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  • 1
    Publication Date: 2020-02-06
    Description: Shallow gas migration along hydrocarbon wells constitutes a potential methane emission pathway that currently is not recognized in any regulatory framework or greenhouse gas inventory. Recently, the first methane emission measurements at three abandoned offshore wells in the Central North Sea (CNS) were conducted showing that considerable amounts of biogenic methane originating from shallow gas accumulations in the overburden of deep reservoirs were released by the boreholes. Here, we identify numerous wells poking through shallow gas pockets in 3D seismic data of the CNS indicating that about one third of the wells may leak, potentially releasing a total of 3-17 kt of methane per year into the North Sea. This poses a significant contribution to the North Sea methane budget. A large fraction of this gas (~42 %) may reach the atmosphere via direct bubble transport (0-2 kt yr-1) and via diffusive exchange of methane dissolving in the surface mixed layer (1-5 kt yr-1), as indicated by numerical modeling. In the North Sea and in other hydrocarbon-prolific provinces of the world shallow gas pockets are frequently observed in the sedimentary overburden and aggregate leakages along the numerous wells drilled in those areas may be significant.
    Type: Article , PeerReviewed , info:eu-repo/semantics/article
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  • 2
    Publication Date: 2019-10-17
    Description: Methane (CH4) emissions from small rivers and streams, particularly via ebullition, are currently under-represented in the literature. Here, we quantify the methane effluxes and drivers in a small, Northern European river. Methane fluxes are comparable to those from tropical aquatic systems, with average emissions of 320 mg CH4 m-2 d-1. Two important drivers of methane flux variations were identified in the studied system: 1) temperature-driven sediment methane ebullition and 2) flow-dependent contribution suspected to be hydraulic exchange with adjacent wetlands and small side-bays. This flow-dependent contribution to river methane loading is shown to be negligible for flows less than 4 m3 s-1, and greater than 50% as flows exceed 7 m3 s-1. While the temperature - ebullition relationship is comparable to other systems, the flow rate dependency has not been previously demonstrated. In general, we found that about 80% of the total emissions were due to methane bubbles. Applying ebullition rates to global estimates for fluvial systems, which currently are not considered, could dramatically increase emission rates to ranges from lakes or wetlands. This work illustrates that small rivers can emit significant methane, and highlights the need for further studies, especially the link between hydrodynamics and connected wetlands.
    Type: Article , PeerReviewed
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  • 3
    Publication Date: 2022-01-31
    Description: Carbon dioxide (CO2) capture and storage (CCS) has been discussed as a potentially significant mitigation option for the ongoing climate warming. Natural CO2 release sites serve as natural laboratories to study subsea CO2 leakage in order to identify suitable analytical methods and numerical models to develop best-practice procedures for the monitoring of subseabed storage sites. We present a new model of bubble (plume) dynamics, advection-dispersion of dissolved CO2, and carbonate chemistry. The focus is on a medium-sized CO2 release from 294 identified small point sources around Panarea Island (South-East Tyrrhenian Sea, Aeolian Islands, Italy) in water depths of about 40–50 m. This study evaluates how multiple CO2 seep sites generate a temporally variable plume of dissolved CO2. The model also allows the overall flow rate of CO2 to be estimated based on field measurements of pH. Simulations indicate a release of ∼6900 t y–1 of CO2 for the investigated area and highlight an important role of seeps located at 〉20 m water depth in the carbon budget of the Panarea offshore gas release system. This new transport-reaction model provides a framework for understanding potential future leaks from CO2 storage sites.
    Type: Article , PeerReviewed , info:eu-repo/semantics/article
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  • 4
    Publication Date: 2024-04-11
    Description: Groundwater discharge into the sea occurs along many coastlines around the world in different geological settings and constitutes an important component of global water and matter budget. Estimates of how much water flows into the sea worldwide vary widely and are largely based on onshore studies and hydrological or hydrogeological modeling. In this study, we propose an approach to quantify a deep submarine groundwater outflow from the seafloor by using autonomously measured ocean surface data, i.e., 222Rn as groundwater tracer, in combination with numerical modeling of plume transport. The model and field data suggest that groundwater outflows from a water depth of ∼100 m can reach the sea surface implying that several cubic meters per second of freshwater are discharged into the sea. We postulate an extreme rainfall event 6 months earlier as the likely trigger for the groundwater discharge. This study shows that measurements at the sea surface, which are much easier to conduct than discharge measurements at the seafloor, can be used not only to localize submarine groundwater discharges but, in combination with plume modeling, also to estimate the magnitude of the release flow rate.
    Type: Article , PeerReviewed
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