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Experimental studies of the vapor phase nucleation of refractory compounds. III - The condensation of silver (1986)

Lilleleht, L. U. ; Nuth, J. A. ; Donn, B. ; [et al.]

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Publication Date: 2011-08-19

Description: Measurements are reported of the critical supersaturation necessary to initiate the vapor phase nucleation of silver over the ambient temperature range 500-950 K at total pressures of 250 and 500 torr of hydrogen. The results are compared with the predictions of both classical nucleation theory and the theory of a physical spinodal developed by Rasmussen (1982), neither of which adequately describes the present observations. The nucleation of silver appears to be dependent on the total pressure of the system in a manner which suggests that three-body reactions are necessary in order to form the initial silver cluster (e.g., dimers) from the monoatomic vapor.

Keywords: INORGANIC AND PHYSICAL CHEMISTRY

Type: Journal of Chemical Physics (ISSN 0021-9606); 85; 1116-112

Format: text

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