Spin Fluctuations of Paramagnetic Rh Clusters Revealed by X-Ray Magnetic Circular Dichroism

V. M. T. S. Barthem, A. Rogalev, F. Wilhelm, M. M. Sant’Anna, S. L. A. Mello, Y. Zhang, P. Bayle-Guillemaud, and D. Givord
Phys. Rev. Lett. 109, 197204 – Published 9 November 2012
PDFHTMLExport Citation

Abstract

The magnetic moment induced on Rh atoms, forming 1.6 nm average diameter clusters, embedded in an Al2O3 matrix, has been determined using x-ray magnetic circular dichroism measurements. The magnetic moment varies linearly with the applied magnetic field. At 2.3 K and under 17 T, the spin magnetic moment amounts to 0.067(2)μB/Rh atom. The orbital moment does not exceed 2% of the spin moment. The susceptibility is highly temperature dependent. This is in agreement with a prediction due to Moriya and Kawabata, that in itinerant electron systems, close to the onset of magnetism, the renormalization of the magnetic susceptibility by electron correlations, leads to a Curie-like behavior.

  • Figure
  • Figure
  • Figure
  • Figure
  • Received 15 March 2012

DOI:https://doi.org/10.1103/PhysRevLett.109.197204

© 2012 American Physical Society

Authors & Affiliations

V. M. T. S. Barthem1, A. Rogalev2, F. Wilhelm2, M. M. Sant’Anna1, S. L. A. Mello1, Y. Zhang3, P. Bayle-Guillemaud4, and D. Givord1,3

  • 1Instituto de Física, Universidade Federal do Rio de Janeiro, 21941-972 Rio de Janeiro, Brazil
  • 2European Synchrotron Radiation Facility, BP 220, F-38043 Grenoble, France
  • 3Institut Néel, CNRS/UJF, BP 166, 38042 Grenoble cedex 9, France
  • 4CEA-INAC/UJF, SP2M, LEMMA, Minatec Grenoble, F-38054, France

Article Text (Subscription Required)

Click to Expand

Supplemental Material (Subscription Required)

Click to Expand

References (Subscription Required)

Click to Expand
Issue

Vol. 109, Iss. 19 — 9 November 2012

Reuse & Permissions
Access Options
Author publication services for translation and copyediting assistance advertisement

Authorization Required


×
×

Images

×

Sign up to receive regular email alerts from Physical Review Letters

Log In

Cancel
×

Search


Article Lookup

Paste a citation or DOI

Enter a citation
×