Abstract
We have performed high-field multifrequency electron spin resonance and magnetization measurements in magnetic field up to about 53 T on single crystals of a multiferroic triangular-lattice antiferromagnet . We observed that one of the resonance modes showed a discontinuous change around 5.3 T for , where the system undergoes a first-order phase transition accompanying a remarkable magnetoelectric effect. We explain the observed anomaly quantitatively in terms of the spiral-plane flop, considering a distorted triangular-lattice model with two kinds of antiferromagnetic in-plane exchange interactions and rhombic anisotropy.
- Received 29 September 2009
DOI:https://doi.org/10.1103/PhysRevB.81.033104
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