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  • American Institute of Physics (AIP)  (21)
  • Oxford University Press  (18)
  • American Meteorological Society (AMS)
  • 1
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 85 (1986), S. 1252-1260 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: Nine rotational transitions of v=0 X˜ 2B1 H2O+ have been measured by laser magnetic resonance. Optical combination differences have been combined with the LMR data in a weighted least-squares analysis using a Watson S-reduced rotational-fine structure Hamiltonian. Twenty-four molecular constants were simultaneously determined, including three hyperfine parameters and the axial components of both the anisotropic and rotational g tensors. The anisotropic g tensors are compared with their calculated values using the Curl relationship. An r0 structure was determined and is in good agreement with several ab initio results.
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  • 2
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 84 (1986), S. 2489-2496 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: Far IR rotational transitions between the four lowest rotational levels in the X 3Σ− vibronic ground states of OH+ and OD+ have been observed by laser magnetic resonance spectroscopy. Ground state molecular constants, including the three g factors, have been determined and employed in the calculation of a Born–Oppenheimer equilibrium geometry. The centrifugal distortion of the spin-rotation interaction is found to have a significant effect on the determination of other molecular constants. Hyperfine splittings have been resolved and analyzed for OH+, but could not be observed in OD+ spectra with a 6 MHz collision-broadened linewidth.
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  • 3
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 109 (1998), S. 906-911 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: The rotational structure of the vibrationless S1←S0 transition of pentacene has been investigated using a strongly collimated seeded supersonic argon beam. Because single rotational lines could not be completely resolved, a band contour analysis was performed. The rotational constants of the electronic ground state X 1A1g were found to be under the asymmetric rotor approximation A″=1320.6(9), B″=117.97(9), C″=108.28(15) MHz, whereas the differences to the first electronic excited state A 1B2u are ΔA=A′−A″=13.2(3), ΔB=−0.764(45), ΔC=−0.54(6) MHz. A new value of the band origin was determined to be ν00=18 648.996(4) cm−1 and the band type was confirmed to be of type b as proposed by symmetry arguments. Good agreement between observed and calculated spectra was obtained assuming planarity in both ground and excited state. From the fit procedure a rotational temperature of about 7 K was deduced. The nuclear statistical weights of the electronic ground state are reported. © 1998 American Institute of Physics.
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  • 4
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 105 (1996), S. 6088-6089 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: The relative stability of clusters of fullerenes has been investigated. By heating the clusters before ionization we have obtained mass spectra where only the monomer and (C60)13 are present in significant amounts. An approximately 20% increase of the activation energy for evaporation of a monomer from (C60)13 compared to that from (C60)14 explains the experimental results. © 1996 American Institute of Physics.
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  • 5
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 110 (1999), S. 10393-10402 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: Static electric polarizabilities of the S0(1A1g) ground electronic and the vibronically excited 61 S1(1B2u) state of benzene were measured by applying ultraviolet (UV) laser Stark spectroscopy. The experimental setup consisted of a frequency doubled tunable narrow-band continuous wave (cw) laser system operating at 259 nm, a molecular beam apparatus, and a capacitor capable of generating strong static and homogeneous electric fields up to 250 kV/cm. Experimental linewidths of less than 30 MHz were achieved for the rotational transitions, and Stark displacements of typically several 10 MHz could be detected. Stark patterns of 16 rotational lines were recorded and analyzed under different field strengths. Validity of second-order perturbation theory was confirmed by the observed effects, and the diagonal components of the polarizability tensors could be adjusted by a weighted least-squares technique. Results were applied to calculating Stark spectra and comparing them to experimental data. Good agreement could be found, except for an obscure singular perturbation within one rotational line. The new polarizabilities were compared to both experimental and theoretical results in the literature. Ground state data are in general agreement, whereas no comparable experimental work addressing the excited electronic state exists. Finally, polarizabilities of the beginning five polyacenes were compiled and compared with the benzene data. © 1999 American Institute of Physics.
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  • 6
    Electronic Resource
    Electronic Resource
    Woodbury, NY : American Institute of Physics (AIP)
    Applied Physics Letters 64 (1994), S. 830-832 
    ISSN: 1077-3118
    Source: AIP Digital Archive
    Topics: Physics
    Notes: The switching dynamics between TE- and TM-polarization states is studied in a strained ridge-waveguide InGaAsP/InP laser that exhibits TE/TM bistability. Using current modulation with frequencies between 50 and 500 MHz, three types of emission are distinguished. With increasing modulation amplitude, the laser runs through a region of TE emission, a range of stochastic switching between TE and TM modes, and a third region of regular polarization switching. The minimum modulation amplitude for regular switching rises strongly with frequency while the respective switching times decrease from about 700 ps at 50 MHz down to 250 ps around 500 MHz, corresponding to gigahertz mode switching.
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  • 7
    Electronic Resource
    Electronic Resource
    Woodbury, NY : American Institute of Physics (AIP)
    Applied Physics Letters 73 (1998), S. 3908-3910 
    ISSN: 1077-3118
    Source: AIP Digital Archive
    Topics: Physics
    Notes: Thermally induced strain caused by device packaging is studied in high-power semiconductor lasers by a noninvasive technique. Fourier-transform photocurrent measurements with intentionally strained laser array devices for 808 nm emission reveal spectral shifts of quantum-confined optical transitions in the optical active region. These shifts by up to 7 meV serve as a measure for strain and are compared with model calculations. For a given packaging architecture, about one quarter of the mounting-induced strain is transferred to the quantum-well region of the device. Spatially resolved measurements demonstrate a lateral strain gradient in the devices. © 1998 American Institute of Physics.
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  • 8
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 77 (1995), S. 6135-6144 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: New experimental and theoretical results on TE/TM bistability in 1.3 μm ridge-waveguide InGaAsP/InP bulk lasers at room temperature are presented. Measured polarization resolved light power–current (P–I) characteristics as well as lateral near- and far-field patterns are compared with results from a theoretical model based on the paraxial wave equations for TE- and TM-polarized modes and the diffusion equation for the carrier distribution. The model was numerically evaluated by use of the beam propagation method. The observed TE/TM bistability is explained by the interplay of three different effects: (i) Tensile stress of about 109 dyn/cm2 promotes the TM gain strongly enough to compete with the TE mode. (ii) Improved TM waveguiding due to an enhancement of the effective refractive index near the beam axis caused by carrier depletion with increasing current leads to the onset of TM lasing and TE/TM switching. (iii) The TE/TM transition is accompanied by an abrupt increase of spatial hole burning in the lateral carrier distribution. Because of this nonlinear effect, a lower current is needed to switch the laser back to TE, giving rise to a hysteresis loop in the P–I characteristics and to TE/TM polarization bistability. © 1995 American Institute of Physics.
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  • 9
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 75 (1994), S. 1442-1455 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: The effect of particulate volume fraction vp and diameter dp on the composite Young's modulus Ec is studied both experimentally, using a silica bead/epoxy system, as well as with the help of computer simulations. The experimental and simulation results show that for a given particulate size, the overall Ec vs vp curve displays a concave upward shape and not a linear shape. This superlinear trend of the data implies that the average strain normalized to the applied strain λ=ε¯p/εc transferred to the particulates increases with volume fraction. The above finding is explained in terms of a mean-field picture, where a single particle interacts with an effective medium consisting of the remaining particles embedded in the matrix. As the modulus of the effective medium surrounding a reference particle increases with vp, the modulus mismatch between the reference particulate and the medium is consequently reduced. This leads to an overall increase in the normalized average strain λ transferred to each particulate as vp is increased. The experimental results using silica particulates with various sizes dp, as well as the simulation results, show that smaller particulates provide an increased composite modulus as compared to larger particulates, at constant vp. General equations are developed, which relate the composite modulus to the average particle stress or strain, given only information about the volume fraction and the Young's modulus of each of the phases present.Through the application of these relations, it is found that smaller particulates display a greater amount of normalized average strain λ transferred than larger particulates. The effect of particulate Young's modulus Ep in combination with particulate size on the resulting Ec is also studied using simulations only. It is found that for a low particulate to matrix modulus ratio Ep/Em, the particulate size has very little influence on Ec. Moreover, the shape of the Ec vs vp curve can be well approximated by a straight line up to large values of vp. On the other hand, as the ratio Ep/Em is increased, the superlinear trend of the composite modulus Ec vs vp data is more apparent. This results in a smaller range of the Ec vs vp curve, which can be approximated by a linear function. It is also found that the extent of this linear region also decreases with particle size.
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  • 10
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 81 (1997), S. 2064-2069 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: Light emission from a ridge waveguide 1.3 μm InGaAsP/InP semiconductor laser pumped both electrically and optically was analyzed by polarization- and time-resolved measurements. The electric and the optical excitation was realized with a dc-bias current and with 150 ps pulses from a Q-switched Nd-YAG laser at 1.064 μm wavelength, respectively. The pump light was introduced into the InGaAsP/InP laser through a window opened in the substrate gold contact. The steady-state P–I characteristics of the semiconductor laser exhibited a transition from TM- to TE-polarized light emission if the injection current surpasses a certain value that depends on the heatsink temperature. Depending on the dc-bias current and the optical pulse power, a variety of different emission characteristics of the semiconductor laser were observed: pure TE or TM pulsations, in combination with a background cw emission in some cases; simultaneous emission of TE and TM pulses and switching between TM and TE emission states with switching times as short as 30 ps. © 1997 American Institute of Physics.
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