Successive magnetic transitions and static magnetic order in RCoAsO (R=La, Ce, Pr, Nd, Sm, Gd) confirmed by muon-spin rotation and relaxation

Jun Sugiyama, Martin Månsson, Oren Ofer, Kazuya Kamazawa, Masashi Harada, Daniel Andreica, Alex Amato, Jess H. Brewer, Eduardo J. Ansaldo, Hiroto Ohta, Chishiro Michioka, and Kazuyoshi Yoshimura
Phys. Rev. B 84, 184421 – Published 16 November 2011

Abstract

The presence of antiferromagnetic (AF) order seems to be a common feature for the parent compounds of cuprate as well as some pnictide high-temperature superconductors. In order to search for antiferromagnetic order in the closely related rare-earth cobalt arsenic oxides (RCoAsO), we have measured muon-spin rotation and relaxation (μ+SR) spectra on a series of powder samples with R=La, Ce, Pr, Nd, Sm, and Gd. It was found that, besides GdCoAsO, all the other five compounds enter into a static ferromagnetic ordered phase below around 70 K (=TC), while additional transitions into a static AF ordered phase were found for NdCoAsO and SmCoAsO. For GdCoAsO, a static ferrimagnetic phase appeared below 60.5 K and then an incommensurate spin-density-wave ordered phase followed below 3.2 K. The AF spin structure was also found to strongly depend on R.

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  • Received 24 June 2011

DOI:https://doi.org/10.1103/PhysRevB.84.184421

©2011 American Physical Society

Authors & Affiliations

Jun Sugiyama1,*, Martin Månsson2, Oren Ofer3, Kazuya Kamazawa1,†, Masashi Harada1, Daniel Andreica4, Alex Amato5, Jess H. Brewer3,6, Eduardo J. Ansaldo3, Hiroto Ohta7,‡, Chishiro Michioka7, and Kazuyoshi Yoshimura7

  • 1Toyota Central Research and Development Laboratories Inc., Nagakute, Aichi 480-1192, Japan
  • 2Laboratory for Solid State Physics, ETH Zürich, CH-8093 Zürich, Switzerland
  • 3TRIUMF, 4004 Wesbrook Mall, Vancouver, British Columbia, Canada V6T 2A3
  • 4Faculty of Physics, Babes-Bolyai University, 3400 Cluj-Napoca, Romania
  • 5Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institut, CH-5232 Villigen PSI, Switzerland
  • 6Department of Physics and Astronomy, University of British Columbia, Vancouver, British Columbia, Canada V6T 1Z1
  • 7Division of Chemistry, Faculty of Science, Kyoto University, Kyoto 606-8502, Japan

  • *e0589@mosk.tytlabs.co.jp
  • Present address: Comprehensive Research Organization for Science and Society (CROSS), Tokai, Ibaraki 319-1106, Japan.
  • Present address: Faculty of Engineering, Tokyo University of Agriculture and Technology, Koganei, Tokyo 184-8588, Japan.

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Vol. 84, Iss. 18 — 1 November 2011

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