Incommensurate to commensurate antiferromagnetism in CeRhAl4Si2: An Al27 NMR study

H. Sakai, T. Hattori, Y. Tokunaga, S. Kambe, N. J. Ghimire, F. Ronning, E. D. Bauer, and J. D. Thompson
Phys. Rev. B 93, 014402 – Published 4 January 2016

Abstract

Al27 nuclear magnetic resonance (NMR) experiments have been performed on a single crystal of CeRhAl4Si2, which is an antiferromagnetic Kondo-lattice compound with successive antiferromagnetic transitions of TN1=14 K and TN2=9 K at zero external field. In the paramagnetic state, the Knight shifts, quadrupolar frequency, and asymmetric parameter of electrical field gradient on the Al sites have been determined, which have local orthorhombic symmetry. The transferred hyperfine coupling constants are also determined. Analysis of the NMR spectra indicates that a commensurate antiferromagnetic structure exists below TN2, but an incommensurate modulation of antiferromagnetic moments is present in the antiferromagnetic state between TN1 and TN2. The spin-lattice relaxation rate suggests that the 4f electrons behave as local moments at temperatures above TN1.

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  • Received 24 September 2015
  • Revised 6 December 2015

DOI:https://doi.org/10.1103/PhysRevB.93.014402

©2016 American Physical Society

Authors & Affiliations

H. Sakai*, T. Hattori, Y. Tokunaga, and S. Kambe

  • Advanced Science Research Center, Japan Atomic Energy Agency, Tokai, Ibaraki, 319-1195, Japan

N. J. Ghimire, F. Ronning, E. D. Bauer, and J. D. Thompson

  • Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA

  • *sakai.hironori@jaea.go.jp
  • Present address: Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439, USA.

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Vol. 93, Iss. 1 — 1 January 2016

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