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  • American Institute of Physics (AIP)  (154)
  • 2015-2019  (20)
  • 1985-1989  (134)
  • 1
    Publication Date: 2015-11-24
    Description: The patterning of graphene by a 30 kV Ga + focused ion beam (FIB) is studied by in-situ and ex-situ Raman spectroscopy. It is found that the graphene surrounding the patterned target area can be damaged at remarkably large distances of more than 10  μ m. We show that scattering of the Ga ions in the residual gas of the vacuum system is the main cause of the large range of lateral damage, as the size and shape of the tail of the ion beam were strongly dependent on the system background pressure. The range of the damage was therefore greatly reduced by working at low pressures and limiting the total amount of ions used. This makes FIB patterning a feasible alternative to electron beam lithography as long as residual gas scattering is taken into account.
    Print ISSN: 0003-6951
    Electronic ISSN: 1077-3118
    Topics: Physics
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  • 2
    Publication Date: 2016-07-07
    Description: The counter-propagating shear campaign is examining instability growth and its transition to turbulence in the high-energy-density physics regime using a laser-driven counter-propagating flow platform. In these experiments, we observe consistent complex break-up of and structure growth in a tracer layer placed at the shear flow interface during the instability growth phase. We present a wavelet-transform based analysis technique capable of characterizing the scale- and directionality-resolved average intensity perturbations in static radiographs of the experiment. This technique uses the complete spatial information available in each radiograph to describe the structure evolution. We designed this analysis technique to generate a two-dimensional power spectrum for each radiograph from which we can recover information about structure widths, amplitudes, and orientations. The evolution of the distribution of power in the spectra for an experimental series is a potential metric for quantifying the structure size evolution as well as a system’s evolution towards isotropy.
    Print ISSN: 0034-6748
    Electronic ISSN: 1089-7623
    Topics: Electrical Engineering, Measurement and Control Technology , Physics
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  • 3
    Publication Date: 2016-07-01
    Description: In this study, we generalize the impulse response approach and Poisson statistics proposed by Smith [Phys. Rev. B 64 , 155106 (2001)] to evaluate the longitudinal and transverse magneto-optical conductivities in an electron gas system in Faraday geometry. Comparing with the standard Drude model, the coefficients a n are introduced in the Drude-Smith formula to describe the backscattering or localization effect for the n th electronic scattering event. Such a formula can also be applied to study the elements of the dielectric function matrix in the presence of magnetic and radiation fields in electron gas systems. This theoretical work is primely motivated by recent experimental activities in measuring the real and imaginary parts of longitudinal and transverse magneto-optical conductivities in condensed matter materials and electronic devices using terahertz time-domain spectroscopy. We believe that the results obtained from this study can provide an appropriate theoretical tool in reproducing the experimental findings and in fitting with experimental data to determine the important sample and material parameters.
    Print ISSN: 0021-8979
    Electronic ISSN: 1089-7550
    Topics: Physics
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  • 4
    Publication Date: 2015-04-18
    Description: An indirectly-driven shock tube experiment fielded on the National Ignition Facility (NIF) was used to create a high-energy-density hydrodynamics platform at unprecedented scale. Scaling up a shear-induced mixing experiment previously fielded at OMEGA, the NIF shear platform drives 130  μ m/ns shocks into a CH foam-filled shock tube (∼ 60 mg/cc) with interior dimensions of 1.5 mm diameter and 5 mm length. The pulse-shaping capabilities of the NIF are used to extend the drive for 〉10 ns, and the large interior tube volumes are used to isolate physics-altering edge effects from the region of interest. The scaling of the experiment to the NIF allows for considerable improvement in maximum driving time of hydrodynamics, in fidelity of physics under examination, and in diagnostic clarity. Details of the experimental platform and post-shot simulations used in the analysis of the platform-qualifying data are presented. Hydrodynamic scaling is used to compare shear data from OMEGA with that from NIF, suggesting a possible change in the dimensionality of the instability at late times from one platform to the other.
    Print ISSN: 1070-664X
    Electronic ISSN: 1089-7674
    Topics: Physics
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  • 5
    Publication Date: 2015-06-25
    Description: Counter-propagating shear experiments conducted at the OMEGA Laser Facility have been evaluating the effect of target initial conditions, specifically the characteristics of a tracer foil located at the shear boundary, on Kelvin-Helmholtz instability evolution and experiment transition toward nonlinearity and turbulence in the high-energy-density (HED) regime. Experiments are focused on both identifying and uncoupling the dependence of the model initial turbulent length scale in variable-density turbulence models of k- ϵ type on competing physical instability seed lengths as well as developing a path toward fully developed turbulent HED experiments. We present results from a series of experiments controllably and independently varying two initial types of scale lengths in the experiment: the thickness and surface roughness (surface perturbation scale spectrum) of a tracer layer at the shear interface. We show that decreasing the layer thickness and increasing the surface roughness both have the ability to increase the relative mixing in the system, and thus theoretically decrease the time required to begin transitioning to turbulence in the system. We also show that we can connect a change in observed mix width growth due to increased foil surface roughness to an analytically predicted change in model initial turbulent scale lengths.
    Print ISSN: 1070-664X
    Electronic ISSN: 1089-7674
    Topics: Physics
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  • 6
    Publication Date: 2016-12-08
    Description: In this study we present a combined optical sizing and acoustical characterization technique for the study of the dynamics of single freely-floating ultrasound contrast agent microbubbles exposed to long burst ultrasound excitations up to the milliseconds range. A co-axial flow device was used to position individual microbubbles on a streamline within the confocal region of three ultrasound transducers and a high-resolution microscope objective. Bright-field images of microbubbles passing through the confocal region were captured using a high-speed camera synchronized to the acoustical data acquisition to assess the microbubble response to a 1-MHz ultrasound burst. Nonlinear bubble vibrations were identified at a driving pressure as low as 50 kPa. The results demonstrate good agreement with numerical simulations based on the shell-buckling model proposed by Marmottant et al . [J. Acoust. Soc. Am. 118 , 3499–3505 (2005)]. The system demonstrates the potential for a high-throughput in vitro characterization of individual microbubbles.
    Print ISSN: 0003-6951
    Electronic ISSN: 1077-3118
    Topics: Physics
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  • 7
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 91 (1989), S. 6989-7001 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: The theory of atoms in molecules is extended to the case where the molecule is in the presence of an electromagnetic field. This theory is based upon a generalization of quantum mechanics to an open system, as obtained through a corresponding extension of Schwinger's principle of stationary action. The extension of this principle is possible only if the open system satisfies a particular boundary condition, one which is expressed as a constraint on the variation of the action integral. This is the condition that it be bounded by a surface of zero flux in the gradient vector field of the charge density, the definition of an atom in a molecule. It is shown that this boundary constraint again suffices to define an atom as a quantum subsystem when the molecule is in the presence of an electromagnetic field. The mechanics of an open system and its properties are determined by the fluxes in corresponding vector current densities through its surface. As in the fieldfree case, the obtainment of these currents from the variation of the action integral is a direct result of the variation of the atomic surface and of the imposition of the variational constraint on its boundary. The currents in this case consist of a paramagnetic and a diamagnetic contribution, currents whose presence are a necessary requirement for the description of the properties of a system in the presence of external fields. The variational statement of the Heisenberg equation of motion obtained from the principle of stationary action is used to derive the Ehrenfest force and virial theorems for an atom in a molecule in the presence of external electric and magnetic fields. In this case, there are forces acting on the interior of the atom which arise from the magnetic pressures acting on its surface. It is shown that the molecular electric polarizability and magnetic susceptibility, like other properties, are rigorously expressible as a sum of atomic contributions.
    Type of Medium: Electronic Resource
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  • 8
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 88 (1988), S. 3792-3804 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: This paper reports on the effect of electron correlation on the topological properties of the charge density and its associated gradient vector and Laplacian fields. The properties of these fields define the atoms, their reactivity, and the structure of a molecular system within the theory of atoms in molecules. The singlet and triplet states of CH2, CF2, and SiH2 are investigated using a configuration interaction method which includes all single and double excitations with respect to suitable zero-order reference wave functions, together with a number of hydrocarbon molecules including unsaturated and geometrically strained systems for which the correlation is introduced via the generalized valence bond approach. It is found that the correlated charge distributions possess the same number and kind of critical points in both the ρ(r) and ∇2ρ(r) fields as are found for SCF charge distributions. Thus the topology of a charge distribution and the structure it defines are unaffected by the addition of Coulomb correlation. The quantitative changes in the properties of the charge density at the critical points in both ρ(r) and ∇2ρ(r) induced by correlation are found to be small in magnitude and to be more pronounced for shared or covalent atomic interactions than for systems with pronounced charge transfer between the atoms. The properties of the atoms in these molecules also exhibit correspondingly small changes in value.
    Type of Medium: Electronic Resource
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  • 9
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 87 (1987), S. 4241-4241 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Type of Medium: Electronic Resource
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  • 10
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 87 (1987), S. 6354-6363 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: Extended x-ray absorption fine structure (EXAFS) studies were conducted on catalysts containing platinum and rhenium, or palladium and rhenium, on alumina. The atomic ratio of rhenium to either platinum or palladium was close to one in the catalysts investigated. The metallic entities in the catalysts were characterized by analyses of the EXAFS associated with the LI absorption edge of platinum, the LIII edge of rhenium, and the K absorption edge of palladium. It was concluded that Pt–Re and Pd–Re bimetallic clusters are present in the catalysts. However, the clusters have regions rich in rhenium and other regions which are rich in either platinum or palladium. Exposure of Pt–Re clusters to sulfur has little influence on their structure.
    Type of Medium: Electronic Resource
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