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  • 1
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    Evidence of silicic acid leakage to the tropical Atlantic via Antarctic Intermediate Water during Marine Isotope Stage 4 (2013)
    John Wiley & Sons
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    Publication Date: 2022-05-25
    Description: Author Posting. © American Geophysical Union, 2013. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Paleoceanography 28 (2013): 307–318, doi:10.1002/palo.20030.
    Description: Antarctic Intermediate Water (AAIW) and Subantarctic Mode Water (SAMW) are the main conduits for the supply of dissolved silicon (silicic acid) from the deep Southern Ocean (SO) to the low-latitude surface ocean and therefore have an important control on low-latitude diatom productivity. Enhanced supply of silicic acid by AAIW (and SAMW) during glacial periods may have enabled tropical diatoms to outcompete carbonate-producing phytoplankton, decreasing the relative export of inorganic to organic carbon to the deep ocean and lowering atmospheric pCO2. This mechanism is known as the “silicic acid leakage hypothesis” (SALH). Here we present records of neodymium and silicon isotopes from the western tropical Atlantic that provide the first direct evidence of increased silicic acid leakage from the Southern Ocean to the tropical Atlantic within AAIW during glacial Marine Isotope Stage 4 (~60–70 ka). This leakage was approximately coeval with enhanced diatom export in the NW Atlantic and across the eastern equatorial Atlantic and provides support for the SALH as a contributor to CO2 drawdown during full glacial development.
    Description: The work is part of a wider project on the MIS 5/4 transition, supervised by S. B. and supported by NERC (UK) grant NE/F002734/1. K.R.H. is funded by National Science Foundation grant MCG-1029986. T.v.d.F. acknowledges funding from the European Commission (IRG 230828).
    Description: 2013-12-27
    Keywords: Silica leakage ; Diatom ; Carbon dioxide ; SAMW ; AAIW
    Repository Name: Woods Hole Open Access Server
    Type: Article
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  • 2
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    Abrupt changes in deep Atlantic circulation during the transition to full glacial conditions (2013)
    John Wiley & Sons
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    Publication Date: 2022-05-25
    Description: Author Posting. © American Geophysical Union, 2013. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Paleoceanography 28 (2013): 253–262, doi:10.1002/palo.20025.
    Description: Six Ocean Drilling Program (ODP) sites, in the Northwest Atlantic have been used to investigate kinematic and chemical changes in the “Western Boundary Undercurrent” (WBUC) during the development of full glacial conditions across the Marine Isotope Stage 5a/4 boundary (~70,000 years ago). Sortable silt mean grain size inline image measurements are employed to examine changes in near bottom flow speeds, together with carbon isotopes measured in benthic foraminifera and % planktic foraminiferal fragmentation as proxies for changes in water-mass chemistry. A depth transect of cores, spanning 1.8–4.6 km depth, allows changes in both the strength and depth of the WBUC to be constrained across millennial scale events. inline image measurements reveal that the flow speed structure of the WBUC during warm intervals (“interstadials”) was comparable to modern (Holocene) conditions. However, significant differences are observed during cold intervals, with higher relative flow speeds inferred for the shallow component of the WBUC (~2 km depth) during all cold “stadial” intervals (including Heinrich Stadial 6), and a substantial weakening of the deep component (~3–4 km) during full glacial conditions. Our results therefore reveal that the onset of full glacial conditions was associated with a regime shift to a shallower mode of circulation (involving Glacial North Atlantic Intermediate Water) that was quantitatively distinct from preceding cold stadial events. Furthermore, our chemical proxy data show that the physical response of the WBUC during the last glacial inception was probably coupled to basin-wide changes in the water-mass composition of the deep Northwest Atlantic.
    Description: This work was supported by the Natural Environment Research Council (NERC, UK) grants NE/F002734/1, NE/I006370/1 and NE/G004021/1. We also thank the Comer Science and Education Foundation and the Leverhulme Trust for financial support.
    Description: 2013-11-30
    Keywords: Western Boundary Undercurrent ; Abrupt climate change ; North Atlantic ; Glacial ; Ocean circulation
    Repository Name: Woods Hole Open Access Server
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  • 3
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    Calibration and application of B/Ca, Cd/Ca, and δ11B in Neogloboquadrina pachyderma (sinistral) to constrain CO2 uptake in the subpolar North Atlantic during the last deglaciation (2013)
    John Wiley & Sons
    Details
    Publication Date: 2022-05-25
    Description: Author Posting. © American Geophysical Union, 2013. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Paleoceanography 28 (2013): 237–252, doi:10.1002/palo.20024.
    Description: The North Atlantic and Norwegian Sea are prominent sinks of atmospheric CO2 today, but their roles in the past remain poorly constrained. In this study, we attempt to use B/Ca and δ11B ratios in the planktonic foraminifera Neogloboquadrina pachyderma (sinistral variety) to reconstruct subsurface water pH and pCO2 changes in the polar North Atlantic during the last deglaciation. Comparison of core-top results with nearby hydrographic data shows that B/Ca in N. pachyderma (s) is mainly controlled by seawater B(OH)4−/HCO3− with a roughly constant partition coefficient of 1.48 ± 0.15 × 10−3 (2σ), and δ11B in this species is offset below δ11B of the borate in seawater by 3.38 ± 0.71‰ (2σ). These values represent our best estimates with the sparse available hydrographic data close to our core-tops. More culturing and sediment trap work is needed to improve our understanding of boron incorporation into N. pachyderma (s). Application of a constant KD of 1.48 × 10−3 to high resolution N. pachyderma (s) B/Ca records from two adjacent cores off Iceland shows that subsurface pCO2 at the habitat depth of N. pachyderma (s) (~50 m) generally followed the atmospheric CO2 trend but with negative offsets of ~10–50 ppmv during 19–10 ka. These B/Ca-based reconstructions are supported by independent estimates from low-resolution δ11B measurements in the same cores. We also calibrate and apply Cd/Ca in N. pachyderma (s) to reconstruct nutrient levels for the same down cores. Like today's North Atlantic, past subsurface pCO2 variability off Iceland was significantly correlated with nutrient changes that might be linked to surface nutrient utilization and mixing within the upper water column. Because surface pCO2 (at 0 m water depth) is always lower than at deeper depths and if the application of a constant KD is valid, our results suggest that the polar North Atlantic has remained a CO2 sink during the calcification seasons of N. pachyderma (s) over the last deglaciation.
    Description: This research is funded by Lamont-Doherty Postdoctoral Fellowship, Lawrence Livermore Fellowship and the Australian National University (J.Y.), by NERC RAPID grant NER/T/S/2002/00436 (N. M. and D. T.), and by a NERC PhD studentship (J.R.).
    Description: 2013-11-30
    Keywords: Neogloboquadrina pachyderma (s) ; B/Ca, Cd/Ca, d11B ; Subsurface pH and pCO2 and nutrients
    Repository Name: Woods Hole Open Access Server
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  • 4
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    Holocene North Atlantic Overturning in an atmosphere-ocean-sea ice model compared to proxy-based reconstructions (2016)
    John Wiley & Sons
    Details
    Publication Date: 2022-05-25
    Description: Author Posting. © American Geophysical Union, 2015. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Paleoceanography 30 (2015): 1503–1524, doi:10.1002/2015PA002828.
    Description: Climate and ocean circulation in the North Atlantic region changed over the course of the Holocene, partly because of disintegrating ice sheets and partly because of an orbital-induced insolation trend. In the Nordic Seas, this impact was accompanied by a rather small, but significant, amount of Greenland ice sheet melting. We have employed the EMIC LOVECLIM and compared our model simulations with proxy-based reconstructions of δ13C, sortable silt, and magnetic susceptibility (κ) used to infer changes in past ocean circulation over the last 9000 years. The various reconstructions exhibit different long-term evolutions suggesting changes in either the overturning of the Atlantic in total or of subcomponents of the ocean circulation, such as the overflow waters across the Greenland-Scotland ridge. Thus, the question arises whether these reconstructions are consistent with each other or not. A comparison with model results indicates that δ13C, employed as an indicator of overturning, agrees well with the long-term evolution of the modeled Atlantic meridional overturning circulation (AMOC). The model results suggest that different long-term trends in subcomponents of the AMOC, such as Iceland-Scotland overflow water, are consistent with proxy-based reconstructions and allow some of the reconstructions to be reconciled with the modeled and reconstructed (from δ13C) AMOC evolution. We find a weak early Holocene AMOC, which recovers by 7 kyr B.P. and shows a weak increasing trend of 88 ± 1 mSv/kyr toward present, with relatively low variability on centennial to millennial timescales.
    Description: European Community's 7th Framework Program Grant Number: FP7/2007-2013; Marie-Curie Actions Grant Number: 238111
    Description: 2016-05-24
    Keywords: Holocene ; Paleoclimate modeling ; AMOC ; Sortable silt ; δ13C ; Magnetic susceptibility
    Repository Name: Woods Hole Open Access Server
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