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  • 1
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    Intercomparison of measurements of stratospheric hydrogen fluoride (1990)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Description: Observations of the vertical profile of hydrogen fluoride (HF) vapor in the stratosphere and of the vertical column amounts of HF above certain altitudes were made using a variety of spectroscopic instruments in the 1982 and 1983 Balloon Intercomparison Campaigns. Both emission instruments working in the far-infrared spectral region and absorption instruments using solar occultation in the 2.5-micron region were employed. No systematic differences were seen in results from the two spectral regions. A mean profile from 20 - 45 km is presented, with uncertainties ranging from 20 to 50 percent. Total columns measured from ground and from 12 km are consistent with the profile if the mixing ratio for HF is small in the troposphere and low stratosphere.
    Keywords: GEOPHYSICS
    Type: Journal of Atmospheric Chemistry (ISSN 0167-7764); 10; 219-236
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  • 2
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    Ozone intercomparisons from the Balloon Intercomparison Campaign (1985)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Description: Intercomparisons of remote and in-situ techniques used to measure stratospheric ozone are made using results obtained on the Balloon Intercomparison Campaign of 1982 and 1983. Two in-situ and four remote instruments participated. These included ECC ozonesondes, a UV absorption photometer, and microwave emission, IR emission, and absorption spectrometers. Differences are generally less than 15 percent, and are within the quoted error bars. Flights which involved different sets of instruments were made on four separate days, and results are intercompared in plots of ozone density versus altitude. A careful assessment of errors was made for each instrument, and a plot of absolute errors versus altitude is given.
    Keywords: GEOPHYSICS
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  • 3
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    Far-infrared spectroscopy of the earth's stratosphere (1985)
    In:  Other Sources
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    Publication Date: 2019-06-28
    Description: This paper discusses the spectrum of the earth's stratosphere in the far-infrared, from 5 to 250/cm. Many of the trace gases that are important in stratospheric photochemistry have been measured, or are potentially measurable in the far-infrared. The spectral features of these gases are discussed with application to spacecraft measurements. In particular, the suitability of the spectrum for measurements of the HO(x) and ClO(x) families and of O3 are compared for different classes of instruments: Fourier transform spectrometers, filter radiometers, and scanning high-resolution Fabry-Perot instruments. It is found that these types of instruments have complementary capabilities that would best be used in combination in a comprehensive multispecies measurement scheme.
    Keywords: GEOPHYSICS
    Type: AIAA PAPER 85-3006
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  • 4
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    Far-infrared radiometer to map OH in the middle atmosphere (1985)
    In:  Other Sources
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    Publication Date: 2019-06-28
    Description: A baseline design is evaluated for a far-infrared radiometer to map global concentration profiles of OH from a satellite platform. The instrument performance is modeled using the spectral database and radiative transfer models developed from recent balloon-based studies of the upper atmosphere. The results indicate that the OH concentration can be measured by limb sounding with 10-percent accuracy in the region of its peak concentration near 40 km, but with useful data for the altitude range between 25 and 120 km. The resolution is 3.5 km in the vertical and 500 km in the horizontal direction. The same technique in principle can be expanded in a multichannel mode to address other related species, e.g. H2O, O3, and HO2, which have accessible rotational emission features in the far-infrared spectral region.
    Keywords: GEOPHYSICS
    Type: AIAA PAPER 85-3007
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  • 5
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    Stratospheric HF and HCl observations /15 June 1981/ (1981)
    In:  Other Sources
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    Publication Date: 2019-06-28
    Description: Balloon measurements of the stratospheric HF/HCl ratio are reported. Seven far-infrared rotational lines of HF and HCl were observed at elevation angles of 25, 18 and 8 deg by a far-infrared Fourier-transform spectrometer on board a balloon platform at 28.5 km. Analysis of line intensities yields an average HF/HCl ratio of 0.18 + or - 0.02 at an effective altitude of 33 km, with a water vapor mixing ratio of about 4 ppmv. Results are noted to be in reasonable agreement with the calculated profile of Sze and Ko (1981) with 4.5 ppmv H2O.
    Keywords: GEOPHYSICS
    Type: Geophysical Research Letters; 8; Oct. 198
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  • 6
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    An upper limit for stratospheric hydrogen peroxide (1984)
    In:  Other Sources
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    Publication Date: 2019-06-28
    Description: It has been postulated that hydrogen peroxide is important in stratospheric chemistry as a reservoir and sink for odd hydrogen species, and for its ability to interconvert them. The present investigation is concerned with an altitude dependent upper limit curve for stratospheric hydrogen peroxide, taking into account an altitude range from 21.5 to 38.0 km for January 23, 1983. The data employed are from balloon flight No. 1316-P, launched from the National Scientific Balloon Facility (NSBF) in Palestine, Texas. The obtained upper limit curve lies substantially below the data reported by Waters et al. (1981), even though the results are from the same latitude and are both wintertime measurements.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 89; 11655-11
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  • 7
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    Far infrared measurement of stratospheric HCl (1980)
    In:  Other Sources
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    Publication Date: 2019-06-27
    Description: Thermal emission from three rotational lines of H(Cl-35) and H(Cl-37) was observed with a Fourier transform spectrometer from a balloon platform at 28.9 km. The measured HCl line-of-sight density at 1.9 deg elevation above 28.9 km is 4.7 + or - 1.3 x 10 to the 15th/sq cm, implying an average volume mixing ratio of 0.8 + or - 0.2 x 10 to the -9th at the mean sampling altitude of 32.5 km. For a uniform mixing ratio model, this corresponds to a vertical column density of 2.4 + or - 0.6 x 10 to the 14th/sq cm. This result is in reasonable agreement with near infrared spectroscopic determinations and an abundance from a chemical sampling technique of HCl at this altitude; a pressure modulator radiometer measurement yields a significantly higher amount of HCl.
    Keywords: GEOPHYSICS
    Type: Geophysical Research Letters; 7; Sept
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  • 8
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    Theoretical atmospheric transmission in the mid- and far-infrared at four altitudes (1976)
    In:  Other Sources
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    Publication Date: 2019-06-27
    Description: The IR transmission of the terrestrial atmosphere is calculated at four altitudes of interest: Mauna Kea at 4.2 km (2-1000 microns), aircraft at 14 km (5-1000 microns), and balloon at 28 km and 41 km (10-1000 microns). We show both high resolution spectra and broadband averages. The results are intended to serve both as a detailed guide to the interference that is expected from the atmosphere for astronomical spectroscopy and also as an indicator of the relative change in absorption and emission that can be expected at various observing altitudes. One salient result for the spectral region around 100 microns is that the absorption (and emissivity) of the atmosphere drops by a factor of 10 for each increase in altitude of 15 km throughout the aircraft and balloon range; thus balloon-borne astronomical photometry and spectroscopy should both enjoy a considerable advantage over aircraft observations in the 30-300-micron region.
    Keywords: GEOPHYSICS
    Type: Applied Optics; 15; Feb. 197
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  • 9
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    Upper limit for stratospheric HBr using far-infrared thermal emission spectroscopy (1992)
    In:  Other Sources
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    Publication Date: 2019-07-12
    Description: An upper limit is measured for stratospheric HBr from three balloon flights. The observations were made with the FIRS-2 far-infrared Fourier transform spectrometer. The 1sigma upper limits from the 1988, 1989, and 1990 balloon flights are 13 pptv at 35 km, 7 pptv at 32 km, and 3 pptv at 31 km, respectively. Combining all 3 flights, the weighted average 1sigma upper limit for HBr is 4 pptv at 32 km. This value is significantly smaller than the only other previously published spectroscopic value of 20 +/- 7 pptv (2sigma), but is consistent with a theoretical estimate which predicts roughly 0.4 pptv at this altitude.
    Keywords: GEOPHYSICS
    Type: Geophysical Research Letters (ISSN 0094-8276); 19; 16 A
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  • 10
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    Measurement of stratospheric HOCl - Concentration profiles, including diurnal variation (1989)
    In:  Other Sources
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    Publication Date: 2019-07-12
    Description: Determinations have been made of concentration profiles of HOCl in the earth's stratosphere, including the diurnal variation. Measurements of the rotational Q2 branch at 99.5/cm and of five RR(J3) transitions between 143 and 159/cm were made using far-infrared thermal emission spectroscopy. The spectra were obtained during a balloon flight of the FIRS 2 far-infrared Fourier-transform spectrometer and telescope from Palestine, Texas on May 12-13, 1988. From these measurements, altitude profiles of HOCl from 23 to 42 km are obtained. Daytime and nighttime average profiles of HOCl, as well as measurements on a 30-min time scale through the sunset transition at a single (35 km) altitude are presented. The measured profiles are lower than the current predictions from several modeling groups by a factor of approximately 0.6.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 94; 11059-11
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