensional Keldysh potential and the electron-hole effective mass ratio. Excited state biexcitons are shown to be bound, with binding energies of the state showing good agreement with experimental measurements of biexciton binding energies. Ground and newly discussed excited state exciton-trions are predicted to be bound and their structures are investigated.
- Received 14 January 2016
- Revised 25 February 2016
DOI:https://doi.org/10.1103/PhysRevB.93.125423
©2016 American Physical Society