Dynamical Correlation in Double Excitations of Helium Studied by High-Resolution and Angular-Resolved Fast-Electron Energy-Loss Spectroscopy in Absolute Measurements

Xiao-jing Liu, Lin-fan Zhu, Zhen-sheng Yuan, Wen-bin Li, Hua-dong Cheng, Yu-ping Huang, Zhi-ping Zhong, Ke-zun Xu, and Jia-Ming Li
Phys. Rev. Lett. 91, 193203 – Published 6 November 2003

Abstract

The momentum transfer dependence of fundamental double excitation processes of helium is studied by absolute measurements using an angular resolved fast-electron energy loss spectrometer with high energy resolution. It elucidates the dynamical correlations, in terms of internal correlation quantum numbers, K, T, and A. The Fano profile parameters q, fa, ρ2, f, and S of doubly excited states (21,0)2+Se1, (21,0)2+De1, and (20,1)2+Po1 are reported as functions of momentum transfer K2. Qualitative analysis is given for the states of (21,0)2+Se1 and (21,0)2+Se1.

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  • Received 6 February 2003

DOI:https://doi.org/10.1103/PhysRevLett.91.193203

©2003 American Physical Society

Authors & Affiliations

Xiao-jing Liu1,*, Lin-fan Zhu1, Zhen-sheng Yuan1, Wen-bin Li1, Hua-dong Cheng1, Yu-ping Huang1, Zhi-ping Zhong2, Ke-zun Xu1, and Jia-Ming Li3

  • 1Laboratory of Bond-Selective Chemistry, Department of Modern Physics, University of Science and Technology of China, Hefei, Anhui, 230027, China
  • 2Department of Physics, The Graduate School of the Chinese Academy of Science, P.O. Box 3908, Beijing 100039, China
  • 3Department of Physics, Center of Atomic and Molecular Nanosciences, Tsinghua University, Beijing 100084, China

  • *Electronic address: xjliu@ustc.edu.cn

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Issue

Vol. 91, Iss. 19 — 7 November 2003

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