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  • 1
    Publication Date: 2011-08-24
    Description: Stratospheric concentrations of HO2, H2O2, and OH have been retrieved simultaneously from the far-infrared emission spectra obtained with a balloon-borne Fourier transform spectrometer in June 1983 at 32 deg N latitude. Retrieved concentrations of HO2 and H2O2 are reported, along with vertical distributions of OH which were reported in an earlier paper for the afternoon, sunset, and nighttime periods for altitudes from 26 to 38 km. HO2 distributions are obtained with uncertainties that are about the same as OH for the same vertical range and for the afternoon and sunset periods. H2O2 concentration is obtained at an altitude of 30 km for the period that covers afternoon and sunset hours. The retrieved concentrations of these HO(x) species agree well with other individually measured results and the steady state photochemical predictions. The ratio HO2/OH at around 32 km seems to increase from the afternoon period to the sunset period.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 96; 22
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  • 2
    Publication Date: 2011-08-19
    Description: The Atmospheric Trace Molecule Spectroscopy (ATMOS) instrument recorded 19 sets of interferograms during solar occultations in both the Northern and Southern Hemispheres over the course of the Spacelab 3 mission. The resulting IR spectra furnish concentration profiles for over 25 atmospheric species. Attention is presently given to the volume mixing ratio profiles for HCl and HF in the 15-60-km altitude region, retrieved from northern sunsets and southern sunrises. The HF/HCl ratios deduced are in good agreement with model predictions. The total atmospheric chlorine at 50 km is nearly all in the form of HCl.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 92; 9851-985
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  • 3
    Publication Date: 2011-08-19
    Description: An analysis method that uses the nonlinear least-squares fit technique has been developed for emission spectra obtained with a Fourier transform spectrometer. This method is used for the analysis of submillimeter-region atmospheric emission spectra obtained with a balloon-borne FT spectrometer that was carried out as a correlative measurement for the Limb IR Monitor of the Stratosphere (LIMS) satellite experiment. The retrieved mixing ratios of H2O and O3 in the stratosphere from four spectral intervals have standard deviations of about 10 percent, and the average values agree to within 10 percent of corresponding results from the LIMS satellite experiment which used a broadband emission radiometer in the IR region.
    Keywords: INSTRUMENTATION AND PHOTOGRAPHY
    Type: Applied Optics (ISSN 0003-6935); 25; 3490-350
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  • 4
    Publication Date: 2011-08-19
    Description: Infrared solar absorption spectra of the stratosphere recorded at a resolution of 0.01/cm by the ATMOS (Atmospheric Trace Molecule Spectroscopy) instrument from onboard Spacelab 3 (04/30 to 05/6/85) have revealed the existence of many previously unobserved absorption features in the 1925 to 1960/cm and 1249 to 1255/cm regions and one at 774/cm. On the basis of comparisons with laboratory spectra, these features have been identified as belonging to the nu1, nu4, and nu6 bands of carbonyl fluoride, respectively. Volume mixing ratios of COF2 between 17 and 40 km have been deduced from analysis of the nu1 and nu6 bands.
    Keywords: GEOPHYSICS
    Type: Geophysical Research Letters (ISSN 0094-8276); 13; 769-772
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  • 5
    Publication Date: 2011-08-19
    Description: Absorptions due to the nu1 band of CH3Cl have been identified for the first time in infrared solar absorption spectra of the upper troposphere and lower stratosphere. The spectral data were obtained with the ATMOS Fourier transform spectrometer on board Spacelab 3 in May 1985 during four solar occultation events near latitudes of 30 deg N, 26 deg N, 25 deg N, and 49 deg S. Volume mixing ratio profiles of CH3Cl retrieved for the altitude range 12 to 23 km at these four latitudes do not show appreciable differences. Vertical mixing ratio distributions vary from 6 x 10 to the -10th at 12 km to 3 x 10 to the -10th at 23 km with an average uncertainty of about 25 percent. The retrieved mixing ratio does not decrease with altitude as rapidly as the data obtained by in situ techniques.
    Keywords: GEOPHYSICS
    Type: Geophysical Research Letters (ISSN 0094-8276); 13; 765-768
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  • 6
    Publication Date: 2011-08-19
    Description: Stratospheric solar absorption spectra recorded at about 0.01/cm resolution by the ATMOS (Atmospheric Trace Molecule Spectroscopy) Fourier transform spectrometer during the Spacelab 3 Shuttle mission (4/30-5/6/85) show a weak absorption feature covering about 802.5-803.3/cm. This feature is identified as the unresolved Q branch of the 802.7/cm band of HO2NO2 and profiles for 31 deg N and 47 deg S are reported.
    Keywords: GEOPHYSICS
    Type: Geophysical Research Letters (ISSN 0094-8276); 13; 761-764
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  • 7
    Publication Date: 2011-08-19
    Keywords: INSTRUMENTATION AND PHOTOGRAPHY
    Type: NASA, Washington Upper Atmosphere Res. Program; p 236-237
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  • 8
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    Publication Date: 2011-08-19
    Keywords: GEOPHYSICS
    Type: NASA, Washington Upper Atmopshere Res. Program; p 201-202
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  • 9
    Publication Date: 2011-08-19
    Keywords: INORGANIC AND PHYSICAL CHEMISTRY
    Type: NASA, Washington Upper Atmosphere Res. Program; p 49-50
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  • 10
    Publication Date: 2011-08-18
    Description: An analytical method for the analysis of absorption spectra obtained from the interferograms of an interferometer operated in the solar occultation mode, in which an interferogram is smeared with individual interferogram components generated by the passage of rays at different tangent altitudes, is described. The creation of strong sidelobes on absorption lines by the interferogram smearing leads to the recommendation of a strong apodization on the interferogram for the solar occultation experiment. The application of these concepts to the simultaneous retrieval of temperature and pressure from CO2 4.3-micron band stratospheric absorption spectra includes the analysis of the continuum absorptions by the pressure-induced N2 fundamental bands and by far wings of the CO2 v3 band. Agreement is reported between observed and simulated spectra.
    Keywords: GEOPHYSICS
    Type: Applied Optics; 21; Apr. 15
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