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  • 1
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    Noble gas constraints on air-sea gas exchange and bubble fluxes (2010)
    American Geophysical Union
    Details
    Publication Date: 2022-05-25
    Description: Author Posting. © American Geophysical Union, 2009. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Journal of Geophysical Research 114 (2009): C11020, doi:10.1029/2009JC005396.
    Description: Air-sea gas exchange is an important part of the biogeochemical cycles of many climatically and biologically relevant gases including CO2, O2, dimethyl sulfide and CH4. Here we use a three year observational time series of five noble gases (He, Ne, Ar, Kr, and Xe) at the Bermuda Atlantic Time series Study (BATS) site in tandem with a one-dimensional upper ocean model to develop an improved parameterization for air-sea gas exchange that explicitly includes separate components for diffusive gas exchange and bubble processes. Based on seasonal timescale noble gas data, this parameterization, which has a 1σ uncertainty of ±14% for diffusive gas exchange and ±29% for bubble fluxes, is more tightly constrained than previous parameterizations. Although the magnitude of diffusive gas exchange is within errors of that of Wanninkhof (1992), a commonly used parameterization, we find that bubble-mediated exchange, which is not explicitly included by Wanninkhof (1992) or many other formulations, is significant even for soluble gases. If one uses observed saturation anomalies of Ar (a gas with similar characteristics to O2) and a parameterization of gas exchange to calculate gas exchange fluxes, then the calculated fluxes differ by ∼240% if the parameterization presented here is used compared to using the Wanninkhof (1992) parameterization. If instead one includes the gas exchange parameterization in a model, then the calculated fluxes differ by ∼35% between using this parameterization and that of Wanninkhof (1992). These differences suggest that the bubble component should be explicitly included in a range of marine biogeochemical calculations that incorporate air-sea gas fluxes.
    Description: Funding from the National Science Foundation Chemical Oceanography program (OCE-0221247 and OCE-0623034).
    Keywords: Air-sea gas exchange ; Noble gas ; Bubbles
    Repository Name: Woods Hole Open Access Server
    Type: Article
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  • 2
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    Spreading of Greenland meltwaters in the ocean revealed by noble gases (2015)
    John Wiley & Sons
    Details
    Publication Date: 2022-05-25
    Description: Author Posting. © American Geophysical Union, 2015. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Geophysical Research Letters 42 (2015): 7705–7713, doi:10.1002/2015GL065003.
    Description: We present the first noble gas observations in a proglacial fjord in Greenland, providing an unprecedented view of surface and submarine melt pathways into the ocean. Using Optimum Multiparameter Analysis, noble gas concentrations remove large uncertainties inherent in previous studies of meltwater in Greenland fjords. We find glacially modified waters with submarine melt concentrations up to 0.66 ± 0.09% and runoff 3.9 ± 0.29%. Radiogenic enrichment of Helium enables identification of ice sheet near-bed melt (0.48 ± 0.08%). We identify distinct regions of meltwater export reflecting heterogeneous melt processes: a surface layer of both runoff and submarine melt and an intermediate layer composed primarily of submarine melt. Intermediate ocean waters carry the majority of heat to the fjords' glaciers, and warmer deep waters are isolated from the ice edge. The average entrainment ratio implies that ocean water masses are upwelled at a rate 30 times the combined glacial meltwater volume flux.
    Description: We gratefully acknowledge funding from WHOI's Ocean and Climate Change Institute, the Doherty Postdoctoral Scholarship, and ship time from the Advanced Climate Dynamics Summer School (SiU grant NNA-2012/10151).
    Description: 2016-03-30
    Keywords: Glacial melt ; Noble gases ; Tracers ; Meltwater ; Greenland ; Fjord
    Repository Name: Woods Hole Open Access Server
    Type: Article
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  • 3
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    A compilation of dissolved noble gas and N2/Ar ratio measurements collected from 1999-2016 in locations spanning the globe (2022)
    Biological and Chemical Oceanography Data Management Office (BCO-DMO). Contact: bco-dmo-data@whoi.edu
    Details
    Publication Date: 2022-10-31
    Description: Dataset: Global Noble Gases
    Description: Inert gases dissolved in the ocean are powerful tracers of the impact of physical processes on gases, particularly air-sea gas exchange (by both diffusive and bubble-meditated processes), temperature change, atmospheric pressure variation, mixing between different water masses, and ice processes. We have compiled a global ocean database of dissolved neon, argon, and krypton measurements, supplemented by helium, xenon, and nitrogen/argon (N2/Ar) ratios in some locations. Samples were collected on board multiple research cruises spanning the period 1999 through 2016 and analyzed by mass spectrometry at four different shore-based laboratories (University of Victoria, Woods Hole Oceanographic Institution, University of Washington, and Scripps Institution of Oceanography). Version 2.0 corrects an incorrect sign in the longitude for cruise 33KI20040814:HOT162 in version 1.0. The error in the database does not affect any figures in the publication (doi: 10.1146/annurev-marine-121916-063604). For a complete list of measurements, refer to the full dataset description in the supplemental file 'Dataset_description.pdf'. The most current version of this dataset is available at: https://www.bco-dmo.org/dataset/743867
    Description: NSF Division of Ocean Sciences (NSF OCE) OCE-0623034, NSF Division of Ocean Sciences (NSF OCE) OCE-0926659, National Sciences and Engineering Research Council of Canada (NSERC) 328290-2006, NSF Division of Ocean Sciences (NSF OCE) OCE-1130870, NSF Division of Ocean Sciences (NSF OCE) OCE-1232991, NSF Division of Ocean Sciences (NSF OCE) OCE-1029299, National Sciences and Engineering Research Council of Canada (NSERC) 329290-2012, National Sciences and Engineering Research Council of Canada (NSERC) 433848-2012, National Sciences and Engineering Research Council of Canada (NSERC) 433898-2012, NSF Division of Ocean Sciences (NSF OCE) OCE-9617487, NSF Division of Ocean Sciences (NSF OCE) OCE-9819181, NSF Division of Ocean Sciences (NSF OCE) OCE-9906922, NSF Division of Ocean Sciences (NSF OCE) OCE-0221247, NSF Division of Ocean Sciences (NSF OCE) OCE-0242139, NSF Division of Ocean Sciences (NSF OCE) OCE-0647979, NSF Division of Ocean Sciences (NSF OCE) OCE-0825394
    Keywords: Noble gases ; Nitrogen ; Neon ; Argon ; Krypton ; Carbon pumps
    Repository Name: Woods Hole Open Access Server
    Type: Dataset
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  • 4
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    The five stable noble gases are sensitive unambiguous tracers of glacial meltwater (2014)
    John Wiley & Sons
    Details
    Publication Date: 2022-05-26
    Description: Author Posting. © American Geophysical Union, 2014. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Geophysical Research Letters 41 (2014): 2835–2841, doi:10.1002/2013GL058804.
    Description: The five inert noble gases—He, Ne, Ar, Kr, and Xe—exhibit a unique dissolved gas saturation pattern resulting from the formation and addition of glacial meltwater to seawater. He and Ne become oversaturated, and Ar, Kr, and Xe become undersaturated to varying percentages. For example, addition of 10‰ glacial meltwater to seawater results in a saturation anomaly of ΔHe = 12.8%, ΔNe = 8.9%, ΔAr = −0.5%, ΔKr = −2.2%, and ΔXe = −3.3%. This pattern in noble gas saturation reflects a unique meltwater signature that is distinct from the other major physical processes that modify the gas concentration and saturation, namely, seasonal changes in temperature at the ocean surface and bubble mediated gas exchange. We use Optimum Multiparameter analysis to illustrate how all five noble gases can help distinguish glacial meltwater from wind-driven bubble injection, making them a potentially valuable suite of tracers for glacial melt and its concentration in the deep waters of the world ocean.
    Description: We are grateful to the National Science Foundation (OCE825394 and OCE0752980) for support of this research.
    Description: 2014-10-16
    Keywords: Tracers ; Noble gases ; Meltwater ; Glacier ; Glacial ice ; Latent heat
    Repository Name: Woods Hole Open Access Server
    Type: Article
    Format: application/msword
    Format: application/postscript
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