ALBERT

Description: Cloud droplet number concentration (Nd) is an important parameter of liquid clouds and is crucial to understanding aerosol-cloud interactions. It couples boundary layer aerosol composition, size and concentration with cloud reflectivity. It affects cloud evolution, precipitation, radiative forcing, global climate and, through observation, can be used to partially monitor the first indirect effect. With its unique combination of multi-wavelength, multi-angle, total and polarized reflectance measurements, the Research Scanning Polarimeter (RSP) retrieves Nd with relatively few assumptions. The approach involves measuring cloud optical thickness, mean droplet extinction cross-section and cloud physical thickness. Polarimetric observations are capable of measuring the effective variance, or width, of the droplet size distribution. Estimating cloud geometrical thickness is also an important component of the polarimetric Nd retrieval, which is accomplished using polarimetric measurements in a water vapor absorption band to retrieve the amount of in-cloud water vapor and relating this to physical thickness. We highlight the unique abilities and quantify uncertainties of the polarimetric approach. We validate the approach using observational data from the North Atlantic and Marine Ecosystems Study (NAAMES). NAAMES targets specific phases in the seasonal phytoplankton lifecycle and ocean-atmosphere linkages. This study provides an excellent opportunity for the RSP to evaluate its approach of sensing Nd over a range of concentrations and cloud types with in situ measurements from a Cloud Droplet Probe (CDP). The RSP and CDP, along with an array of other instruments, are flown on the NASA C-130 aircraft, which flies in situ and remote sensing legs in sequence. Cloud base heights retrieved by the RSP compare well with those derived in situ (R=0.83) and by a ceilometer aboard the R.V. Atlantis (R=0.79). Comparing geometric mean values from 12 science flights throughout the NAAMES-1 and NAAMES-2 campaigns, we find a strong correlation between Nd retrieved by the RSP and CDP (R=0.96). A linear least squares fit has a slope of 0.92 and an intercept of 0.3 cm3. Uncertainty in this comparison can be attributed to cloud 3D effects, nonlinear liquid water profiles, multilayered clouds, measurement uncertainty, variation in spatial and temporal sampling, and assumptions used within the method. Radiometric uncertainties of the RSP measurements lead to biases on derived optical thickness and cloud physical thickness, but these biases largely cancel out when deriving Nd for most conditions and geometries. We find that a polarimetric approach to sensing Nd is viable and the RSP is capable of accurately retrieving Nd for a variety of cloud types and meteorological conditions.

Description: The ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) campaign is taking place in the SouthEast Atlantic during the Austral Spring for three consecutive years from 20162018. The study area encompasses one of the Earths three semipermanent subtropical Stratocumulus (Sc) cloud decks,and experiences very large aerosol optical depths, mainly biomass burning, originating from Africa. Over time, cloud optical depth (COD), lifetime and cloud microphysics (number concentration, effective radii Reff and precipitation) are expected to be influenced by indirect aerosol effects. These changes play a key role in the energetic balance of the region, and are part of the core investigation objectives of the ORACLES campaign, which acquires measurements of clean and polluted scenes of above cloud aerosols (ACA). Simultaneous retrievals of aerosol and cloud optical properties are being developed (e.g. MODIS, OMI), butstill challenging, especially for passive, single viewing angle instruments. By comparison, multiangle polarimetric instruments like RSP (Research Scanning Polarimeter) show promise for detection and quantification of ACA, however, there are no operational retrieval algorithms available yet. Here we describe anew algorithm to retrieve cloud and aerosol optical properties from observations by RSP flown on the ER2and P3 during the 2016 ORACLES campaign. The algorithm is based on training a NN, and is intended to retrieve aerosol and cloud properties simultaneously. However, the first step was to establish the retrievalscheme for low level Sc cloud optical properties. The NN training was based on simulated RSP total and polarized radiances for a range of COD, Reff, and effective variances, spanning 7 wavelength bands and 152 viewing zenith angles. Random and correlated noise were added to the simulations to achieve a morerealistic representation of the signals. Before introducing the input variables to the network, the signals are projected on a principle component plane that retains the maximal signal information but minimizes the noise contribution. We will discuss parameter choices for the network and present preliminary results of cloudretrievals from ORACLES, compared with standard RSP low-levelcloud retrieval method that has been validated against in situ observations.

Description: This work develops a method to compare the radiometric calibration between a radiometer and imagers hosted on aircraft and satellites. The radiometer is the airborne Research Scanning Polarimeter (RSP), which takes multi-angle, photo-polarimetric measurements in several spectral channels. The RSP measurements used in this work were coincident with measurements made by the Airborne Visible/Infrared Imaging Spectrometer (AVIRIS), which was on the same aircraft. These airborne measurements were also coincident with an overpass of the Landsat 8 Operational Land Imager (OLI). First we compare the RSP and OLI radiance measurements to AVIRIS since the spectral response of the multispectral instruments can be used to synthesize a spectrally equivalent signal from the imaging spectrometer data. We then explore a method that uses AVIRIS as a transfer between RSP and OLI to show that radiometric traceability of a satellite-based imager can be used to calibrate a radiometer despite differences in spectral channel sensitivities. This calibration transfer shows agreement within the uncertainty of both the various instruments for most spectral channels.

Description: For remote sensing of aerosol over the ocean, there is a contribution from light scattered underwater. The brightness and spectrum of this light depends on the biomass content of the ocean, such that variations in the color of the ocean can be observed even from space. Rayleigh scattering by pure sea water, and Rayleigh-Gans type scattering by plankton, causes this light to be polarized with a distinctive angular distribution. To study the contribution of this underwater light polarization to multiangle, multispectral observations of polarized reflectance over ocean, we previously developed a hydrosol model for use in underwater light scattering computations that produces realistic variations of the ocean color and the underwater light polarization signature of pure sea water. In this work we review this hydrosol model, include a correction for the spectrum of the particulate scattering coefficient and backscattering efficiency, and discuss its sensitivity to variations in colored dissolved organic matter (CDOM) and in the scattering function of marine particulates. We then apply this model to measurements of total and polarized reflectance that were acquired over open ocean during the MILAGRO field campaign by the airborne Research Scanning Polarimeter (RSP). Analyses show that our hydrosol model faithfully reproduces the water-leaving contributions to RSP reflectance, and that the sensitivity of these contributions to Chlorophyll a concentration [Chl] in the ocean varies with the azimuth, height, and wavelength of observations. We also show that the impact of variations in CDOM on the polarized reflectance observed by the RSP at low altitude is comparable to or much less than the standard error of this reflectance whereas their effects in total reflectance may be substantial (i.e. up to 〉30%). Finally, we extend our study of polarized reflectance variations with [Chl] and CDOM to include results for simulated spaceborne observations.

Description: NASA Langley recently developed the world's first airborne multi-wavelength high spectral resolution lidar (HSRL). This lidar employs the HSRL technique at 355 and 532 nm to make independent, unambiguous retrievals of aerosol extinction and backscatter. It also employs the standard backscatter technique at 1064 nm and is polarization-sensitive at all three wavelengths. This instrument, dubbed HSRL-2 (the secondgeneration HSRL developed by NASA Langley), is a prototype for the lidar on NASA's planned Aerosols- Clouds-Ecosystems (ACE) mission. HSRL-2 completed its first science mission in July 2012, the Two-Column Aerosol Project (TCAP) conducted by the Department of Energy (DOE) in Hyannis, MA. TCAP presents an excellent opportunity to assess some of the remote sensing concepts planned for ACE: HSRL-2 was deployed on the Langley King Air aircraft with another ACE-relevant instrument, the NASA GISS Research Scanning Polarimeter (RSP), and flights were closely coordinated with the DOE's Gulfstream-1 aircraft, which deployed a variety of in situ aerosol and trace gas instruments and the new Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR). The DOE also deployed their Atmospheric Radiation Measurement Mobile Facility and their Mobile Aerosol Observing System at a ground site located on the northeastern coast of Cape Cod for this mission. In this presentation we focus on the capabilities, data products, and applications of the new HSRL-2 instrument. Data products include aerosol extinction, backscatter, depolarization, and optical depth; aerosol type identification; mixed layer depth; and rangeresolved aerosol microphysical parameters (e.g., effective radius, index of refraction, single scatter albedo, and concentration). Applications include radiative closure studies, studies of aerosol direct and indirect effects, investigations of aerosol-cloud interactions, assessment of chemical transport models, air quality studies, present (e.g., CALIPSO) and future (e.g., EarthCARE) satellite calibration/validation, and development/assessment of advanced retrieval techniques for future satellite applications (e.g., lidar+polarimeter retrievals of aerosol and cloud properties). We will also discuss the relevance of HSRL-2 measurement capabilities to the ACE remote sensing concept.

Description: The ObseRvations of Aerosols above Clouds and their interactions (ORACLES) project is making a series of field deployments to the southeastern Atlantic with NASA ER-2 and P3 aircraft to acquire both detailed remote sensing observations and in situ measurements of the aerosols and clouds in that region. This area is home to one of the largest low-level cloud decks on Earth that is seasonally affected by vast plumes of smoke from biomass burning, which in effect provides a natural experiment testing the radiative and microphysical interactions between the smoke and the clouds. The downward solar radiation at the surface, or cloud top, is always reduced by the presence of smoke. However, whether the amount of sunlight reflected back out to space is increased, or decreased by the presence of smoke is sensitively dependent on the brightness of the clouds and the fraction of light that the smoke absorbs each time light hits a smoke particle. In this study we use data from the Research Scanning Polarimeter, an along track scanning instrument, that provides measurements of the Stokes parameters I, Q and U at 410, 470, 555, 670, 865, 960, 1590, 1880 and 2260 nm at 150 viewing angles over a range of +/- 60 from nadir for each contiguous sub-aircraft pixel (~ 300 m in size). A retrieval algorithm is applied to the data acquired with a table look up technique, similar to that of the operational POLDER algorithm, to provide a first guess of the complex refractive index, optical depth and size distribution of the smoke particles together with cloud droplet size and optical depth. A subsequent iterative fitting procedure, where the fact that the doubling/adding method allows the construction of the Green's function for the radiative transfer equation, is used to obtain an efficient and statistically optimal estimate of the aerosol and cloud retrieval parameters. These retrieval parameters are evaluated against in situ observations, when available, and the optical depth and intensive lidar variables that are measured by the High Spectral Resolution Lidar 2. Finally, the aerosol and cloud retrievals are used to evaluate the variations in top of the atmosphere, surface/cloud top shortwave radiative forcing and atmospheric absorption that are caused by variations in the smoke and clouds.

Description: The Two-Column Aerosol Project (TCAP), conducted from June 2012 through June 2013, was a unique study designed to provide a comprehensive data set that can be used to investigate a number of important climate science questions, including those related to aerosol mixing state and aerosol radiative forcing. The study was designed to sample the atmosphere be tween and within two atmospheric columns; one fixed near the coast of North America (over Cape Cod, MA) and a second moveable column over the Atlantic Ocean several hundred kilometers from the coast. The U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Mobile Facility (AMF) was deployed at the base of the Cape Cod column, and the ARM Aerial Facility was utilized for the summer and winter intensive observation periods. One important finding from TCAP is that four of six nearly cloud-free flight days had aerosol layers aloft in both the Cape Cod and maritime columns that were detected using the nadir pointing second-generation NASA high-spectral resolution lidar (HSRL-2).These layer s contributed up to 60 of the total observed aerosol optical depth (AOD). Many of these layers were also intercepted by the aircraft configured for in situ sampling, and the aerosol in the layers was found to have increased amounts of biomass burning material and nitrate compared to aerosol found near the surface. In addition, while there was a great deal of spatial and day-to-day variability in the aerosol chemical composition and optical properties, no systematic differences between the two columns were observed.

Description: Accurate aerosol and cloud retrievals from space remain quite challenging and typically involve solving a severely ill-posed inverse scattering problem. In this Perspective, we formulate in general terms an aerosol and aerosol-cloud interaction space mission concept intended to provide detailed horizontal and vertical profiles of aerosol physical characteristics as well as identify mutually induced changes in the properties of aerosols and clouds. We argue that a natural and feasible way of addressing the ill-posedness of the inverse scattering problem while having an exquisite vertical-profiling capability is to fly a multistatic (including bistatic) lidar system. We analyze theoretically the capabilities of a formation-flying constellation of a primary satellite equipped with a conventional monostatic (backscattering) lidar and one or more additional platforms each hosting a receiver of the scattered laser light. If successfully implemented, this concept would combine the measurement capabilities of a passive multi-angle multi-spectral polarimeter with the vertical profiling capability of a lidar; address the ill-posedness of the inverse problem caused by the highly limited information content of monostatic lidar measurements; address the ill-posedness of the inverse problem caused by vertical integration and surface reflection in passive photopolarimetric measurements; relax polarization accuracy requirements; eliminate the need for exquisite radiative-transfer modeling of the atmosphere-surface system in data analyses; yield the day-and-night observation capability; provide direct characterization of ground-level aerosols as atmospheric pollutants; and yield direct measurements of polarized bidirectional surface reflectance. We demonstrate, in particular, that supplementing the conventional backscattering lidar with just one additional receiver flown in formation at a scattering angle close to 170deg can dramatically increase the information content of the measurements. Although the specific subject of this Perspective is the multistatic lidar concept, all our conclusions equally apply to a multistatic radar system intended to study from space the global distribution of cloud and precipitation characteristics.

Description: A dual-photoelastic-modulator- (PEM-) based spectropolarimetric camera concept is presented as an approach for global aerosol monitoring from space. The most challenging performance objective is to measure degree of linear polarization (DOLP) with an uncertainty of less than 0.5% in multiple spectral bands, at moderately high spatial resolution, over a wide field of view, and for the duration of a multiyear mission. To achieve this, the tandem PEMs are operated as an electro-optic circular retardance modulator within a high-performance reflective imaging system. Operating the PEMs at slightly different resonant frequencies generates a beat signal that modulates the polarized component of the incident light at a much lower heterodyne frequency. The Stokes parameter ratio q = Q/I is obtained from measurements acquired from each pixel during a single frame, providing insensitivity to pixel responsivity drift and minimizing polarization artifacts that conventionally arise when this quantity is derived from differences in the signals from separate detectors. Similarly, u = U/I is obtained from a different pixel; q and u are then combined to form the DOLP. A detailed accuracy and tolerance analysis for this polarimeter is presented.

Description: Key characteristics of the PACE observatory include: the Ocean Color Instrument (OCI), built at GSFC; the Hyper Angular Rainbow Polarimeter (HARP-2), contributed by the Earth and Space Institute at the University of Maryland Baltimore County; the Spectro-polarimeter for Planetary Exploration (SPEXone), contributed by a Netherlands-based consortium consisting of the Netherlands Institute for Space Research (SRON) and Airbus Defence and Space Netherlands; 676.5 km altitude and 13:00 local Equatorial crossing time; Sun synchronous, polar, ascending orbit with 98 inclination; and fall 2022 launch, three-year design life.