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  • Copernicus  (18)
  • Beijing, China : Scienc Press  (1)
  • 1
    Monographie ausleihbar
    Monographie ausleihbar
    Atlas of climate physics of tropical Pacific ocean Scale not given (1990)
    Beijing, China : Scienc Press
    Details Verfügbarkeit
    Signatur: PIK N 456-16-90158
    Materialart: Monographie ausleihbar
    Seiten: IV, 190 S. (1 Atlas) , farbige Kt. , 26 cm
    ISBN: 7030021231
    Sprache: Unbestimmte Sprache
    Anmerkung: Chinese and English.
    Standort: A 18 - Bitte bestellen
    Zweigbibliothek: PIK Bibliothek
    Standort Signatur Erwartet Verfügbarkeit
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  • 2
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    Impacts of black carbon on the formation of advection–radiation fog during a haze pollution episode in eastern China (2019)
    Copernicus
    Details
    Publikationsdatum: 2019-06-12
    Beschreibung: Aerosols can not only participate in fog formation by acting as condensation nuclei of droplets but also modify the meteorological conditions such as air temperature and moisture, planetary boundary layer height (PBLH) and regional circulation during haze events. The impact of aerosols on fog formation, yet to be revealed, can be critical in understanding and predicting fog–haze events. In this study, we used the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) to investigate a heavy fog event during a multiday intense haze pollution episode in early December 2013 in the Yangtze River Delta (YRD) region in eastern China. Using the WRF-Chem model, we conducted four parallel numerical experiments to evaluate the roles of aerosol–radiation interaction (ARI), aerosol–cloud interaction (ACI), black carbon (BC) and non-BC aerosols in the formation and maintenance of the heavy fog event. We find that only when the aerosols' feedback processes are considered can the model capture the haze pollution and the fog event well. And the effects of ARI during the fog–haze episode in early December 2013 played a dominant role, while the effects of ACI were negligible. Furthermore, our analyses show that BC was more important in inducing fog formation in the YRD region on 7 December than non-BC aerosols. The dome effect of BC leads to an increase in air moisture over the sea by reducing PBLH and weakening vertical mixing, thereby confining more water vapor to the near-surface layer. The strengthened daytime onshore flow by a cyclonic wind anomaly, induced by contrast temperature perturbation over land and sea, transported moister air to the YRD region, where the suppressed PBLH and weakened daytime vertical mixing maintained the high moisture level. Then heavy fog formed due to the surface cooling at night. This study highlights the importance of anthropogenic emissions in the formation of advection–radiation fog in the polluted coastal areas.
    Print ISSN: 1680-7316
    Digitale ISSN: 1680-7324
    Thema: Geologie und Paläontologie
    Publiziert von Copernicus im Namen von European Geosciences Union.
    Standort Signatur Erwartet Verfügbarkeit
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  • 3
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    Transport, mixing and feedback of dust, biomass burning and anthropogenic pollutants in eastern Asia: a case study (2018)
    Copernicus
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    Publikationsdatum: 2018-11-19
    Beschreibung: Anthropogenic fossil fuel (FF) combustion, biomass burning (BB) and desert dust are the main sources of air pollutants around the globe but are particularly intensive and important for air quality in Asia in spring. In this study, we investigate the vertical distribution, transport characteristics, source contribution and meteorological feedback of these aerosols in a unique pollution episode that occurred in eastern Asia based on various measurement data and modeling methods. In this episode, the Yangtze River Delta (YRD) in eastern China experienced persistent air pollution, dramatically changing from secondary fine particulate pollution to dust pollution in late March 2015. The Eulerian and Lagrangian models were conducted to investigate the vertical structure, transport characteristics and mechanisms of the multi-scale, multisource and multiday air pollution episode. The regional polluted continental aerosols mainly accumulated near the surface, mixed with dust aerosol downwash from the upper planetary boundary layer (PBL) and middle–lower troposphere (MLT), and further transported by large-scale cold fronts and warm conveyor belts. BB smoke from Southeast Asia was transported by westerlies around the altitude of 3 km from southern China, was further mixed with dust and FF aerosols in eastern China and experienced long-range transport over the Pacific. These pollutants could all be transported to the YRD region and cause a structure of multilayer pollution there. These pollutants could also cause significant feedback with MLT meteorology and then enhance local anthropogenic pollution. This study highlights the importance of intensive vertical measurement in eastern China and the downwind Pacific Ocean and raises the need for quantitative understanding of environmental and climate impacts of these pollution sources.
    Print ISSN: 1680-7316
    Digitale ISSN: 1680-7324
    Thema: Geologie und Paläontologie
    Publiziert von Copernicus im Namen von European Geosciences Union.
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  • 4
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    The surface aerosol optical properties in the urban area of Nanjing, west Yangtze River Delta, China (2017)
    Copernicus
    Details
    Publikationsdatum: 2017-01-25
    Beschreibung: Observational studies of aerosol optical properties are useful for reducing uncertainties in estimations of aerosol radiative forcing and forecasting visibility. In this study, the observed near-surface aerosol optical properties in urban Nanjing are analysed from March 2014 to February 2016. Results show that near-surface urban aerosols in Nanjing are mainly from local emissions and the surrounding regions. They have lower loadings but are more scattering than aerosols in most cities in China. The annual mean aerosol extinction coefficient (EC), single-scattering albedo (SSA) and asymmetry parameter (ASP) at 550 nm are 381.96 Mm−1, 0.9 and 0.57, respectively. The aerosol absorption coefficient (AAC) is about 1 order of magnitude smaller than its scattering coefficient (SC). However, the absorbing aerosol has a larger Ångström exponent (AAE) value, 1.58 at 470∕660 nm, about 0.2 larger than the scattering aerosols (SAE). All the aerosol optical properties follow a near-unimodal pattern, and their values are mostly concentrated around their averages, accounting for more than 60 % of the total samplings. Additionally, they have substantial seasonality and diurnal variations. High levels of SC and AAC all appear in winter due to higher aerosol and trace gas emissions. AAE (ASP) is the smallest (largest) in summer, possibly because of high relative humidity (RH) which also causes considerably larger SC and smaller SAE, although intensive gas-to-particle transformation could produce a large number of finer scattering aerosols in this season. Seasonality of EC is different from the columnar aerosol optical depth. Larger AACs appear during the rush hours of the day while SC and back-scattering coefficient (Bsp) only peak in the early morning. Aerosols are fresher in the daytime than at night-time, leading to their larger Ångström exponent and smaller ASP. Different temporal variations between AAC and SC cause the aerosols to be more absorbing (smaller SSA) in autumn, winter and around rush hours. ASP has a good quasi-log-normal growth trend with increasing SC when RH is below 60 %. The correlation between AAC and SC at the site is close but a little smaller than that in suburban Nanjing in spring. Atmospheric visibility decreases exponentially with increasing EC or SC, more sharply in spring and summer, and it could be further deteriorated with increasing SSA and ASP.
    Print ISSN: 1680-7316
    Digitale ISSN: 1680-7324
    Thema: Geologie und Paläontologie
    Publiziert von Copernicus im Namen von European Geosciences Union.
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  • 5
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    Aerosol optical properties at SORPES in Nanjing, east China (2018)
    Copernicus
    Details
    Publikationsdatum: 2018-04-18
    Beschreibung: Aerosol optical properties (AOPs) and supporting parameters – particle number size distributions, PM2.5 mass concentrations, and the concentrations of trace gases (NOx and NOy) – were measured at SORPES, a regional background station in Nanjing, China from June 2013 to May 2015. The aerosol was highly scattering: the average scattering coefficient was σsp=403 ± 314 Mm−1, the absorption coefficient σap=26 ± 19 Mm−1, and the single-scattering albedo SSA = 0.93 ± 0.03 for green light. The SSA in Nanjing appears to be slightly higher than published values from several other sites in China and elsewhere. The average Ångström exponent of absorption (AAE) for the wavelength range 370–950 nm was 1.04 and the AAE range was 0.7–1.4. These AAE values can be explained with different amounts of non-absorbing coating on pure black carbon (BC) cores and different core sizes rather than contribution by brown carbon. The AOPs had typical seasonal cycles with high σsp and σap in winter and low ones in summer: the averages were σsp=544 ± 422 and σap=36 ± 24 Mm−1 in winter and σsp=342 ± 281 and σap=20 ± 13 Mm−1 in summer. The intensive AOPs had no clear seasonal cycles, the variations in them were rather related to the evolution of pollution episodes. The diurnal cycles of the intensive AOPs were clear and in agreement with the cycle of the particle number size distribution. The diurnal cycle of SSA was similar to that of the air photochemical age, suggesting that the darkest aerosol originated from fresh traffic emissions. A Lagrangian retroplume analysis showed that the potential source areas of high σsp and σap are mainly in eastern China. Synoptic weather phenomena dominated the cycle of AOPs on a temporal scale of 3–7 days. During pollution episodes, modeled boundary layer height decreased, whereas PM2.5 concentrations and σsp and σap typically increased gradually and remained high during several days but decreased faster, sometimes by even more than an order of magnitude within some hours. During the growth phase of the pollution episodes the intensive AOPs evolved clearly. The mass scattering efficiency MSE of PM2.5 grew during the extended pollution episodes from ∼ 4 to ∼ 6 m2 g−1 and the mass fraction of BCe decreased from ∼ 10 to ∼ 3 % during the growth phase of the episodes. Particle growth resulted in the backscatter fraction decreasing from more than 0.16 to less than 0.10, SSA growing from less than 0.9 to more than 0.95, and radiative forcing efficiency (RFE) changing from less than −26 W m−2 to more than −24 W m−2, which means that the magnitude of RFE decreased. The RFE probability distribution at SORPES was clearly narrower than at a clean background site which is in agreement with a published RFE climatology.
    Print ISSN: 1680-7316
    Digitale ISSN: 1680-7324
    Thema: Geologie und Paläontologie
    Publiziert von Copernicus im Namen von European Geosciences Union.
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  • 6
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    Multivariable integrated evaluation of model performance with the vector field evaluation diagram (2017)
    Copernicus
    Details
    Publikationsdatum: 2017-10-23
    Beschreibung: This paper develops a multivariable integrated evaluation (MVIE) method to measure the overall performance of climate model in simulating multiple fields. The general idea of MVIE is to group various scalar fields into a vector field and compare the constructed vector field against the observed one using the vector field evaluation (VFE) diagram. The VFE diagram was devised based on the cosine relationship between three statistical quantities: root mean square length (RMSL) of a vector field, vector field similarity coefficient, and root mean square vector deviation (RMSVD). The three statistical quantities can reasonably represent the corresponding statistics between two multidimensional vector fields. Therefore, one can summarize the three statistics of multiple scalar fields using the VFE diagram and facilitate the intercomparison of model performance. The VFE diagram can illustrate how much the overall root mean square deviation of various fields is attributable to the differences in the root mean square value and how much is due to the poor pattern similarity. The MVIE method can be flexibly applied to full fields (including both the mean and anomaly) or anomaly fields depending on the application. We also propose a multivariable integrated evaluation index (MIEI) which takes the amplitude and pattern similarity of multiple scalar fields into account. The MIEI is expected to provide a more accurate evaluation of model performance in simulating multiple fields. The MIEI, VFE diagram, and commonly used statistical metrics for individual variables constitute a hierarchical evaluation methodology, which can provide a more comprehensive evaluation of model performance.
    Print ISSN: 1991-959X
    Digitale ISSN: 1991-9603
    Thema: Geologie und Paläontologie
    Publiziert von Copernicus im Namen von European Geosciences Union.
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  • 7
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    On the characteristics of aerosol indirect effect based on dynamic regimes in global climate models (2016)
    Copernicus
    Details
    Publikationsdatum: 2016-03-04
    Beschreibung: Aerosol–cloud interactions continue to constitute a major source of uncertainty for the estimate of climate radiative forcing. The variation of aerosol indirect effects (AIE) in climate models is investigated across different dynamical regimes, determined by monthly mean 500 hPa vertical pressure velocity (ω500), lower-tropospheric stability (LTS) and large-scale surface precipitation rate derived from several global climate models (GCMs), with a focus on liquid water path (LWP) response to cloud condensation nuclei (CCN) concentrations. The LWP sensitivity to aerosol perturbation within dynamic regimes is found to exhibit a large spread among these GCMs. It is in regimes of strong large-scale ascent (ω500   0.1 mm day−1) contributes the most to the total aerosol indirect forcing (from 64 to nearly 100 %). Results show that the uncertainty in AIE is even larger within specific dynamical regimes compared to the uncertainty in its global mean values, pointing to the need to reduce the uncertainty in AIE in different dynamical regimes.
    Print ISSN: 1680-7316
    Digitale ISSN: 1680-7324
    Thema: Geologie und Paläontologie
    Publiziert von Copernicus im Namen von European Geosciences Union.
    Standort Signatur Erwartet Verfügbarkeit
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  • 8
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    Significant reduction of PM2.5 in eastern China due to regional-scale emission control: evidence from SORPES in 2011–2018 (2019)
    Copernicus
    Details
    Publikationsdatum: 2019-09-24
    Beschreibung: Haze pollution caused by PM2.5 is the largest air quality concern in China in recent years. Long-term measurements of PM2.5 and the precursors and chemical speciation are crucially important for evaluating the efficiency of emission control, understanding formation and transport of PM2.5 associated with the change of meteorology, and accessing the impact of human activities on regional climate change. Here we reported long-term continuous measurements of PM2.5, chemical components, and their precursors at a regional background station, the Station for Observing Regional Processes of the Earth System (SORPES), in Nanjing, eastern China, since 2011. We found that PM2.5 at the station has experienced a substantial decrease (−9.1 % yr−1), accompanied by even a very significant reduction of SO2 (−16.7 % yr−1), since the national “Ten Measures of Air” took action in 2013. Control of open biomass burning and fossil-fuel combustion are the two dominant factors that influence the PM2.5 reduction in early summer and winter, respectively. In the cold season (November–January), the nitrate fraction was significantly increased, especially when air masses were transported from the north. More NH3 available from a substantial reduction of SO2 and increased oxidization capacity are the main factors for the enhanced nitrate formation. The changes of year-to-year meteorology have contributed to 24 % of the PM2.5 decrease since 2013. This study highlights several important implications on air pollution control policy in China.
    Print ISSN: 1680-7316
    Digitale ISSN: 1680-7324
    Thema: Geologie und Paläontologie
    Publiziert von Copernicus im Namen von European Geosciences Union.
    Standort Signatur Erwartet Verfügbarkeit
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  • 9
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    Multivariable Integrated Evaluation of Model Performance with the Vector Field Evaluation Diagram (2017)
    Copernicus
    Details
    Publikationsdatum: 2017-05-12
    Beschreibung: This paper develops a multivariable integrated evaluation (MVIE) method to measure the overall performance of climate model in simulating multiple fields. The general idea of MVIE is to group various scalar fields into a vector field and compare the constructed vector field against the observed one using the vector field evaluation (VFE) diagram. The VFE diagram was devised based on the cosine relationship between three statistical quantities: root mean square length (RMSL) of a vector field, vector field similarity coefficient, and root mean square vector deviation (RMSVD). The three statistical quantities can reasonably represent the corresponding statistics between two multidimensional vector fields. Therefore, one can summarize the three statistics of multiple scalar fields using VFE diagram and facilitate the intercomparison of model performances. The VFE diagram can illustrate how much the overall root mean square deviation of various fields is attributable to the differences in the root mean square value and how much is due to the poor pattern similarity. The MVIE method can be flexibly applied to full fields (including both the mean and anomaly) or anomaly fields depending on the application. We also propose a multivariable integrated evaluation index (MIEI) which takes the amplitude and pattern similarity of multiple scalar fields into account. The MIEI is expected to provide a more accurate evaluation of model performance in simulating multiple fields. The MIEI, VFE diagram, and commonly used statistical metrics for individual variables constitute a hierarchical evaluation methodology, which can provide a more comprehensive evaluation on model performance.
    Print ISSN: 1991-9611
    Digitale ISSN: 1991-962X
    Thema: Geologie und Paläontologie
    Publiziert von Copernicus im Namen von European Geosciences Union.
    Standort Signatur Erwartet Verfügbarkeit
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  • 10
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    Transport, mixing, and feedback of dust, biomass burning and anthropogenic pollutants in eastern Asia: A case study (2018)
    Copernicus
    Details
    Publikationsdatum: 2018-06-27
    Beschreibung: Anthropogenic fossil fuel (FF) combustion, biomass burning (BB) and desert dust are main sources of air pollutants around the globe. The emission of the three sources in Asia are all very intensive and their influences on air quality is very important, especially in spring. In this study, we investigate the vertical distribution, transport characteristics, source contribution, and meteorological feedback of the dust, BB and FF aerosols in a unique pollution episode occurred in eastern Asia based on various measurement data and modelling methods. Ground-based observations indicated a persistent pollution episode dramatically changing from secondary fine particulate pollution to dust pollution in late March 2015 over the Yangtze River Delta (YRD) region, eastern China. The online-coupled meteorology–chemistry–aerosol modelling together with Lagrangian particle dispersion simulations were conducted to investigate the vertical structure, transport characteristics and mechanisms of the multi-scale, multi-source, and multi-day air pollution episode. The regional polluted continental aerosols mainly accumulated near surface by local anthropogenic emissions mixed with dust aerosols, downwash from the upper planetary boundary layer (PBL) and middle/lower troposphere (MLT), and further transported downwardly by large-scale cold fronts and warm conveyor belts. BB smoke from the Southeast Asia, mainly from forest burning in Indochina, were transported by westerlies around the altitude of 3km from southern China to eastern China, further mixed with dust and FF aerosols in eastern China and experienced long-range transport over the subtropical Pacific Ocean. The three pollutant sources could all transport to eastern China, especially the YRD region around the latitude of 30°N, caused a structure of multi-layer pollutants and well mixed pollutants there. These solar absorption aerosols from FF, BB and dust could also cause significant feedback with MLT meteorology and then enhance local anthropogenic pollution. This study highlights the importance of intensive vertical measurement in the eastern China and the downwind Pacific Ocean with a focus of understanding the complex physical and chemical processes of various pollution sources, and also raises the needs of quantitative understanding of environmental and climate impacts of these pollution sources in regional even global scales.
    Digitale ISSN: 1680-7375
    Thema: Geologie und Paläontologie
    Publiziert von Copernicus im Namen von European Geosciences Union.
    Standort Signatur Erwartet Verfügbarkeit
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