ALBERT

Description: An analysis of nadir reflectivity Fourier spatial power spectra and autocorrelation functions at solar wavelengths and for cloudy conditions has been carried out. The data come from Landsat Thematic Mapper (TM) observations, while Monte Carlo (MC) simulations are used to aid the interpretation of the Landsat results. We show that radiative processes produce consistent signatures on power spectra and autocorrelation functions. The former take a variety of forms not shown or explained in previous observational studies. We demonstrate that the TM spectra can potentially be affected by both radiative "roughening" at intermediate scales (approx. 1 -5 km), being more prevalent at large solar zenith angles, and the already documented radiative "smoothing" at small scales (less than 1 km). These processes are wavelength dependent, as shown by systematic differences between conservative (for cloud droplets) TM band 4 (approx. 0.8 microns) and absorbing band 7 (approx. 2.2 microns): band 7 exhibits more roughening and less smoothing. This is confirmed quantitatively by comparing least-squared fitted power spectral slopes for the two bands. It is also corroborated by a slower decrease with distance of autocorrelation function values for band 4 compared to band 7. The appearance of roughening at large solar zenith angles is a result of side illumination and shadowing and adds an additional complexity to the power spectra. MC spectra are useful in illustrating that scale invariant optical depth fields can produce complex power spectra that take a variety of shapes under different conditions. We show that radiative roughening increases with the decrease of single scattering albedo and with the increase of solar zenith angle (as in the observations). For high Sun there is also a clear shift of the radiative smoothing scale to smaller values as droplet absorption increases. The shape of the power spectrum is sensitive to the magnitude and type of cloud top height variability, with the spectral signatures of decorrelation between reflectance and optical depth at large scales becoming stronger as the magnitude of cloud top variations increase. Finally, the usefulness of power spectral analysis in evaluating the skill of novel optical depth retrieval techniques in removing 3D radiative effects is demonstrated. New techniques using inverse Non-local Independent Pixel Approximation (NIPA) and Normalized Difference of Nadir Reflectivity (NDNR) yield optical depth fields which better match the scale-by-scale variability of the true optical depth field.

Description: 3D aerosol-cloud interaction is examined by analyzing two images containing cumulus clouds in biomass burning regions in Brazil. The research consists of two parts. The first part focuses on identifying 3D clo ud impacts on the reflectance of pixel selected for the MODIS aerosol retrieval based purely on observations. The second part of the resea rch combines the observations with radiative transfer computations to identify key parameters in 3D aerosol-cloud interaction. We found that 3D cloud-induced enhancement depends on optical properties of nearb y clouds as well as wavelength. The enhancement is too large to be ig nored. Associated biased error in 1D aerosol optical thickness retrie val ranges from 50% to 140% depending on wavelength and optical prope rties of nearby clouds as well as aerosol optical thickness. We caution the community to be prudent when applying 1D approximations in comp uting solar radiation in dear regions adjacent to clouds or when usin g traditional retrieved aerosol optical thickness in aerosol indirect effect research.

Description: There are several dozen papers that study the effects of cloud horizontal inhomogeneity on the retrievals of cloud optical thickness, but only a few of them deal with cloud droplet sizes. This paper is one of the first comprehensive attempts to fill this gap: It takes a close theoretical look at the radiative effects of cloud 3-D structure in retrievals of droplet effective radii. Under some general assumptions, it was found that ignoring subpixel (unresolved) variability produces a negative bias in the retrieved effective radius, while ignoring cloud inhomogeneity at scales larger than a pixel scale (resolved variability), on the contrary, leads to overestimation of the domain average droplet size. The theoretical results are illustrated with examples from Large Eddy Simulations (LES) of cumulus (Cu) and stratocumulus (Sc) cloud fields. The analysis of cloud drop size distributions retrieved from both LES fields confirms that ignoring shadowing in 1-D retrievals results in substantial overestimation of effective radii which is more pronounced for broken Cu than for Sc clouds. Collocated measurements of broken Cu clouds by Moderate Resolution Imaging Spectrometer (MODIS) and Advanced Spaceborne Thermal Emission and Reflection Radiometer (ASTER) are used to check simulations and theory with observations. The analysis of ASTER and MODIS data and associated derived products recommends against blindly using retrieved effective radii for broken cloud fields, especially if one wants to relate aerosol amounts to cloud droplet sizes.

Description: The uncertainty in ground-based estimates of solar irradiance is quantitatively related to the temporal variability of the atmosphere's optical thickness. The upper and lower bounds of the accuracy of estimates using the Langley Plot technique are proportional to the standard deviation of aerosol optical thickness (approx. +/- 13 sigma(delta tau)). The estimates of spectral solar irradiance (SSI) in two Cimel sun photometer channels from the Mauna Loa site of AERONET are compared with satellite observations from SOLSTICE (Solar Stellar Irradiance Comparison Experiment) on UARS (Upper Atmospheric Research Satellite) for almost two years of data. The true solar variations related to the 27-day solar rotation cycle observed from SOLSTICE are about 0.15% at the two sun photometer channels. The variability in ground-based estimates is statistically one order of magnitude larger. Even though about 30% of these estimates from all Level 2.0 Cimel data fall within the 0.4 to approx. 0.5% variation level, ground-based estimates are not able to capture the 27-day solar variation observed from SOLSTICE.

Description: Two scenarios of spectral solar forcing, namely Spectral Irradiance Monitor (SIM)-based out-of-phase variations and conventional in-phase variations, are input to a time-dependent radiative-convective model (RCM), and to the GISS modelE. Both scenarios and models give maximum temperature responses in the upper stratosphere, decreasing to the surface. Upper stratospheric peak-to-peak responses to out-of-phase forcing are approx.0.6 K and approx.0.9 K in RCM and modelE, approx.5 times larger than responses to in-phase forcing. Stratospheric responses are in-phase with TSI and UV variations, and resemble HALOE observed 11-year temperature variations. For in-phase forcing, ocean mixed layer response lags surface air response by approx.2 years, and is approx.0.06 K compared to approx.0.14 K for atmosphere. For out-of-phase forcing, lags are similar, but surface responses are significantly smaller. For both scenarios, modelE surface responses are less than 0.1 K in the tropics, and display similar patterns over oceanic regions, but complex responses over land.

Description: Studies on aerosol direct and indirect effects require a precise separation of cloud-free and cloudy air. However, separation between cloud-free and cloudy areas from remotely-sensed measurements is ambiguous. The transition zone in the regions around clouds often stretches out tens of km, which are neither precisely clear nor precisely cloudy. We study the transition zone between cloud-free and cloudy air using MODerate-resolution Imaging Spectroradiometer (MODIS) and Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) measurements. Both instruments show enhanced clear-sky reflectance (MODIS) and clear-sky backscatterer (CALIPSO) near clouds, Analyzing a large dataset of MODIS observations we examine the effect of three-dimensional (3D) radiative interactions between clouds and cloud-free areas, also known as a cloud adjacency effect. Comparing with CALIPSO clear-sky backscatterer measurements, we show that the cloud adjacency effect may be responsible for a large portion of the enhanced clear sky reflectance observed by MODIS. While aerosol particles are responsible for a large part of the near-cloud enhancements in CALIPSO observations, misidentified or undetected cloud particles are also likely to contribute. As a result, both the nature of these particles (cloud vs. aerosol) and the processes creating them need to be clarified using a quantitative assessment of remote sensing limitations in particle detection and identification. The width and ubiquity of the transition zone near clouds imply that studies of aerosol-cloud interactions and aerosol direct radiative effects need to account for aerosol changes near clouds. Not accounted, these changes can cause systematic biases toward smaller aerosol radiative forcing. On the other hand, including aerosol products near clouds despite their uncertainties may overestimate aerosol radiative forcing. Therefore, there is an urgent need for developing methods that can assess and account for remote sensing challenges and thus allow for including the transition zone into the study. We describe a simple model that estimates the cloud-induced enhanced reflectances of cloud-free areas in the vicinity of clouds. The model assumes that the enhancement is due entirely to Rayleigh scattering and is therefore bigger at shorter wavelengths, thus creating a so-called apparent "bluing" of aerosols in remote sensing retrievals.

Description: To characterize aerosol-cloud interactions it is important to correctly retrieve aerosol optical depth in the vicinity of clouds. It is well reported in the literature that aerosol optical depth increases with cloud cover. Part of the increase comes from real physics as humidification; another part, however, comes from 3D cloud effects in the remote sensing retrievals. In many cases it is hard to say whether the retrieved increased values of aerosol optical depth are remote sensing artifacts or real. In the presentation, we will discuss how the 3D cloud affects can be mitigated. We will demonstrate a simple model that can assess the enhanced illumination of cloud-free columns in the vicinity of clouds. This model is based on the assumption that the enhancement in the cloud-free column radiance comes from the enhanced Rayleigh scattering due to presence of surrounding clouds. A stochastic cloud model of broken cloudiness is used to simulate the upward flux.

Description: Large amounts of SO2 injected into the stratosphere by the El Chichon volcanic eruption greatly enhanced the sulfuric acid aerosol loading. According to laboratory studies, the increase in aerosol surface area would lead to a loss of ozone. Radiation measurements from the solar backscatter ultraviolet spectroradiometer are used to probe the absorbing and scattering properties of the stratosphere after the eruption. The backscattered radiation is enhanced for wavelengths greater than 290 nm, with a peak at about 302 nm. The enhancements associated with aerosol backscattering and ozone change can be separated. A decrease in column ozone of 8 to 30 Dobson units was deduced within the aerosol layer at an altitude between 20 and 30 km following the month of the eruption.

Description: No abstract available

Description: Studies on aerosol direct and indirect effects require a precise separation of cloud-free and cloudy air. However, separation between cloud-free and cloudy areas from remotely-sensed measurements is ambiguous. The transition zone in the regions around clouds often stretches out tens of km, which are neither precisely clear nor precisely cloudy. We study the transition zone between cloud-free and cloudy air using MODerate-resolution Imaging Spectroradiometer (MODIS) and Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) measurements. Both instruments show enhanced clear-sky reflectance (MODIS) and clear-sky backscatterer (CALIPSO) near clouds. Analyzing a large dataset of MODIS observations we examine the effect of three-dimensional (3D) radiative interactions between clouds and cloud-free areas, also known as a cloud adjacency effect. Comparing with CALIPSO clear-sky backscatterer measurements, we show that the cloud adjacency effect may be responsible for a large portion of the enhanced clear sky reflectance observed by MODIS. While aerosol particles are responsible for a large part of the near-cloud enhancements in CALIPSO observations, misidentified or undetected cloud particles are also likely to contribute. As a result, both the nature of these particles (cloud vs. aerosol) and the processes creating them need to be clarified using a quantitative assessment of remote sensing limitations in particle detection and identification. "The width and ubiquity of the transition zone near clouds imply that studies of-aerosol-cloud -interactions and aerosol direct radiative effects need to account for aerosol changes near clouds. Not accounted, these changes can cause systematic biases toward smaller aerosol radiative forcing. On the other hand, including aerosol products near clouds despite their uncertainties may overestimate aerosol radiative forcing. Therefore, there is an urgent need for developing methods that can assess and account for remote sensing challenges and thus allow for including the transition zone into the study. We describe a simple model that estimates the cloud-induced enhanced reflectances of cloud-free areas in the vicinity of clouds. The model assumes that the enhancement is due entirely to Rayleigh scattering and is therefore bigger at shorter wavelengths, thus creating a so-called apparent "bluing" of aerosols in remote sensing retrievals.