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Nitrate concentrations in snow from remote areas: implication for the global NO x flux

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Abstract

Increased emissions of nitrogen compounds to the atmosphere by human activities have been well documented. However, in order to better quantify these anthropogenic emissions, better knowledge of natural emissions rates must be known. In addition, variation in natural emissions through time should be documented. In this note we present data collected and/or analyzed by us for NO3 in recent snow from remote regions of the world. We also summarize existing data sets from other remote regions. This is done to establish a better understanding of NO3 deposition rates in these regions as well as to add more information to our global understanding of NO3 deposition.

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References

  • Allen B, Mayewski PA, Lyons WB & Spencer MJ (1985) Glaciochemical studies and estimated net mass balances for Rennick Glacier area, Antarctica, Annl. Glaciol. 7: 1–6

    Google Scholar 

  • Aristarain AJ, Delmas RJ & Briat M (1982) Snow chemistry of James Ross Island (Antarctic Peninsula). J. Geophys. Res. 87: 11004–11012

    Google Scholar 

  • Barrie LA (1985) Scavenging ratios, wet deposition and in-cloud oxidation: An application to the oxides of sulphur and nitrogen. J. Geophys. Res. 90: 5789–5799

    Google Scholar 

  • Bowden WB (1986) Gaseous nitrogen emissions from undisturbed terrestrial ecosystems: An assessment of their impacts on local and global nitrogen budgets. Biogeochem. 28: 249–280

    Google Scholar 

  • Bowden WB & Bormann FH (1986) Transport and loss of nitrous oxide in soil water after forest clear-cutting. Science 233: 867–869

    Google Scholar 

  • Butler D, Lyons WB, Hassinger J & Mayewski PA (1980) Shallow core snow chemistry of Athabasca Glacier, Alberta. Can. J. Earth Sci. 17: 278–282

    Google Scholar 

  • Church TM, Galloway JN, Jickells TD & Knap AH (1982) The chemistry of western Atlantic precipitation of the mid-Atlantic coast and on Bermuda. J. Geophys. Res. 87: 11013–11018

    Google Scholar 

  • Delmas R, Briat M & Legrand M (1982) Chemistry of South Polar snow, J. Geophys. Res. 87: 4314–4318

    Google Scholar 

  • Finkel RC, Langway CC & Clausen HB (1986) Changes in atmospheric chemistry at Dye 3, Greenland. J. Geophys. Res. 91: 9849–9856

    Google Scholar 

  • Firestone MK, Firestone RB & Tiedje JM (1980) Nitrous oxide from soil denitrification: Factors controlling its biological production. Science 208: 749–751

    CAS  Google Scholar 

  • Galbally IE (1985) Nitrogen emission. In Galloway JN, Charlson RJ, Andreae MO & Rodhe H (Eds) The Biogeochemical Cycling of Sulfur and Nitrogen in the Remote Atmosphere, NATO ASI Series, Vol. 159 (pp 27–54) Dordrecht

  • Galloway JN & Likens GE (1981) Acid precipitation: The importance of nitric acid. Atmos. Environ. 15: 1081–1087

    Google Scholar 

  • Galloway JN, Likens GE, Keene WC & Miller JM (1982) The composition of precipitation in remote areas of the world. J. Geophys. Res. 87: 8771–8786

    Google Scholar 

  • Ganapathy R (1983). The Tunguska explosion of 1908: Discovery of meteoritic debris near the explosion site and at the South Pole. Science 220: 1158–1161

    Google Scholar 

  • Harding D & Miller JM (1982) The influence on rain chemistry of the Hawaiian volcano Kilauea. J. Geophys. Res. 87: 1225–1230

    Google Scholar 

  • Hendry CD, Berish CW & Edgerton ES (1984) Precipitation chemistry at Turrialba, Costa Rica. Water Res. Res. 20: 1677–1684

    Google Scholar 

  • Herron MM (1982) Impurity sources of F, Cl, NO3 and SO4 = in Greenland and Antarctic precipitation. J. Geophys. Res. 87: 3052–3060

    Google Scholar 

  • Holdsworth G and Peake E (1985) Acid content of snow from a mid-troposphere sampling site on Mount Logan, Yukon Territory, Canada. Ann. Glaciol. 7: 153–160

    Google Scholar 

  • Ivey JP, Davies DM, Morgan V & Ayers GP (1986) Methanesulphonate in Antarctic ice. Tellus 38B: 375–379

    Google Scholar 

  • Jenkins MD, Drever JI, Reider RG & Buchanan T (1987) Chemical composition of fresh snow on Mt. Everest. J. Geophys. Res. 92: 10999–11002

    Google Scholar 

  • Johnson N & Parnell RA (1986) Composition, distribution and neutralization of ‘acid rain’ derived from Masaya volcano, Nicaragua. Tellus 38B: 106–117

    Google Scholar 

  • Jouzel J, Merlivat L, Pourchet M & Lorius C (1979) A continuous record of artificial tritium fallout at the South Pole (1954–1978). Earth Planet. Sci. Lett. 45: 188–200

    Google Scholar 

  • Kauer JW (1986) Chloride, nitrate and sulfate stratigraphy in the annual snowpack near Shrine Pass, Colorado. (MSc. thesis, University of New Hampshire)

  • Laird LB, Taylor HE & Kennedy VC (1986) Snow chemistry of the Cascade-Sierra Nevada Mountains. Environ. Sci. Tech. 20: 275–290

    Google Scholar 

  • Legrand MR (1987) Chemistry of Antarctic Snow and Ice. J. de Physique 48: C1-77–C1-86

  • Legrand MR & Delmas RJ (1984) The ionic balance of Antarctic snow: A 10-year detailed record. Atmos. Environ. 18: 1867–1874

    Google Scholar 

  • Legrand M, deAngelis M & Delmas RJ (1984) Ion chromatographic determination of common ions at ultratrace levels in Antarctic snow and ice. Anal. Chim. Acta 54: 1336–1349

    Google Scholar 

  • Lewis WM (1981) Precipitation chemistry and nutrient loading by precipitation in a tropical watershed. Water Res. Res. 17: 169–181

    Google Scholar 

  • Logan JA (1983) Nitrogen oxides in the troposphere: Global and regional budgets. J. Geophys. Res. 88: 10785–10807

    Google Scholar 

  • Lyons WB & Mayewski PA (1983) Nitrate plus nitrite concentrations in a Himalayan ice core. Geophys. Res. Lett. 10: 1160–1163

    Google Scholar 

  • Lyons WB, Mayewski PA, Thompson LG & Allen B (1985). The glaciochemistry of snowpits from Quelccaya Ice Cap, Peru, 1982. Ann. Glaciol. 7: 84–88

    Google Scholar 

  • Martikainen PJ (1985) Nitrous oxide emission associated with autotrophic ammonium oxidation in acid coniferous forest soil. Appl. Environ. Micro. 50: 1519–1525

    Google Scholar 

  • Mayewski PA and Lyons WB (1982) Source and climatic implication of the reactive iron and reactives silicate concentrations found in a core from Meserve Glacier, Antarctica. Geophys. Res. Lett. 9: 190–192

    Google Scholar 

  • Mayewski PA, Lyons WB & Ahmad N (1983) Chemical composition of a high altitude fresh snowfall in the Ladakh Himalayas. Geophys. Res. Lett. 10: 105–108

    Google Scholar 

  • Mayewski PA, Lyons WB, Ahmad N, Smith G & Pourchet M (1984) Interpretation of the chemical and physical time-series retrieved from Sentik Glacier, Ladakh Himalaya, India. J. Glaciol. 30: 66–76

    Google Scholar 

  • Mayewski PA, Lyons WB, Spencer MJ, Twickler M, Dansgaard W, Koci B, Davidson CI & Honrath RE (1986a). Sulfate and nitrate concentration from a South Greenland ice core, Science 232: 975–977

    Google Scholar 

  • Mayewski PA, Lyons WB, Spencer MJ & Clayton JL (1986b) Snow chemistry from Xixabangma, Tibet, J. Glaciol. 32: 542–543

    Google Scholar 

  • Mayewski PA, Spencer MJ, Lyons WB & Twickler MS (1987) Seasonal and spatial trends in South Greenland snow chemistry. Atmos. Environ. 21: 863–869

    Google Scholar 

  • Meanhaut W, Zoller WH & Coles DB (1979) Radionuclides in the South Pole atmosphere. J. Geophys. Res. 84: 3131–3138

    Google Scholar 

  • Mooney HA, Vitousek PM & Matson PA (1987) Exchange of materials between terrestrial ecosystems and the atmosphere. Science 238: 926–932

    Google Scholar 

  • Mulvaney R & Peel DA (1988) Anions and cations in ice cores from Dolleman Island and the Palmer Land plateau, Antarctic Penninsula. Ann. Glaciol. 10: 121–125

    Google Scholar 

  • Neftel A, Beer J, Oeschger J, Zurchev F & Finkel RC (1985) Sulphate and nitrate concentrations in snow from South Greenland 1895–1978. Nature 314: 611–613

    Google Scholar 

  • Parker BC, Zeller EJ & Gow AJ (1982) Nitrate fluctuations in Antarctic snow and firn: Potential sources and mechanisms of formation. Ann. Glaciol. 3: 243–248

    Google Scholar 

  • Pourchet M, Pinglot F & Lorius C (1983) Some meteorological applications of radioactive fallout measurements in Antarctic snows. J. Geophys. Res. 88: 6013–6020

    Google Scholar 

  • Prospero JM, Savoie DL, Nees RT, Duce RA & Merrill J (1985) Particulate sulfate and nitrate in the boundary layer over the north Pacific Ocean. J. Geophys. Res. 90: 10586–10596

    Google Scholar 

  • Pszenny AAP & Duce RA (1982) Atmospheric deposition of nitrate at Samoa. EOS 63: 987

    Google Scholar 

  • Pszenny AAP & Duce RA (1986) Wet and dry deposition of nitrate at two southwest Pacific marine sites. EOS 67: 885

    Google Scholar 

  • Savoie DL, Prospero JM & Nees RT (1987) Nitrate, non-sea-salt sulfate, and mineral aerosol over the northwestern Indian Ocean. J. Geophys. Res. 92: 933–942

    Google Scholar 

  • Savoie DL, Prospero JM & Saltzman ES (1989) Non-sea-salt sulfate and nitrate in trade wind aerosols at Barbados: Evidence for long-term transport. J. Geophys. Res. 94: 5069–5080

    Google Scholar 

  • Semb A, Brekkan R & Joranger E (1984) Major ions in Spitsbergen snow samples. Geophys. Res. Lett. 11: 445–448

    Google Scholar 

  • Spencer MJ, Mayewski PA, Lyons WB & Hendy MR (1985) A preliminary assessment of the potential application of glaciochemical investigations on Heard Island, South Indian Ocean. J. Glaciol. 31: 233–236

    Google Scholar 

  • Talbot RW, Harriss RC, Browell EV, Gregory GL, Sebacher DI & Beck SM (1986) Distribution and geochemistry of aerosols in tropical North Atlantic troposphere: Relationship to Saharan dust. J. Geophys. Res. 91: 5173–5182

    Google Scholar 

  • Twickler MS, Spencer MJ, Lyons WB & Mayewski PA (1986) Measurement of organic carbon in polar snow samples. Nature 320: 156–158

    Google Scholar 

  • Wake C (1987) Snow accumulation studies in the Central Karakoram, Pakistan. Proc. Eastern Snow Conf. 44th Meeting (pp 19–23)

    Google Scholar 

  • Wagenbach D, Gorlach U, Haffa K, Junghans HG & Munnich KO (1988) A long term aerosol deposition record in a high altitude alpine glacier. WMO Special Environ. Rpt. Series

  • Wolff GT (1984) On the nature of nitrate in coarse continental aerosols. Atmos. Environ. 18: 977–981

    Google Scholar 

Download references

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Berry Lyons, W.L., Mayewski, P.A., Spencer, M.J. et al. Nitrate concentrations in snow from remote areas: implication for the global NO x flux. Biogeochemistry 9, 211–222 (1990). https://doi.org/10.1007/BF00000599

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