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  • 1
    Publication Date: 2014-12-31
    Description: Scattering type scanning near-field optical microscopy (s-SNOM) allows sub diffraction limited spatial resolution. Interferometric homodyne detection in s-SNOM can amplify the signal and extract vibrational responses based on sample absorption. A stable reference phase is required for a high quality homodyne-detected near-field signal. This work presents the development of a phase stabilization mechanism for s-SNOM to provide stable homodyne conditions. The phase stability is found to be better than 0.05 rad for the mid infrared light source. Phase stabilization results in improved near field images and vibrational spectroscopies. Spatial inhomogeneities of the boron nitride nanotubes are measured and compared.
    Print ISSN: 0003-6951
    Electronic ISSN: 1077-3118
    Topics: Physics
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  • 2
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 82 (1985), S. 4813-4830 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: In a recent paper (Az I), well-structured T=300 K resonance Raman (RR) profiles for the 1400, 1260, 900, and 2×825 cm−1 lines of azulene in CS2 and for the 825 cm−1 line of azulene in methanol were reported. Previously developed transform techniques were used to (1) compute RR profile line shapes directly from measured optical absorption spectra, and (2) extract ratios of Stokes loss parameters from the line shape scale factors. The transform analysis indicated that (1) our model assumptions (adiabatic and Condon approximations, harmonic phonons, atomic equilibrium position shifts, and small vibrational frequency shifts upon excitation to a single electronic state) are basically correct allowing forminor modifications, and (2) any deviations from these assumptions are likely to be larger for the 900 cm−1 mode and smaller for the 1400 and 1260 cm−1 modes. In this paper (Az II), we report model calculations of the optical absorption spectra, RR profile line shapes, and relative RR intensities. In these calculations, we use a recently proposed nonzero temperature multimode time-correlator modeling procedure. Compared with the conventional sum-over-states method, our time-correlator modeling procedure is superior in that (1) our optical absorption spectra and RR profiles computed via fast Fourier transform techniques have a practically unlimited spectral range and (2) the computing times are short for nonzero temperature multimode calculations. In our basic model, we adopt the assumptions of Az I and use seven azulene modes to obtain simultaneous good fits of the well-structured RR profile line shapes and optical absorption spectra. However, we find that the basic model does not account for the intensity of the 900 cm−1 Raman line relative to that of the 1400 cm−1 line, even though the individual profile line shape fits for these modes are very good. The basic model is therefore modified to allow mixing of the normal coordinates of these two modes. By introducing a single, relatively small mode-mixing parameter, we obtain a good fit of the relative RR intensities in addition to simultaneous detailed fits of the optical absorption spectra and RR profile line shapes. In an alternate approach, we modify our basic model and find that the inclusion of two relatively small non-Condon parameters, instead of one mode mixing parameter, can also produce simultaneous detailed fits of all of our optical absorption and RR data.A comparison of the two modified models solely on the basis of simplicity favors the mode-mixing model, since only one extra parameter is required to modify our basic model.
    Type of Medium: Electronic Resource
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  • 3
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Review of Scientific Instruments 70 (1999), S. 452-457 
    ISSN: 1089-7623
    Source: AIP Digital Archive
    Topics: Physics , Electrical Engineering, Measurement and Control Technology
    Notes: The detailed design of the magnetic diagnostic for ITER is presented. The system consists of groups of pickup coils and flux loops on the vessel wall, the back plate, and the divertor. These sensors provide the measurements for the equilibrium reconstruction and the fluctuation analysis. The system is supplemented by Rogowski coils for halo current measurements and by a diamagnetic loop. The complete system meets the measurement requirements, matching those of contemporary large divertor tokamaks. The maximum radiation exposure is such that the sensors will survive for the lifetime of the ITER. © 1999 American Institute of Physics.
    Type of Medium: Electronic Resource
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  • 4
    ISSN: 1089-7623
    Source: AIP Digital Archive
    Topics: Physics , Electrical Engineering, Measurement and Control Technology
    Notes: Key objectives of the first ten years of ITER operation are the investigation of the physics of burning plasmas and the demonstration of long-pulse ignited plasma technologies. These include studies of plasma confinement and stability, divertor operation, disruption mitigation and control, noninductive current drive, and steady state operation under conditions when the plasma is heated predominantly by alpha particles. The ITER operational plan envisages two and a half years for commissioning and initial operation with hydrogen plasmas at up to 100 MW of auxiliary heating power when initial tests of divertor operation and evaluation of disruption effects will be made. In order to meet the operational and programmatic goals, it will be necessary to make a wide range of plasma measurements. In this article the preliminary operational plan and physics program are presented and the implications for plasma measurements are outlined. © 1997 American Institute of Physics.
    Type of Medium: Electronic Resource
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  • 5
    ISSN: 1089-7623
    Source: AIP Digital Archive
    Topics: Physics , Electrical Engineering, Measurement and Control Technology
    Notes: Key objectives of the first ten years of ITER operation are the investigation of the physics of burning plasmas and the demonstration of long-pulse ignited plasma technologies. These include studies of plasma confinement and stability, divertor operation, disruption mitigation and control, noninductive current drive, and steady state operation under conditions when the plasma is heated predominantly by alpha particles. The ITER operational plan envisages two and a half years for commissioning and initial operation with hydrogen plasmas at up to 100 MW of auxiliary heating power when initial tests of divertor operation and evaluation of disruption effects will be made. In order to meet the operational and programmatic goals, it will be necessary to make a wide range of plasma measurements. In this article the preliminary operational plan and physics program are presented and the implications for plasma measurements are outlined. © 1997 American Institute of Physics.
    Type of Medium: Electronic Resource
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  • 6
    ISSN: 1089-7623
    Source: AIP Digital Archive
    Topics: Physics , Electrical Engineering, Measurement and Control Technology
    Notes: Reflectometry will be used on ITER to measure the density profile in the main plasma and divertor regions, and to measure the plasma position and shape in order to provide a standby reference for the magnetic diagnostics in long pulse discharges. The high temperatures of the ITER core and the resultant significant relativistic downshift of the second-harmonic electron cyclotron absorption imply that both low-field side O-mode and high-field side lower cut-off (X−l mode) systems are required to access the full plasma profile. A low-field side upper cut-off (X−u mode) system will also be required for measurements of the scrape-off layer. For measurements of the plasma position and shape, an O-mode system is optimum due to the large range of magnetic field along the plasma periphery and the wide range of possible plasma configurations achievable on ITER. A robust real-time calibration technique of the whole transmission line is required. It is likely that an accurate estimate of the position of the plasma will require the simultaneous use of signals from the profile reflectometer. For the divertor, profiles with peak densities in the range 1019–1022/m3 are to be measured with a target resolution of 3 mm. The large density range will necessitate the use of more than one system. Installing these reflectometers on ITER incurs additional difficulties such as the routing of the millimetre wave radiation around the complicated first wall and divertor structures and design of antennas able to operate through the first wall and blanket. © 1997 American Institute of Physics.
    Type of Medium: Electronic Resource
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  • 7
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 84 (1986), S. 2497-2502 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: Resonance Raman (RR) profiles of the 1005, 1155, and 1525 cm−1 modes of β-carotene dissolved in carbon disulfide have been measured at room temperature and at 172 K. Previous studies, based upon room temperature measurements, have indicated that inhomogeneous (i.e., site) broadening may be important for this system. Our measurements are the first RR data for this system at two temperatures. Such data are necessary in order to study the relative importance of inhomogeneous broadening and thermal broadening. Using previously developed transform techniques, we analyze our RR data by calculating profile line shapes directly from our measured optical absorption data for each temperature. The assumptions underlying this analysis do not include inhomogeneous broadening, and the calculations yield profile line shapes which are in quite good overall agreement with the measured profile line shapes for all three modes at both temperatures. We have also extended the transform calculations in order to incorporate inhomogeneous broadening. However, the agreement between the measured and calculated RR profile line shapes is not substantially improved by the inclusion of inhomogeneous broadening in the transform analysis.
    Type of Medium: Electronic Resource
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  • 8
    Publication Date: 2016-02-09
    Description: Investigating nanometer and micron sized materials thought to exhibit topological surface properties that can present a challenge, as clean surfaces are a pre-requisite for band structure measurements when using nano-ARPES or laser-ARPES in ultra-high vacuum. This issue is exacerbated when dealing with nanometer or micron sized materials, which have been prepared ex-situ and so have been exposed to atmosphere. We present the findings of an XPS study where various cleaning methods have been employed to reduce the surface contamination and preserve the surface quality for surface sensitive measurements. Microcrystals of the topological crystalline insulator SnTe were grown ex-situ and transferred into ultra high vacuum (UHV) before being treated with either atomic hydrogen, argon sputtering, annealing, or a combination of treatments. The samples were also characterised using the scanning electron microscopy, both before and after treatment. It was found that atomic hydrogen cleaning with an anneal cycle (200 °C) gave the best clean surface results.
    Print ISSN: 0003-6951
    Electronic ISSN: 1077-3118
    Topics: Physics
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