ALBERT

Description: During a 4-week run in October–November 2006, a pilot experiment was performed at the CERN Proton Synchrotron in preparation for the CLOUD1 experiment, whose aim is to study the possible influence of cosmic rays on clouds. The purpose of the pilot experiment was firstly to carry out exploratory measurements of the effect of ionising particle radiation on aerosol formation from trace H2SO4 vapour and secondly to provide technical input for the CLOUD design. A total of 44 nucleation bursts were produced and recorded, with formation rates of particles above the 3 nm detection threshold of between 0.1 and 100 cm−3s−1, and growth rates between 2 and 37 nm h−1. The corresponding H2SO4 concentrations were typically around 106 cm−3 or less. The experimentally-measured formation rates and H2SO4 concentrations are comparable to those found in the atmosphere, supporting the idea that sulphuric acid is involved in the nucleation of atmospheric aerosols. However, sulphuric acid alone is not able to explain the observed rapid growth rates, which suggests the presence of additional trace vapours in the aerosol chamber, whose identity is unknown. By analysing the charged fraction, a few of the aerosol bursts appear to have a contribution from ion-induced nucleation and ion-ion recombination to form neutral clusters. Some indications were also found for the accelerator beam timing and intensity to influence the aerosol particle formation rate at the highest experimental SO2 concentrations of 6 ppb, although none was found at lower concentrations. Overall, the exploratory measurements provide suggestive evidence for ion-induced nucleation or ion-ion recombination as sources of aerosol particles. However in order to quantify the conditions under which ion processes become significant, improvements are needed in controlling the experimental variables and in the reproducibility of the experiments. Finally, concerning technical aspects, the most important lessons for the CLOUD design include the stringent requirement of internal cleanliness of the aerosol chamber, as well as maintenance of extremely stable temperatures (variations below 0.1°C). 1CLOUD is an acronym of Cosmics Leaving OUtdoor Droplets.

Description: Natural ecosystems respond to, and may affect climate change through uptake and storage of atmospheric CO2. Here we use the land-surface and carbon cycle model JULES to simulate the contemporary European carbon balance and its sensitivity to rising CO2 and changes in climate. We find that the impact of climate change is to decrease the ability of Europe to store carbon by 97 TgC yr−1. In contrast, the effect of rising atmospheric CO2 has been to stimulate increased uptake and storage. The CO2 effect is currently dominant leading to a net increase of 114 TgC yr−1. Our simulations do not at present include other important factors such as land use and management, the effects of forest age classes and nitrogen deposition. Understanding this balance and its implications for mitigation policies is becoming increasingly important.

Description: We present a new reconstruction of the interplanetary magnetic field (IMF, B) for 1846–2012 with a full analysis of errors, based on the homogeneously constructed IDV(1d) composite of geomagnetic activity presented in Part 1 (Lockwood et al., 2013a). Analysis of the dependence of the commonly used geomagnetic indices on solar wind parameters is presented which helps explain why annual means of interdiurnal range data, such as the new composite, depend only on the IMF with only a very weak influence of the solar wind flow speed. The best results are obtained using a polynomial (rather than a linear) fit of the form B = χ · (IDV(1d) − β)α with best-fit coefficients χ = 3.469, β = 1.393 nT, and α = 0.420. The results are contrasted with the reconstruction of the IMF since 1835 by Svalgaard and Cliver (2010).

Description: Svalgaard (2014) has recently pointed out that the calibration of the Helsinki magnetic observatory's H component variometer was probably in error in published data for the years 1866–1874.5 and that this makes the interdiurnal variation index based on daily means, IDV(1d), (Lockwood et al., 2013a), and the interplanetary magnetic field strength derived from it (Lockwood et al., 2013b), too low around the peak of solar cycle 11. We use data from the modern Nurmijarvi station, relatively close to the site of the original Helsinki Observatory, to confirm a 30% underestimation in this interval and hence our results are fully consistent with the correction derived by Svalgaard. We show that the best method for recalibration uses the Helsinki Ak (H) and aa indices and is accurate to ±10%. This makes it preferable to recalibration using either the sunspot number or the diurnal range of geomagnetic activity which we find to be accurate to ±20%. In the case of Helsinki data during cycle 11, the two recalibration methods produce very similar corrections which are here confirmed using newly digitised data from the nearby St Petersburg observatory and also using declination data from Helsinki. However, we show that the IDV index is, compared to later years, too similar to sunspot number before 1872, revealing independence of the two data series has been lost; either because the geomagnetic data used to compile IDV has been corrected using sunspot numbers, or vice versa, or both. We present corrected data sequences for both the IDV(1d) index and the reconstructed IMF (interplanetary magnetic field). We also analyse the relationship between the derived near-Earth IMF and the sunspot number and point out the relevance of the prior history of solar activity, in addition to the contemporaneous value, to estimating any "floor" value of the near-Earth interplanetary field.

Description: In the concluding paper of this tetralogy, we here use the different geomagnetic activity indices to reconstruct the near-Earth interplanetary magnetic field (IMF) and solar wind flow speed, as well as the open solar flux (OSF) from 1845 to the present day. The differences in how the various indices vary with near-Earth interplanetary parameters, which are here exploited to separate the effects of the IMF and solar wind speed, are shown to be statistically significant at the 93% level or above. Reconstructions are made using four combinations of different indices, compiled using different data and different algorithms, and the results are almost identical for all parameters. The correction to the aa index required is discussed by comparison with the Ap index from a more extensive network of mid-latitude stations. Data from the Helsinki magnetometer station is used to extend the aa index back to 1845 and the results confirmed by comparison with the nearby St Petersburg observatory. The optimum variations, using all available long-term geomagnetic indices, of the near-Earth IMF and solar wind speed, and of the open solar flux, are presented; all with ±2σ uncertainties computed using the Monte Carlo technique outlined in the earlier papers. The open solar flux variation derived is shown to be very similar indeed to that obtained using the method of Lockwood et al. (1999).

Description: Electricity in the atmosphere provides an ideal topic for educational outreach in environmental science. To support this objective, a simple instrument to measure real atmospheric electrical parameters has been developed and its performance evaluated. This project compliments educational activities undertaken by the Coupling of Atmospheric Layers (CAL) European research collaboration. The new instrument is inexpensive to construct and simple to operate, readily allowing it to be used in schools as well as at the undergraduate University level. It is suited to students at a variety of different educational levels, as the results can be analysed with different levels of sophistication. Students can make measurements of the fair weather electric field and current density, thereby gaining an understanding of the electrical nature of the atmosphere. This work was stimulated by the centenary of the 1906 paper in which C. T. R. Wilson described a new apparatus to measure the electric field and conduction current density. Measurements using instruments based on the same principles continued regularly in the UK until 1979. The instrument proposed is based on the same physical principles as C. T. R. Wilson's 1906 instrument.

Description: We present a new composite of geomagnetic activity which is designed to be as homogeneous in its construction as possible. This is done by only combining data that, by virtue of the locations of the source observatories used, have similar responses to solar wind and IMF (interplanetary magnetic field) variations. This will enable us (in Part 2, Lockwood et al., 2013a) to use the new index to reconstruct the interplanetary magnetic field, B, back to 1846 with a full analysis of errors. Allowance is made for the effects of secular change in the geomagnetic field. The composite uses interdiurnal variation data from Helsinki for 1845–1890 (inclusive) and 1893–1896 and from Eskdalemuir from 1911 to the present. The gaps are filled using data from the Potsdam (1891–1892 and 1897–1907) and the nearby Seddin observatories (1908–1910) and intercalibration achieved using the Potsdam–Seddin sequence. The new index is termed IDV(1d) because it employs many of the principles of the IDV index derived by Svalgaard and Cliver (2010), inspired by the u index of Bartels (1932); however, we revert to using one-day (1d) means, as employed by Bartels, because the use of near-midnight values in IDV introduces contamination by the substorm current wedge auroral electrojet, giving noise and a dependence on solar wind speed that varies with latitude. The composite is compared with independent, early data from European-sector stations, Greenwich, St Petersburg, Parc St Maur, and Ekaterinburg, as well as the composite u index, compiled from 2–6 stations by Bartels, and the IDV index of Svalgaard and Cliver. Agreement is found to be extremely good in all cases, except two. Firstly, the Greenwich data are shown to have gradually degraded in quality until new instrumentation was installed in 1915. Secondly, we infer that the Bartels u index is increasingly unreliable before about 1886 and overestimates the solar cycle amplitude between 1872 and 1883 and this is amplified in the proxy data used before 1872. This is therefore also true of the IDV index which makes direct use of the u index values.

Description: The vertical columnar current density in the global atmospheric electrical circuit depends on the local columnar resistance. A simple model for the columnar resistance is suggested, which separates the local boundary layer component from the upper troposphere cosmic ray component, and calculates the boundary layer component from a surface measurement of air conductivity. This theory is shown to provide reasonable agreement with observations. One application of the simple columnar model theory is to provide a basis for the synthesis of surface atmospheric electrical measurements made simultaneously at several European sites. Assuming the ionospheric potential to be common above all the sites, the theoretical air-earth current density present in the absence of a boundary layer columnar resistance can be found by extrapolation. This is denoted the free troposphere limit air-earth current density, J0. Using early surface data from 1909 when no ionospheric potential data are available for corroboration, J0 is found to be ~6 pA m−2, although this is subject to uncertainties in the data and limitations in the theory. Later (1966–1971) European balloon and surface data give J0=2.4 pA m−2.

Description: The Nagycenk Geophysical Observatory in Hungary (47° 38 ' N, 16° 43 ' E) has made continuous measurements of the vertical atmospheric electric Potential Gradient (PG) since 1962. Global signals have previously been identified in the Nagycenk PG data. A long-term (1920–1981) decrease has been discovered in the PG measured at the Eskdalemuir Observatory, Scotland (55° 19 ' N, 3° 12 ' W), suggesting that this represents a global change in the atmospheric electricity related to a decline in cosmic rays. A 40% decline in PG is shown here to have occurred at Nagycenk between 1962 and 2001, also consistent with changes in the air-Earth current measured at Kew (51° 28 ' N, 0° 19 ' W), London, 1966–1978. Comparison of the long-term PG measurements at both Eskdalemuir and Nagycenk gives further evidence to support the hypothesis of a global atmospheric electrical decline from the early twentieth century to the present time, as it is shown that local effects at Nagycenk are unlikely to have dominated the changes there.Key words. Meteorology and atmospheric dynamics (atmospheric electricity)

Description: Long-term decreases found recently in both the atmospheric electrical potential gradient (PG) and the air-Earth current density (Jz), using observation series from the UK and Hungary, have motivated studies of other European data. Two surface data series somewhat longer than a decade were available: PG data obtained at Serra do Pilar (Portugal), and PG, Jz and positive air conductivity measurements at Athens (Greece). Selecting data to minimise local effects, the 1960–1971 Serra do Pilar PG values decrease at dawn and in the evening. Dawn data obtained at Athens (1967–1977) indicate a reduction in Jz, while the simultaneous PG values there increase (coincident air conductivity values decrease) for the periods investigated. The Athens PG increase is attributed to local aerosol influences, typical of urban environments. Despite the urban influence, the Athens Jz shows similarities with soundings of the ionospheric potential. The decline in Jz at Athens occurs simultaneously with a decrease reported previously in Jz at Kew (UK), indicating that, at least, a regional decrease in the global atmospheric electrical circuit occurred during part of the twentieth century. Similar surface changes occur in European atmospheric electrical parameters, with a decrease of about 0.5% to 0.7% per year between 1920 and 1970 (possibly extending back to 1898), an annual decrease of between 2.7 and 3.4%, between 1959 and 1971 and a continued decrease of about ~1% per year between 1967 and 1984, possibly still continuing. Keywords. Meteorology and atmospheric dynamics (Atmospheric electricity) – Geomagnetism and paleomagnetism (Time variations, secular and long term) – Atmospheric composition and structure (Aerosols and particles)