Thermodynamic consistency of the charge response in dynamical mean-field based approaches

Erik G. C. P. van Loon, Hartmut Hafermann, Alexander I. Lichtenstein, and Mikhail I. Katsnelson
Phys. Rev. B 92, 085106 – Published 4 August 2015

Abstract

We consider the thermodynamic consistency of the charge response function in the (extended) Hubbard model. In dynamical mean-field theory (DMFT), thermodynamic consistency is preserved. We prove that the static, homogeneous DMFT susceptibility is consistent as long as vertex corrections obtained from the two-particle impurity correlation function are included. In the presence of a nonlocal interaction, the problem may be treated within extended DMFT (EDMFT), or its diagrammatic extension, the dual boson approach. We show that here maintaining thermodynamic consistency requires knowledge of three- and four-particle impurity correlation functions, which are typically neglected. Nevertheless, the dual boson approximation to the response is remarkably close to consistency. This holds even when two-particle vertex corrections are neglected. EDMFT is consistent only in the strongly correlated regime and near half-filling, where the physics is predominantly local.

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  • Received 21 May 2015

DOI:https://doi.org/10.1103/PhysRevB.92.085106

©2015 American Physical Society

Authors & Affiliations

Erik G. C. P. van Loon1,*, Hartmut Hafermann2,†, Alexander I. Lichtenstein3, and Mikhail I. Katsnelson1

  • 1Radboud University, Institute for Molecules and Materials, NL-6525 AJ Nijmegen, The Netherlands
  • 2Mathematical and Algorithmic Sciences Lab, France Research Center, Huawei Technologies Co. Ltd., 92100 Boulogne Billancourt, France
  • 3I. Institut für Theoretische Physik, Universität Hamburg, Jungiusstraße 9, D-20355 Hamburg, Germany

  • *evloon@science.ru.nl
  • Part of this work was conducted while the author was at Institut de Physique Théorique (IPhT), CEA, CNRS, 91191 Gif-sur-Yvette, France.

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Vol. 92, Iss. 8 — 15 August 2015

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