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  • 1
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    Airborne observations of the infrared emission bands (1989)
    In:  CASI
    Details
    Publication Date: 2013-08-31
    Description: Earlier airborne studies of the infrared bands between 5 and 8 microns have now been extended to a sample of southern sources selected from the IRAS Low Resolution Spectra (LRS) atlas. The correlation between the strongest bands at 6.2 and 7.7 microns is now based on a total sample of 40 sources and is very strong. A new emission band at 5.2 microns, previously predicted for polycyclic aromatic hydrocarbons (PAHs), is recognized in 27 sources; it too correlates with the dominant 7.7 micron band, showing that the 5.2 micron feature also belongs to the generic spectrum of PAH features at 3.3, 5.6, 6.2, 6.2, 7.7, 8.7, 11.3, and 12.7 microns. Sufficient sources are had now to define the relative strengths of most of these bands in three separate nebular environments: planetaries, H II regions, and reflection nebulae. Significant variations are detected in the generic spectra of PAHs in these different environments which are echoed by variations in the exact wavelength of the strong 7.7 micron peak. The earlier suggestion that, in planetaries, the fraction of total emission observed by IRAS that is carried by the PAH emissions is correlated with nebular gas-phase C/O ratio is supported by the addition of newly-observed southern planetaries, including the unusually carbon-rich (WC10) nebular nuclei. These (WC10) nuclei also exhibit a strong plateau of emission linking the 6.2 and 7.7 micron features.
    Keywords: ASTRONOMY
    Type: Interstellar Dust: Contributed Papers; p 93
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  • 2
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    Interstellar grain chemistry and the composition of comets (1988)
    In:  CASI
    Details
    Publication Date: 2013-08-31
    Description: During the past 15 years considerable progress in observational techniques has been achieved in the middle infrared, the spectral region most diagnostic of molecular vibrations. Spectra of many different astronomical infrared sources are now available. By comparing these astronomical spectra with the spectra of lab ices, one can determine the composition and abundance of the icy materials frozen on the cold dust grains present in the interior of molecular clouds. In the experiments described, the assumption is made that cometary ices are similar to interstellar ices. As an illustration of the processes which can take place as an ice is irradiated and subsequently warmed, the infrared spectra is presented of the mixture H2O:CH3OH:CO:NH3:C6H14 (100:50:10:10:10). Apart from the last species, the ratio of these compounds is representative of the simplest ices found in interstellar clouds.
    Keywords: ASTRONOMY
    Type: NASA, Washington, Infrared Observations of Comets Halley and Wilson and Properties of the Grains; p 127-128
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  • 3
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    Aromatic components in cometary materials (1988)
    In:  CASI
    Details
    Publication Date: 2013-08-31
    Description: The Raman spectra of interplanetary dust particles (IDPs) collected in the stratosphere show that two bands at about 1350 and 1600 delta/cm and a broader feature between 2200 and 3300 delta/cm that are characteristic of aromatic molecular units with ordered domains smaller than 25 A in diameter. This suggests that the carbonaceous material in IDPs may be similar to the polymeric component seen in meteorites, where this material is thought to consist of aromatic molecular units that are randomly interlinked by short aliphatic bridges. The features in the Raman spectra of IDPs are similar in position, and relative strength to interstellar infrared emission features that have been attributed to vibrational transitions in free molecular polycyclic aromatic hydrocarbons. Taken together, these observations suggest that some fraction of the carbonaceous materials in IDPs may have been produced in circumstellar dust shells and only slightly modified in interstellar space.
    Keywords: ASTRONOMY
    Type: NASA, Washington, Infrared Observations of Comets Halley and Wilson and Properties of the Grains; p 73-74
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  • 4
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    Spatial variations of the 3 micron emission features within nebulae (1989)
    In:  CASI
    Details
    Publication Date: 2013-08-31
    Description: The 3 micron spectra is presented for the Orion bar region and the Red Rectangle. In both objects spectra were obtained at more than one location, corresponding to different distances from the excitation source. The well known 3.3 and 3.4 micron emission bands are seen in both objects as well as the recently discovered features at 3.46, 3.51, and 3.57 microns in the Orion bar spectra. The spectra show that the relative strengths of the 3 micron emission features vary within the Orion bar. As distance from the exciting star increases, the 3.4 and 3.51 micron features increase, and the 3.46 micron feature decreases in strength, relative to the strong 3.3 micron feature. These are two possible interpretations which are postulated, each of which involves the breaking of bonds by UV radiation, which removes the modes responsible for the 3.4 micron emission near the star. The two possible bond ruptures are the CH bond in small polycyclic aromatic hydrocarbons (PAHs), or the bond to an aliphatic subgroup. It has to be pointed out that neither interpretation appears entirely satisfactory. The vibrational overtone interpretation cannot explain the presence or behavior of the 3.46 micron feature, whereas the laboratory spectra of aliphatic sidegroups contain many more features in the 3 micron region than are observed in the astronomical sources.
    Keywords: ASTRONOMY
    Type: Interstellar Dust: Contributed Papers; p 10
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  • 5
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    A multicomponent model of the infrared emission from Comet Halley (1988)
    In:  CASI
    Details
    Publication Date: 2013-08-31
    Description: A model based on a mixture of coated silicates and amorphous carbon grains produces a good spectral match to the available Halley data and is consistent with the compositional and morphological information derived from interplanetary dust particle studies and Halley flyby data. The dark appearance of comets may be due to carbonaceous coatings on the dominant (by mass) silicates. The lack of a 10 micrometer feature may be due to the presence of large silicate grains. The optical properties of pure materials apparently are not representative of cometary materials. The determination of the optical properties of additional silicates and carbonaceous materials would clearly be of use.
    Keywords: ASTRONOMY
    Type: NASA, Washington, Infrared Observations of Comets Halley and Wilson and Properties of the Grains; p 184-185
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  • 6
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    Airborne observations of the infrared emission bands (1989)
    In:  CASI
    Details
    Publication Date: 2013-08-29
    Description: The data concerning low resolution airborne spectra from 5 to 8 microns available for a sample of 40 sources selected from the Infrared Astronomy Satellite low resolution spectral Atlas with polycyclic aromatic hydrocarbon (PAH) emission features, are discussed. A new emission band at 5.2 microns, previously predicted for PAHs, was found in 33 sources; it also correlates with the 7.7 microns band. This extends the spectrum of narrow observed PAH features to 3.3, 5.2, 5.6, 6.2, 6.9, 7.7, 8.7, 11.3, and 12.7 microns. From the data the relative strengths of most of these bands are defined in three separate nebular environments: planetaries, H II regions, and reflection nebulae. The differences in the PAHs spectra in those environments are analyzed.
    Keywords: ASTRONOMY
    Type: ESA, Infrared Spectroscopy in Astronomy; p 149-154
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  • 7
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    The Unidentified Emission Features: a Study of the Orion Bar and Planetary Nebulae (1984)
    In:  CASI
    Details
    Publication Date: 2014-09-17
    Description: The unidentified emission features which are a group of broad emission bands found between 3.3 and 11.3 micro m in many objects which emit UV radiation and are associated with dust were studied. The features emit a substantial fraction of the energy in this wavelength range, and must therefore be an important constituent of the material around these objects. A two phase approach to the problem to better define the factors affecting the features was undertaken. The number of objects with good spectra between 3 and 13 micro m to look for correlations of the features with each other and with chemical and physical conditions were expanded and several positions in a single region, the Orion Bar, where the chemical composition was homogeneous, but the physical conditions varied are examined.
    Keywords: ASTRONOMY
    Type: Airborne Astron. Symp.; p 140-147
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