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  • 1
    Publication Date: 2011-08-24
    Description: Enhanced concentrations of CH4 in the unpolluted atmospheric mixed layer over both Arctic and subarctic tundra landscapes are documented here using data from the NASA Arctic Boundary Layer Expedition (ABLE 3A). The CH4 concentration gradients were determined mainly by interactions of biogenic emission from wet tundra and turbulent mixing proceses. The gradient were most frequently associated with intrusion of upper tropospheric or stratospheric air into the midtroposphere, emissions from forest and tundra fires, and long-range transport of enhanced concentration of these gases from unidentified sources. Summertime haze layers exhibited midtropospheric enhancements of CH4 similar to those measured in winter Arctic events. The observations confirm the importance of Arctic and Subarctic wetland environments as a regional source of global atmospheric CH4.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 97; D15; p. 16,589-16,599.
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  • 2
    Publication Date: 2011-08-24
    Description: In situ airborne flux values for O3, CO, an CH4 over selected wetlands of Alaska are reported, and airborne CH4 flux measurements are presented for the first time. The source/sink distribution over the Yukon-Kuskokwim Delta (YKD) is qualitatively correlated with surface vegetation type. The CH4 source strength over the YKD ranged from 25 to 85 mg/sq m/d. A spatially averaged, seasonally adjusted source strength of 51 mg/sq m/d was established for the YKD. Indirect CH4 flux estimates obtained over the Alaskan North Slope indicate a much lower source strength. The global CH4 emission from tundra are estimated to be 44 Tg/a at an upper limit. Airborne CO flux measurements over the YKD indicate low negative flux values over the coastal areas, while some positive fluxes were observed in the inland sparsely forested regions. An inspection of the cospectrum of CO with vertical velocity for sample runs in coastal areas indicate the possibility of in situ photochemical destruction/production of CO.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 97; D15; p. 16,601-16,625.
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  • 3
    Publication Date: 2011-08-19
    Description: Measurements of NO, NO2, O3, and CO were obtained for tropopause fold events encountered during two flights of the NASA global tropospheric experiment aircraft in 1984. The results suggest that NO(x) may not always be a good tracer of air of recent stratospheric origin. It is suggested that the stratospheric source of NO(x) acts to introduce NO(x) over a short period and through a large vertical region of the troposphere.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 93; 15813-15
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  • 4
    Publication Date: 2011-08-19
    Description: The variations of ozone and carbon monoxide with respect to the atmospheric flow structure are investigated for two aircraft flights: one in the upper troposphere/lower stratosphere over the continental United States on April 20, 1984, and the other in the marine troposphere over the eastern Pacific on April 26, 1984. The high frequency (1 Hz) and precision of the measurements allow detailed analysis of the species distribution down to length scales of the order of 1 km. Correlations between the two species are made on large, medium, and small scales of motion, and the results are interpreted. In general, the correlations are negative with some regions of positive correlation. The interpretation of these results is discussed.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 92; 2121-213
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  • 5
    Publication Date: 2011-08-19
    Description: Results from an airborne intercomparison of techniques to measure tropospheric levels of carbon monoxide (CO) are discussed. The intercomparison was conducted as part of the National Aeronautics and Space Administration's Global Tropospheric Experiment and included a laser differential absorption method and two grab sample/gas chromatograph methods. Measurements were obtained during approximately 90 flight hours, during which the CO mixing ratios ranged from about 60 to 140 ppbv. The level of agreement observed for the ensemble of measurements was well within the overall accuracy stated for each instrument. The correlation observed between the measurements from the respective pairs of instruments ranged from 0.85 to 0.98, with no evidence for the presence of either a constant or proportional bias between any of the instruments.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 92; 2009-201
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  • 6
    Publication Date: 2011-08-19
    Description: A set of 14 pairs of vertical profiles of ozone and carbon monoxide, obtained with fast-response instrumentation, is presented. Most of these profiles, which were measured in the remote troposphere, also have supporting fast-response dew-point temperature profiles. The data suggest that the continental boundary layer is a source of tropospheric ozone, even in October and November, when photochemical activity should be rather small. In general, the small-scale vertical variability between CO and O3 is in phase. At low latitudes this relationship defines levels in the atmosphere where midlatitude air is being transported to lower latitudes, since lower dew-point temperatures accompany these higher CO and O3 concentrations. A set of profiles which is suggestive of interhemispheric transport is also presented. Independent meteorological analyses support these interpretations.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 92; 2083-209
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  • 7
    Publication Date: 2011-08-19
    Description: The usability and reliability of potential vorticity as a meteorological stratospheric tracer are evaluated. The concept of potential vorticity conservation during transport in which stratospheric and tropospheric air are mixing is tested. Aircraft data collected on April 20, 1984 in the western and southwestern U.S. are analyzed in order to derive potential vorticity data; vertical cross sections of constant-pressure data and temperature and wind speed gradients are examined. The tropopause fold observed during the April 20, 1984 aircraft flights is described. The potential vorticity, ozone mixing ratio, and carbon monoxide mixing ratio are compared; a positive correlation between potential vorticity and the ozone mixing ratio and a negative correlation between the potential vorticity and the carbon monoxide mixing ratio are detected. The data support the concepts of the conservation of potential vorticity, the entrainment and mixing of tropospheric air across the boundaries of the fold, and the applicability of potential vorticity as a stratospheric tracer.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 92; 2103-211
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  • 8
    Publication Date: 2011-08-19
    Description: An overview of the airborne intercomparisons of CO, NO, and OH instrumentation is presented in this first paper of the series on the NASA Global Tropospheric Experiment/Chemical Instrumentation Test and Evaluation (GTE/CITE 1). This paper provides the reader with background information about several important characteristics of the project. These include the overall objectives and approach, the measurements taken, the intercomparison protocol, aircraft platform, profiles of each aircraft flight, and the participants. A synopsis of the overall results of the CO, NO, and OH instrument intercomparisons is also included. Companion papers discuss the detailed results of the CO and NO intercomparison tests as well as pertinent scientific findings.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 92; 1977-198
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  • 9
    Publication Date: 2019-08-28
    Description: As part of the Global Tropospheric Experiment's Chemical Instrumentation Test and Evaluation (GTE/CITE 1) intercomparison, carbon monoxide (CO) measurements were made from the NASA CV-990 aircraft during the fall of 1983 and again in the spring of 1984. The experimental measurements for CO obtained during those flight series over the eastern and mid-Pacific are presented here. Data were acquired from 10 to 20 deg N latitude over the mid-Pacific and from 30 to 37 deg N latitude over the eastern Pacific off the coast of California. A seasonal variation of approximately 34 parts per billion by volume was measured over the altitudes and latitudes sampled, and a small latitudinal variation was also noted. The data are discussed in terms of the meteorological context in which they were collected.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 92; 2095-210
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