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  • 1
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    Tropical ozone loss following the eruption of Mt. Pinatubo (1993)
    In:  Other Sources
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    Publication Date: 2011-08-24
    Description: Total Ozone Mapping Spectrometer (TOMS) measurements of equatorial total ozone following the eruption of Mt. Pinatubo show a decrease of up to 6 percent over climatology. Ozone losses begin approximately a month following the eruption, consistent with the time required for the SO2 to convert to sulfuric acid aerosol. The thick aerosol layer interferes with the TOMS retrieval, but this interference is small and easily accounted for in the retrieval. Ozone values remain below climatology until December, 1991. Ozonesonde data from Natal, Brazil taken before and two months after the eruption support TOMS observations of ozone loss. These sondes show that the ozone loss region is confined to a 2-3 km thick layer between 24 and 28 km.
    Keywords: GEOPHYSICS
    Type: Geophysical Research Letters (ISSN 0094-8276); 20; 1; p. 29-32.
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  • 2
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    Optical effects of polar stratospheric clouds on the retrieval of TOMS total ozone (1992)
    In:  Other Sources
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    Publication Date: 2011-08-24
    Description: Small areas of sharply reduced ozone density appear frequently in the maps produced from polar region total ozone mapping spectrometer (TOMS) data. These mini-holes are of the order of 1000 km in extent with a lifetime of a few days. On the basis of measurements from ground-based instruments, balloon-borne ozonesondes, and simultaneous measurements of aerosol and ozone concentrations during aircraft flights in the Arctic and Antarctic regions, the appearance of polar stratospheric clouds (PSCs) are frequently associated with false reductions in ozone derived from the TOMS albedo data. By combining radiative transfer calculations with the observed PSC and ozone data, it is shown that PSCs located near or above the ozone density maximum (with optical thickness greater than 0.1) can explain most of the differences between TOMS ozone data and ground or in situ ozone measurements. Several examples of real and false TOMS mini-hole phenomenon are investigated using data from the 1989 Airborne Arctic Stratospheric Expedition (AASE) and from balloon flights over Norway and Sweden.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 97; D12,; 13
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  • 3
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    Aircraft measurements of NO(x) over the eastern Pacific and continental United States and implications for ozone production (1990)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Description: Results are reported from airborne measurements of NO, NO2, O3, and CO obtained in the free troposphere (FT) and boundary layer (BL) over the western U.S. and eastern Pacific during the NASA Global Tropospheric Experiment Chemical Instrumentation Test and Evaluation 2 (CITE 2) in summer 1986. The aircraft instrumentation and the CITE 2 flight protocols are described, and the results are presented in extensive tables and graphs. Over the ocean the median mixing ratios for NO and NO2 were found to be 4.0 and 10.4 parts per trillion by volume (pptv), respectively, in the BL and 12.4 and 18.0 pptv in the FT; the corresponding values over land were 34.5 and 75.0 pptv in the BL and 13.0 and 36.0 pptv in the FT. in continental air masses. NO(x) is shown to be positively correlated with O3 and CO and negatively correlated with dewpoint over the ocean, whereas over land NO(x) was positively correlated with O3, CO, and dewpoint.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 95; 10205-10
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  • 4
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    Ozone climatology at Natal, Brazil, from in situ ozonesonde data (1991)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Description: A large ozone-profile data set has been obtained through balloon ozonesonde soundings at Natal, Brazil, during 1978-1988. Maximum ozone concentrations occur during local spring (September-October), and minimum concentrations during late autumn (April-May); the seasonal variation is much larger in the troposphere than in the stratosphere. If there were no seasonal variation in the stratosphere, the seasonal variation observed in the troposphere alone would be sufficient to drive a total ozone column variation of about 5 percent. This is about half the size of the variation observed in the Natal Dobson spectrophotometer data.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 96; 10
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  • 5
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    Atmospheric peroxyacetyl nitrate measurements over the Brazilian Amazon Basin during the wet season - Relationships with nitrogen oxides and ozone (1990)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Description: An analysis is presented on the distribution and variability of PAN as well as its relationship with measured chemical and meteorological parameters. The chemicals of most interest for which measurements were available are PAN, NO(x), O3, CO, and C2Cl4. PAN was measured by the electron capture gas chromatographic technique, and the technique for calibrations and measurements are detailed. Data show that significant concentrations of PAN (5-125 ppt) are present during the wet season and this PAN is 1-5 times more abundant than NO(x). PAN levels at different atmospheric locations are discussed, and it is noted that PAN shows evidence of a possible latitudinal gradient in the free troposphere, with values falling rapidly from the northern midlatitudes toward the equator. High correlations between O3 and PAN levels suggest that nonmethane hydrocarbons may contribute significantly to high O3 in the free troposphere. Evidence indicates that virtually all of the NO(x) above 4 km could result from PAN decomposition.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 95; 16945-16
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  • 6
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    Ratios of peroxyacetyl nitrate to active nitrogen observed during aircraft flights over the eastern Pacific Ocean and continental United States (1990)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 95; 10179-10
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  • 7
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    Results from the Balloon Ozone Intercomparison Campaign (BOIC) (1986)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Description: Data from the BOIC which consisted of three balloon missions conducted in Palestine, Texas from June 1983 to March 1984 are presented. The BOIC was to assess the ability to perform ozone measurements from balloon platforms. The accuracy and precision of the various ozone measurement systems, which were composed of a photometer, a mass spectrometer, and solar UV absorption sensors, are evaluated. The ozone observations obtained with the instruments on the three flight missions are analyzed and intercompared. The flight in situ data are also compared to the National Bureau of Standards reference photometer, satellite measurements, and under simulated stratospheric pressure and ozone concentrations.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 91; 13137-13
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  • 8
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    Results from the Balloon Ozone Intercomparison Campaign (BOIC) (1985)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Description: In the Balloon Ozone Intercomparison Campaign (BOIC), several in situ UV absorption photometers, two solar UV absorption photometers, electrochemical sondes, and a mass spectrometer were intercompared in three flight missions. Concurrent data from Umkehr and satellite observations are also intercompared. The National Bureau of Standards provided a 'standard' ozone source for intercomparing the in situ instruments and ground pressure. Preliminary findings indicate that the standard deviation of the sensitivities among 17 instruments against the NBS reference was about 11 percent. These differences appear in flight at the lower levels and change at higher altitudes, indicating height-dependent errors. The difference among five in-situ UV photometers flown together ranged by plus or minus 8 percent during ascent to about 41 km. During float at 42 km, the difference nearly doubled. During descent, the difference decreased to about 4 percent, which is much closer to the expected accuracy of these instruments. Results from UV solar radiometers have been systematically higher than those from UV photometers by 15 to 20 percent - a very important disagreement that needs to be resolved.
    Keywords: GEOPHYSICS
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  • 9
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    Tropospheric nitric oxide measurements over the Amazon Basin (1988)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Description: Horizontal and vertical distributions of nitric oxide (NO) were measured over the Amazon Basin during NASA's Global Tropospheric Experiment (GTE) Amazon Boundary Layer Experiment mission in July-August 1985. During transit flights between the Virginia coast and Manaus, Brazil, NO mixing ratios were 12-15 pptv at 5 km altitude. Values up to 200 pptv were observed in electrically active clouds. During longitudinal surveys over the Amazon region, NO mixing ratios in the lower planetary boundary layer decreased from 25-60 pptv over the central basin to 10-12 pptv in coastal regions. In the convective cloud layer or free troposphere, NO mixing ratios averaged 13 pptv in regions not influenced by biomass burning. No longitudinal trend above the mixed layer could be detected. A steep negative gradient with increasing altitude was noted within the mixed layer before midday. Mixing ratios decreased from 60 pptv at 0.2 km to about 15 pptv at the top of the mixed layer (1 km). By midday, growth of the mixed layer height and enhanced mixing reduced the gradient, and evidence for mixing of NO into the convective cloud layer was noted.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 93; 1396-140
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  • 10
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    An intercomparison of results from ferrous sulphate and photolytic converter techniques for measurements of NO(x) made during the NASA GTE/CITE 1 aircraft program (1988)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Description: Two techniques designed for measurements of NO(x (NO + NO2) were intercompared during aircraft flights made in the spring of 1984 in the middle free troposphere over the eastern Pacific Ocean and southwestern U.S. One NO chemiluminescence instrument was equipped with a ferrous sulphate converter, another with a photolytic converter. The ferrous sulphate-equipped instrument was apparently much less specific for NO2. It registered levels about three times larger than the photolytic converter and gave NO2/NO ratios that were much larger than photochemical calculations would indicate as reasonable. Additionally, the results imply that active NO(x) was only 10-20 percent of the total odd nitrogen in the middle free troposphere.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 93; 15803-15
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