Is Haldane's singlet—triplet transition found in CsNiCl3?

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Abstract

We investigated magnetic excitations in CsNiCl3 in magnetic fields up to 9.5 T by means of inelastic unpolarised neutron scattering. Assuming a threefold splitting at Q=(001) as observed in a previous polarised experiment at low fields, we find similar field behaviour at 2 and 7 K. The field dependence of the upper mode at Q=(0.39 0.39 1),T=2 K, could point to a longitudinal character of the excitation as predicted by Affleck.

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