Hostname: page-component-848d4c4894-m9kch Total loading time: 0 Render date: 2024-06-02T16:50:31.627Z Has data issue: false hasContentIssue false

Tritium and 14C in Tree Rings of the Last Three Decades

Published online by Cambridge University Press:  18 July 2016

Kristóf Kozák
Affiliation:
Institute of Isotopes of the Hungarian Academy of Sciences POB 77, 1525 Budapest, Hungary
Bogomil Obelić
Affiliation:
Institute of Isotopes of the Hungarian Academy of Sciences POB 77, 1525 Budapest, Hungary
Nada Horvatinčić
Affiliation:
Institute of Isotopes of the Hungarian Academy of Sciences POB 77, 1525 Budapest, Hungary
Rights & Permissions [Opens in a new window]

Abstract

Core share and HTML view are not available for this content. However, as you have access to this content, a full PDF is available via the ‘Save PDF’ action button.

Tree rings spanning the past three decades were collected from Picea spp trees grown in Matra, northern Hungary. Cellulose was prepared from the wood and samples were separately combusted for tritium and 14C analyses. Methane was synthesized from CO2 obtained by sample combustion via catalytic reaction with tritium-free hydrogen. 14C activity was measured by proportional counter. The exchangeable tritium was removed from cellulose samples used for tritium analysis. Water samples produced by combustion were measured by liquid scintillation counting. The distribution of tritium and 14C activities in tree rings are shown for years 1956–1986. Results are compared with published data on global-scale distribution of 14C and HTO. A comparison of tritium activity in precipitation and wine samples from the same region is presented.

Type
III. Global 14C Variations
Copyright
Copyright © The American Journal of Science 

References

Brown, R M, 1979, Environmental tritium in trees, in Behaviour of tritium in the environment, Proc: IAEA, Vienna, ser STI/PUB/498, p 405418.Google Scholar
Dai, K and Fan, C Y, 1986, Bomb produced 14C content in tree rings grown at different latitudes, in Stuiver, M and Kra, R S, eds, Internatl 14C conf, 12th, Proc: Radiocarbon, v 28, no. 2A, p 346349.Google Scholar
Fairhall, A W and Young, J A, 1970, Radiocarbon in the environment, in Radionuclides in the environment: Advances in chem ser, no. 93, p 401418.Google Scholar
Green, J W, 1963, Wood cellulose, in Whistler, R L, ed, Methods in carbohydrate chemistry: New York, Academic Press, v III, p 921.Google Scholar
Hertelendi, E and Csongor, E, 1982, Anthropogenic 14C excess in the troposphere between 1951 and 1978 measured in tree-rings: Radiochem Radioanal Letters, v 56, p 103110.Google Scholar
IAEA, 1981, Statistical treatment of environmental isotope data in precipitation: Tech repts ser no. 206, 255 p.Google Scholar
IAEA, 1983, Environmental isotope data no. 7, World survey of isotope concentration in precipitation (1976–1979): Tech repts ser no. 226, 241 p.Google Scholar
IAEA, 1986, Environmental isotope data no. 8, World survey of isotope concentration in precipitation (1980–1983): Tech repts ser no. 264, 184 p.Google Scholar
Kigoshi, K and Tomikura, Y, 1961, Tritium and carbon-14 in the tree-rings: Bull Chem Soc Japan, v 34, p 17381739.Google Scholar
Kozák, K, 1982, Analysis of tritium in tree-rings: Acta Phys Hungary, v 52, p 429434.Google Scholar
Kozák, K and Biro, T, 1984, Reconstruction of environmental tritium levels from wine analysis: Health Phys, v 46, p 193203.Google Scholar
Kozák, K, Biró, T, Golder, F, Rajner, V, Rank, D and Staudner, F, 1986, Evaluation of anomalous local tritium fallout by tree ring analysis: Acta Phys Hungary, v 59, p 5962.Google Scholar
Levin, I, Münnich, K O and Weiss, W, 1980, The effect of anthropogenic CO2 and 14C sources on the distribution of 14C in the atmosphere, in Stuiver, M and Kra, R S, eds, Internatl 14C conf, 10th, Proc: Radiocarbon, v 22, no. 2, p 379391.Google Scholar
Mann, J, 1971, Deuteration and tritiation in Bikales, N M and Segal, L, eds, Cellulose and cellulose derivatives, Pt IV: New York, Wiley Interscience, p 89116.Google Scholar
Nydal, R and Lövseth, K, 1970, Prospective decrease in atmospheric radiocarbon: Jour Geophys Research, v 75, p 22712278.CrossRefGoogle Scholar
Obelić, B, Krajcar-Bronić, I, Srdoč, D and Horvatinčić, N, 1986, Environmental 14C levels around the 632 MWe nuclear power plant in Yugoslavia, in Stuiver, M and Kra, R A, ed, Internatl 14C conf, 12th, Proc: Radiocarbon, v 28, no. 2A, p 644648.Google Scholar
Schell, W R, Sauzay, C and Payne, B R, 1974, World distribution of environmental tritium, in Symposium on physical behaviour of the radioactive contaminants in the atmosphere, Proc: IAEA, Vienna, p 375396.Google Scholar
Srdoč, D, Breyer, B and Sliepčević, A, 1971, Ruder Bošković Institute radiocarbon measurements I: Radiocarbon, v 13, no. 1, p 135140.CrossRefGoogle Scholar
Stuiver, M and Polach, H, 1977, Discussion: Reporting of 14C data: Radiocarbon, v 19, no. 3, p 355363.Google Scholar
Tans, P P, de Jong, A F M and Mook, W G, 1978, Chemical pretreatment and radial flow of 14C in tree rings: Nature, v 271, p 234235.Google Scholar
Wadehra, I L and Manley, R, 1965, Irreversible exchange of hydrogen in the drying of cellulose at high temperatures: Jour Applied Polymer Sci, v 9, p 34993502.Google Scholar