Abstract
Whether thermokinetic data obtained on model large single crystals at low surface coverage can be used successfully to calculate yields on real catalysts at high surface coverage is a question that is considered in the conjecture presented in this note.
Similar content being viewed by others
References
J.A. Dumesic, B.A. Milligan, L.A. Greppi, V.R. Balse, K.T. Sarnowski, C.E. Beall, T. Kataoka, D.F. Rudd and A.A. Trevino, Ind. Eng. Chem. REs. 26(7) (1987) 1399.
R. Aris, A.T. Bell, M. Boudart, N.Y. Chen, B.C. Gates, W.O. Haag, G.A. Somorjai and J. Wei,Catalyst Design — Progress and Perspectives, ed. L.L. Hegedus (Wiley-Interscience, New York, 1987).
M. Boudart and G. Djéga-Mariadassou,Kinetics of Heterogeneous Catalytic Reactions (Princeton University Press, Princeton, N.J., 1984).
S. Weller, Adv. Chem. Ser. No. 148 (1975) 156.
M. Boudart, I&EC Fundamentals 25 (1986) 656.
M. Boudart, CHEMTECH (Nov. 1986) p. 688.
S.H. Oh, G.B. Fisher, J.E. Carpenter and D.W. Goodman, J. Catal. 100 (1986) 360.
M. Bowker, I.B. Parker and K.C. Waugh, Appl. Catal. 14 (1985) 101.
G. Ertl,Catalysis — Science and Technology, eds. J.R. Anderson and M. Boudart, Vol. 4 (Springer-Verlag, Heidelberg, 1983) p. 209.
P. Stoltze and J.K. Nørskov, Phys. Rev. Letters 55 (1985) 2502.
P. Stoltze and J.K. Nørskov, J. Vac. Sci. Technol. A5 (1987) 581.
P. Stoltze, Physica Scripta 36 (1987) 824.
M.I. Temkin and V. Pyzhev, Acta Physicochim. URSS 12 (1940) 489.
M. Boudart, Industrie Chimique Belge 19 (1954) 489.
M. Boudart and F. Rumpf, Reaction Kinetics and Catalysis Letters, in press.
Author information
Authors and Affiliations
Rights and permissions
About this article
Cite this article
Boudart, M. Kinetics assisted design of catalysts. Catal Lett 1, 21–25 (1988). https://doi.org/10.1007/BF00765349
Issue Date:
DOI: https://doi.org/10.1007/BF00765349