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  • 1
    ISSN: 1573-0867
    Schlagwort(e): Africa ; biogenic emission ; dry season ; dynamic chamber ; forest ; grassland ; groundnut ; maize ; Miombo typesavanna ecosystem ; nitric oxide ; pulsing ; sorghum ; wet season ; Zimbabwe
    Quelle: Springer Online Journal Archives 1860-2000
    Thema: Land- und Forstwirtschaft, Gartenbau, Fischereiwirtschaft, Hauswirtschaft
    Notizen: Abstract During October to December 1994, we measured diel and seasonal variability in nitric oxide (NO) exchange by a southern African savanna ecosystem (Grasslands Research Station, Marondera, Zimbabwe). A set of automated dynamic chambers was installed in three sub-sites: Miombo forest, natural grassland, and cropped soils (maize, sorghum, groundnut). The latter received a single application of commercialy available in-organic or cowdung fertilizer. The dynamic chamber system is described in detail, including correction of the resulting data for wall losses and gas-phase reactions of the NO-NO2-O3 triad. During the dry season, net vertical NO fluxes were close to the detection limit (0.44 ngN m-2s-1) regardless of vegetation type. During the transition from dry to wet season strong "pulsing" effects of the NO flux were observed: NO emissions increased by a factor of up to 60 within hours. During the wet season, NO emissions varied between the different sub-sites of the ecosystem; corresponding means are in ranking order of fertilized agricultural plots (27.2 ngN m-2 s-1), unfertilized agricultural plots (8.5 ngN m-2 s-1 ), grassland (4.4 ngN m-2 s-1 ), and Miombo forest (1.5 ngN m-2 s-1). Soil moisture was found to be the dominant factor controlling the NO fluxes. Whenever it was not limiting, the diel behaviour of NO emission followed the daily variation of soil temperature measured 1 cm below the surface.
    Materialart: Digitale Medien
    Standort Signatur Erwartet Verfügbarkeit
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  • 2
    Publikationsdatum: 2011-08-19
    Beschreibung: The temporal variation in the concentration and chemistry of the atmospheric aerosol over central Amazonia, Brazil, during the 1987 wet season is discussed based on ground and aircraft collected data obtained during the NASA GTE ABLE 2B expedition conducted in April/May 1987. It is found that wet-season aerosol concentrations and composition are variable in contrast to the more uniform biogenic aerosol observed during the 1985 dry season; four distinct intervals of enhanced aerosol concentration coincided with short periods (3 to 5 d) of extensive rainfall. It is hypothesized that aerosol chemistry in Amazonia during the wet season is strongly influenced by long-range transport of soil dust, marine aerosol, and possibly biomass combustion products advected into the central Basin by large-scale tropospheric circulation, producing periodic pulses of material input to local boundary layer air. The resultant wet-season aerosol regime is dynamic, in contrast to the uniformity of natural biogenic aerosols during the dry season.
    Schlagwort(e): METEOROLOGY AND CLIMATOLOGY
    Materialart: Journal of Geophysical Research (ISSN 0148-0227); 95; 16955-16
    Format: text
    Standort Signatur Erwartet Verfügbarkeit
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  • 3
    Publikationsdatum: 2019-07-12
    Beschreibung: Rain samples from three sites in central Amazonia were collected over a period of 6 weeks during the 1987 wet season and analyzed for ionic species and dissolved organic carbon. A continuous record of precipitation chemistry and amount was obtained at two of these sites, which were free from local or regional pollution, for a time period of over 1 month. The volume-weighted mean concentrations of most species were found to be about a factor of 5 lower during the wet season compared with previous results from the dry season. Only sodium, potassium, and chloride showed similar concentrations in both seasons. When the seasonal difference in rainfall amount is taken into consideration, the deposition fluxes are only slightly lower for most species during the wet season than during the dry season, again with the exception of chloride, potassium, and sodium. Sodium and chloride are present in the same ratio as in sea salt; rapid advection of air masses of marine origin to the central Amazon Basin during the wet season may be responsible for the observed higher deposition flux of these species. Statistical analysis suggests that sulfate is, to a large extent, of marine (sea salt and biogenic) origin, but that long-range transport of combustion-derived aerosols also makes a significant contribution to sulfate and nitrate levels in Amazonian rain. Organic acid concentrations in rain were responsible for a large fraction of the observed precipitation acidity; their concentration was strongly influenced by gas/liquid interactions.
    Schlagwort(e): METEOROLOGY AND CLIMATOLOGY
    Materialart: Journal of Geophysical Research (ISSN 0148-0227); 95; 16987-16
    Format: text
    Standort Signatur Erwartet Verfügbarkeit
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