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Fe-induced magnetic transition in YBa2(Cu1−x 57Fe x )3O6 by NQR and Mössbauer spectroscopy

  • Superconductors
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Abstract

Nuclear quadrupole resonance spectroscopy (around 30 MHz) on the chain site Cu(1) nuclei in oxygen deficient YBa2(Cu1−x Fe x )3O6 doped with different amounts of57Fe (x≤0.01) reveal an onset of magnetic order at low temperatures represented by a symmetrical doublet contribution to the nuclear quadrupole resonance (NQR) spectrum. The onset temperatureT N2 depends on the concentration of Fe reaching 130 K forx=0.01. The splitting forx=0.01 at 100 K corresponds to a net internal field of 0.09 T with a distribution of ≈0.08 T representing about 70 percent of the Cu(1) nuclei.57Fe and57Co Mössbauer spectroscopy at 4.2 K with and without an external magnetic field of 5 T revealed that belowx=0.00015 Fe spins are decoupled from the Cu(2) moments in the antiferromagnetic state. Results are interpreted in terms of the magnetic model structure suggested by Kadowaki et al. [1].

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Authors and Affiliations

  1. Central Research Institute for Physics, P. O. Box 49, H-1525, Budapest, Hungary

    L. Bottyán, A. Jánossy, A. Barcs, I. Fúró & D. L. Nagy

  2. Physikalisches Institut der Universität Erlangen-Nürnberg, Erwin-Rommel-Str. 1, D-8520, Erlangen, FRG

    J. Dengler

Authors
  1. L. Bottyán
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  2. A. Jánossy
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  3. A. Barcs
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  4. I. Fúró
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  5. J. Dengler
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  6. D. L. Nagy
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Bottyán, L., Jánossy, A., Barcs, A. et al. Fe-induced magnetic transition in YBa2(Cu1−x 57Fe x )3O6 by NQR and Mössbauer spectroscopy. Hyperfine Interact 55, 1219–1227 (1990). https://doi.org/10.1007/BF02397152

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  • DOI: https://doi.org/10.1007/BF02397152

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