ALBERT

Description: We introduce the Clouds Above the United States and Errors at the Surface (CAUSES) project with its aim of better understanding the physical processes leading to warm screen-temperature biases over the American Midwest in many numerical models. In this first of four companion papers, 11 different models, from 9 institutes, perform a series of 5-day hindcasts, each initialised from reanalyses. After describing the common experimental protocol and detailing each model configuration, a gridded temperature data set is derived from observations and used to show that all the models have a warm bias over parts of the Midwest. Additionally, a strong diurnal cycle in the screen-temperature bias is found in most models. In some models the bias is largest around midday, while in others it is largest during the night. At the Department of Energy Atmospheric Radiation Measurement Southern Great Plains (SGP) site, the model biases are shown to extend several kilometers into the atmosphere. Finally, to provide context for the companion papers, in which observations from the SGP site are used to evaluate the different processes contributing to errors there, it is shown that there are numerous locations across the Midwest where the diurnal cycle of the error is highly correlated with the diurnal cycle of the error at SGP. This suggests that conclusions drawn from detailed evaluation of models using instruments located at SGP will be representative of errors that are prevalent over a larger spatial scale.

Description: Many numerical weather prediction and climate models exhibit too warm lower tropospheres near the mid-latitude continents. The warm bias has been shown to coincide with important surface radiation biases that likely play a critical role in the inception or the growth of the warm bias. This paper presents an attribution study on the net radiation biases in 9 model simulations, performed in the framework of the CAUSES project (Clouds Above the United States and Errors at the Surface). Contributions from deficiencies in the surface properties, clouds, water vapor and aerosols are quantified, using an array of radiation measurement stations near the ARM SGP site. Furthermore, an in-depth analysis is shown to attribute the radiation errors to specific cloud regimes. The net surface shortwave radiation is overestimated in all models throughout most of the simulation period. Cloud errors are shown to contribute most to this overestimation, although non-negligible contributions from the surface albedo exist in most models. Missing deep cloud events and/or simulating deep clouds with too weak cloud-radiative effects dominate in the cloud-related radiation errors. Some models have compensating errors between excessive occurrence of deep cloud, but largely underestimating their radiative effect, while other models miss deep cloud events altogether. Surprisingly, even the latter models tend to produce too much and too frequent afternoon surface precipitation. This suggests that rather than issues with the triggering of deep convection, cloud-radiative deficiencies are related to too weak convective cloud detrainment and too large precipitation efficiencies.

Description: Many weather forecast and climate models simulate warm surface air temperature (T 2m ) biases over mid-latitude continents during the summertime, especially over the Great Plains. We present here one of a series of papers from a multi-model intercomparison project (CAUSES: Cloud Above the United States and Errors at the Surface), which aims to evaluate the role of cloud, radiation, and precipitation biases in contributing to the T 2m bias using a short-term hindcast approach during the spring and summer of 2011. Observations are mainly from the Atmospheric Radiation Measurement (ARM) Southern Great Plains (SGP) sites. The present study examines the contributions of surface energy budget errors. All participating models simulate too much net shortwave and longwave fluxes at the surface but with no consistent mean bias sign in turbulent fluxes over the Central U.S. and SGP. Nevertheless, biases in the net shortwave and downward longwave fluxes, as well as surface evaporative fraction (EF) are contributors to T 2m bias. Radiation biases are largely affected by cloud simulations, while EF bias is largely affected by soil moisture modulated by seasonal accumulated precipitation and evaporation. An approximate equation based upon the surface energy budget is derived to further quantify the magnitudes of radiation and EF contributions to T 2m bias. Our analysis ascribes that a large EF underestimate is the dominant source of error in all models with a large positive temperature bias, whereas an EF overestimate compensates for an excess of absorbed shortwave radiation in nearly all the models with the smallest temperature bias.

Description: Solar wind dynamic pressure (Pdyn) enhancements have been observed to cause large-scale auroral brightening. The mechanism for this kind of auroral brightening is still a topic of current space research. Using the global piecewise parabolic method Lagrangian remap (PPMLR)-MHD simulation model, we investigate three auroral brightening events caused by dynamic pressure enhancement under different interplanetary magnetic field (IMF) conditions: (1) Bz 〈 0 and By 〉 0 on 11 August 2000, (2) Bz 〈 0 and By 〈 0 on 8 May 2001, and (3) Bz ≥ 0 on 21 January 2005. We show that the auroral location depends on the IMF conditions. Under southward IMF conditions, when By is negative, the duskside aurora is located more equatorward at around 70° magnetic latitude (MLAT) for all magnetic local times; when By is positive, the duskside aurora can even reach beyond 80° MLAT. A smaller and more localized response is seen when the IMF Bz is nearly zero or northward, as shown in previous studies. Our simulation results are consistent with these observations, indicating that the observed aurora activities could be caused by solar wind dynamic pressure enhancements. The simulation results suggest that the enhancement of Pdyn can increase the ionospheric transpolar potential and the corresponding field-aligned currents, leading to the observed auroral brightening.

Description: We examine the effects of the ionospheric conductance on the intensification of the westward electrojet current in the ionosphere based on the piecewise parabolic method with a Lagrangian remap (PPMLR) global MHD simulation model. The ionospheric conductance is empirically linked to the plasma pressure in the plasma sheet. The simulation results are consistent with observations: When the Pedersen and Hall conductances are small, the ionospheric current shows a two-cell pattern; when the conductances increase and the ratio ΣH/ΣP ≥ 2, an intense westward electrojet appears in the midnight sector. This intense westward electrojet is the Cowling current driven by the induced southward electric field due to the blockage of the northward Hall current from closure in the equatorial plasma sheet. The simulation shows the development of the Cowling electrojet is essential to the intensification of the westward electrojet in the ionosphere.

Description: Lower Cretaceous pedogenic carbonates exposed in SE China have been dated by U–Pb isotope measurements on single zircons taken from intercalated volcanic rocks, and the ages integrated with existing stratigraphy. 13 C values of calcretes range from –7.0 to –3.0 and can be grouped into five episodes of increasing–decreasing values. The carbon isotope proxy derived from these palaeosol carbonates suggests p CO 2 mostly in the range 1000–2000 parts per million by volume (ppmV) at S ( z ) (CO 2 contributed by soil respiration) = 2500 ppmV and 25°C during the Hauterivian–Albian interval ( c . 30 Ma duration). Such atmospheric CO 2 levels are 4–8 times pre-industrial values, almost double those estimated by geochemical modelling and much higher than those established from stomatal indices in fossil plants. Rapid rises in p CO 2 are identified for early Hauterivian, middle Barremian, late Aptian, early Albian and middle Albian time, and rapid falls for intervening periods. These episodic cyclic changes in p CO 2 are not attributed to local tectonism and volcanism but rather to global changes. The relationship between reconstructed p CO 2 and the development of large igneous provinces (LIPs) remains unclear, although large-scale extrusion of basalt may well be responsible for relatively high atmospheric levels of this greenhouse gas. Suggested levels of relatively low p CO 2 correspond in timing to intervals of regional to global enrichment of marine carbon in sediments and negative carbon isotope ( 13 C) excursions characteristic of the oceanic anoxic events OAE1a (Selli Event), Kilian and Paquier events (constituting part of the OAE 1b cluster) and OAE1d. Short-term episodes of high p CO 2 coincide with negligible carbon isotope excursions associated with the Faraoni Event and the Jacob Event. Given that episodes of regional organic carbon burial would draw down CO 2 and negative 13 C excursions indicate the addition of isotopically light carbon to the ocean–atmosphere system, controls on the carbon cycle in controlling p CO 2 during Early Cretaceous time were clearly complex and made more so by atmospheric composition also being affected by changes in silicate weathering intensity.

Description: This paper studies the dramatic decadal increase of Taiwan rainfall in the typhoon exit phase. The exit phase is defined as the time interval when a typhoon center leaves the Taiwan coast to 100 km away from the nearest coastline. Typhoons move across Taiwan through its northern (track N), central (track C), or southern (track S) part are selected for a statistical study. Taiwan hourly rainfall data of 21 surface gauge stations from the past 57 years are divided into two periods: 1960-1989 (P1) and 1987-2016 (P2). From P1 to P2, there are decadal increases of rainfall (~60%) and rainfall intensity (~30%, mm h -1 ) in the exit phase. There is also a decadal increase of the track-C typhoons. The southwest monsoon water vapor flux (SWF) in a local region southwest of Taiwan, as computed from the JRA-55 dataset, is substantially larger in the track-C typhoons than that in the track-N typhoons. Our analysis indicates that the increase of SWF leads to the increase of rainfall intensity. Moreover, both the enhanced SWF and the prolonged duration time contribute to the increased rainfall in the exit phase. Typhoon Morakot (2009), a track-C typhoon with extremely slow speed in the exit phase, produced the record-breaking rainfall. Model experiments and potential vorticity tendency diagnosis of Typhoon Morakot are used to understand the dynamics of increased duration time. The slowdown of typhoon motion is shown to be due to the asymmetric convection in the Taiwan Strait, which is produced by the interaction between typhoon circulation and southwest monsoon flow. The enhanced SWF and the prolonged duration time may explain the observed fact that the decadal rainfall increase is much larger than that of rainfall intensity in the exit phase.

Description: [1]  It was recently noted that substorms can occur even under prolonged northward interplanetary magnetic field (IMF) conditions. Based on the substorm list obtained from the IMAGE spacecraft, we perform a statistical study on the features of substorms during northward IMF interval. The strength of the substorm is represented by the AL index decrease and the total intensity of the auroral bulge. Four main features have been found as follows: (1) Most substorms occur soon after a southward IMF, and intense substorms are more likely to occur for short duration of northward IMF period (2 ~ 5 h), whereas no intense substorms occur after prolonged northward IMF condition. (2) There is a positive correlation between the strength of the substorm and the two solar wind parameters (the IMF | B y | and the solar wind dynamic pressure P d ). (3) The average strength of the substorms during the storm period is much larger than that of the substorms during the period without storm. Meanwhile, nearly all strong storm time substorms occurred either during the intense storm period, or during the late main phase or the early recovery phase of the storm. (4) About half of substorms, either an increase or a decrease in the solar wind dynamic pressure, are found within 30 min preceding each onset time. Such features indicate that the energy stored in the magnetotail during a previous southward IMF period is the main energy source for substorms under northward IMF condition, especially for intense substorms, and both the IMF | B y | and the solar wind dynamic pressure play an important role in the energy accumulation during the northward IMF period.

Description: Four compounds 1 to 4 (folic acid, methotrexate and 2 dyes) were used to interact with folate receptor (FR)α and FRβ. The interaction structures and binding energies of the bound complexes were investigated. In order to analyze the differences between FRα and FRβ complexes, the details of the weak intermolecular interactions were analyzed, and the frontier orbital properties of the FR complexes were studied by a dispersion complemented density functional tight-binding method. By comparing the different interaction properties of the 4 compounds with FRα and FRβ, the basic strategies for design of novel compound targeted with FR subtype were suggested. Further, a novel compound with high selectively with FRα based on compound 3 was designed to illustrate our conclusion. These data should be helpful for the design of novel molecules with extreme discerningly with FRα and FRβ. The variety of interaction models between ligands and FRα or FRβ was studied. By the difference between FRα and FRβ complexes, a novel compound with high selectively with FRα was designed, which will improve the recognition accuracy of the tumor cell and the efficiency of targeted drug delivery systems.

Description: This paper describes an investigation of the dynamics and acoustics of cloud cavitation, the structures which are often formed by the periodic breakup and collapse of a sheet or vortex cavity. This form of cavitation frequently causes severe noise and damage, though the precise mechanism responsible for the enhancement of these adverse effects is not fully understood. In this paper, we investigate the large impulsive surface pressures generated by this type of cavitation and correlate these with the images from high-speed motion pictures. This reveals that several types of propagating structures (shock waves) are formed in a collapsing cloud and dictate the dynamics and acoustics of collapse. One type of shock wave structure is associated with the coherent collapse of a well-defined and separate cloud when it is convected into a region of higher pressure. This type of global structure causes the largest impulsive pressures and radiated noise. But two other types of structure, termed 'crescent-shaped regions' and leading-edge structures' occur during the less-coherent collapse of clouds. These local events are smaller and therefore produce less radiated noise but the interior pressure pulse magnitudes are almost as large as those produced by the global events. The ubiquity and severity of these propagating shock wave structures provides a new perspective on the mechanisms reponsible for noise and damage in cavitating flows involving clouds of bubbles. It would appear that shock wave dynamics rather than the collapse dynamics of single bubbles determine the damage and noise in many cavitating flows.