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  • 1
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: The effect of an electric field on GMR oxide films was studied in a MOSFET configuration where the gate dielectric was a layer of SrTiO3 epitaxially grown on an underlying layer of the manganate which served as the source/drain. The response of the manganate channel was studied for different gate voltages. The following significant features were observed. The peak resistance temperature shifted to lower temperature for both polarities of the field. The resistance change varied quadratically with the field indicating the dominance of strain or polarization effects. In dynamical studies of the system using the gate voltage as an excitation the system showed anomalous slowing down near the peak of the resistivity. These results are understood on the basis of a stress effect on the film due to electro-elastic effects in the SrTiO3 layer, which introduces a tensile stress in the manganate layer upon the application of a gate voltage. The anomalous slowing down of the system near the ferromagnetic phase transition suggests a strong coupling between the spins, transport and structural distortions in the system. © 1996 American Institute of Physics.
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  • 2
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: There are different models which to try to explain the transport properties of the manganese oxides in terms of magnetic polarons, Zener double exchange and Jahn-Teller distortions of the lattice which is temperature dependent. Using Rutherford backscattering techniques (2–3 MeV He ions) we are measuring the presence of lattice distortions by studying the angular scans in the channeling mode. The angular widths (FWHM) can be used to extract both dynamic and static displacements of the atoms from their equilibrium sites. The technique is extremely powerful in the sense that local uncorrected displacements as small as 0.01 A(ring) from the equilibrium position can be detected. The extraction of the physics from the data is relatively straight forward compared to other techniques such as XRD or neturon scattering. Using a variable temperature backscattering system at our center (one of three or four systems around the world) the angular width (FWHM) is found to exhibit a dramatic change with temperature increasing with decreasing temperature showing a possible correlation with both the transport and magnetic properties. The results suggest a decrease in the lattice disorder with reduced temperature far in excess of what one would predict on the basis of a simple Debye behavior. The reduction in the lattice disorder correlates very well with the resistance vs temperature dependence. A variety of manganese oxide epitaxial thin films grown by pulsed laser deposition have been studied and the data suggests a role for structural distortions in any mechanism to explain the transport properties of these materials. © 1996 American Institute of Physics.
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  • 3
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: Magnetoresistivity values of the order of 106% (and in some cases even higher) have been obtained in epitaxial AxB1−xMnO3−y (A=La,Nd; B=Ca,Sr,Ba) thin films grown by pulsed laser deposition. Ferromagnetic resonance experiments suggest a granular-type behavior with conducting ferromagnetic regions (Rcond〈10 mΩ cm) in a less conducting matrix (Rinsulazting(approximately-greater-than)100.Rcond). Ion channeling experiments over a range of temperatures clearly reveal the existence of structural distortion at the peak resistivity temperature TP. Systematic studies of samples prepared under a variety of oxygenation conditions show that the resistivity above TP can be modeled with a single functional form: Rcond≈eΔ/kT, where Δ, the activation energy, is of the order of 50–200 meV. This suggests that these different samples represent the same basic material in a semiconducting matrix, with differing volume fractions of the two components which depends on the processing conditions. These "colossal'' values of MR have been obtained at temperatures lower than room temperature and at fields of the order of a few Teslas, both of which are impediments to the development of viable MR sensor and nonvolatile storage technologies.We are therefore addressing the critical scientific and technological issues through a variety of materials integration approaches. Using structural chemistry and lattice matching as fundamental guiding principles, we are growing epitaxial heterostructure superlattices consisting of the CMR oxides interleaved with magnetic perovskites such as La–Sr–Co–O (metallic ferromagnet), rare earth–Fe–O (ferromagnetic insulator). We are also exploring the possibility of using the semiconducting properties of these materials in an all-perovskite field effect transistor device. In this presentation, we will describe our progress to date on these studies to enhance the field and temperature dependence of the MR properties and explore new device architectures that utilize the inherently novel properties of these materials. © 1996 American Institute of Physics.
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  • 4
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: Thermally induced chemical transformations at the interface between a 100 nm α–Fe2O3 and a polycrystalline α–Al2O3 substrate are studied and compared for the cases of the as-formed and ion bombarded interfaces. The thermal annealings are carried out under vacuum at 450 °C for different time durations and the transformations are examined by conversion electron Mössbauer spectroscopy. It is shown that in the sample prebombarded with 110 keV Ar+ ions, the formation of Fe3−xAlxO4, FeAl2O4, and FeO phases is favored at variance with a nonbombarded sample in which primarily a defective Fe3O4-y phase is produced with some amount of FeO. This difference is explained in terms of the annealing process of the oxygen vacancies produced during Ar implantation near the interfacial region. © 1996 American Institute of Physics.
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  • 5
    Electronic Resource
    Electronic Resource
    Woodbury, NY : American Institute of Physics (AIP)
    Applied Physics Letters 72 (1998), S. 1113-1115 
    ISSN: 1077-3118
    Source: AIP Digital Archive
    Topics: Physics
    Notes: C-axis oriented La0.7Sr0.3MnO3−δ (LSMO) films were fabricated on the top of SrTiO3/YBa2Cu3O7 grown on MgO (001) substrates. From x-ray φ-scan and planar transmission electron microscopy measurements, the LSMO layer in the LSMO/SrTiO3/YBa2Cu3O7/MgO heterostructure is found to have coherent in-plane grain boundaries with a predominance of 45° rotations (between [100] and [110] grains) in addition to the cube-on-cube epitaxial relationship. Also, epitaxial LSMO/Bi4Ti3O12/LaAlO3 (001) and c-axis textured LSMO/Bi4Ti3O12/SiO2/Si (001) with random in-plane grain boundaries are introduced as the counterparts for comparison. The resistivity and magnetoresistance (MR) of LSMO layer were measured and compared. The low field MR at low temperature shows a dramatic dependence on the nature of the grain boundary. An attempt is made to interpret these results on the basis of correlation between the magnetic properties and grain structures. © 1998 American Institute of Physics.
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  • 6
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 78 (1995), S. 5204-5205 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: We have found evidence through optical spectroscopy that AgO is indeed generated in the laser plume during pulsed laser deposition of YBa2Cu3O7−δ (YBCO) thin films using Ag-doped YBCO targets. This supports our earlier conjecture that formation of AgO in the plume and its subsequent dissociation at the elevated substrate temperature (since AgO is unstable above 350 °C) provides active oxygen to the YBCO lattice, thereby increasing oxygen incorporation during growth of YBCO thin films. © 1995 American Institute of Physics.
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  • 7
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: Epitaxial films of La0.7Ca0.3MnO3 have been irradiated with 90 MeV oxygen ions at different dose values ranging from 1011–1014 ions/cm2. The structural, magnetization, and magnetotransport properties have been studied as a function of the ion dose. It is found that the properties change gradually up to a dose of 1013 ions/cm2; however, drastic changes occur when the sample is irradiated at the higher dose of 1014 ions/cm2. Specifically, this sample exhibits a large, nearly temperature independent magnetoresistance in the low temperature regime. The Rutherford backscattering channeling data bring out the presence of defects in the irradiated films. The x-ray diffraction data, the temperature dependence of resistivity and magnetization, and the low temperature magnetic hysterisis data collectively indicate the presence of two different phases in the sample irradiated at 1014 ions/cm2. The surface morphology of this film, observed by atomic force microscopy, exhibits swelling, presumably due to subsurface clustering of point defects. The observed results are analyzed in terms of point defect induced random spin disorder and its effect on the magnetotransport properties. © 1998 American Institute of Physics.
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  • 8
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: (110) oriented La1−δMn1−δO3 thin films with different oxygen content were grown on (001) LaAlO3 substrates by pulsed laser deposition. Samples prepared in higher oxygen partial pressures show a ferromagnetic transition around 200 K. The transport is thermally activated with a change in slope at the ferromagnetic transition. Samples prepared and annealed in vacuum show signatures of mixed ferromagnetic and antiferromagnetic phases, and are insulators. The pure antiferromagnetic phase (as expected and observed in bulk materials with optimum oxygen stoichiometry) was not obtained in our experiments, even in the strongly reduced films. © 1999 American Institute of Physics.
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  • 9
    ISSN: 1077-3118
    Source: AIP Digital Archive
    Topics: Physics
    Notes: Thin films of Ag-added La2/3Ca1/3MnO3 exhibit enhancement of several desirable characteristics over the pristine counterparts. We find that the addition of Ag results in a pronounced increase in the insulator–metal transition temperature (Tp) and ferromagnetic transition temperature (Tc). There is also a remarkable improvement in the magnetic and electrical homogeneity of the samples as indicated by narrower ferromagnetic resonance linewidths and narrower resistive transitions, respectively. The observed improvement in properties is inferred to be largely associated with improved oxygen stoichiometry of the films although microstructural effects are not ruled out. © 1999 American Institute of Physics.
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  • 10
    Electronic Resource
    Electronic Resource
    Woodbury, NY : American Institute of Physics (AIP)
    Applied Physics Letters 73 (1998), S. 689-691 
    ISSN: 1077-3118
    Source: AIP Digital Archive
    Topics: Physics
    Notes: A very large positive magnetoresistance (MR) has been discovered in a Fe3O4/SrTiO3/ La0.7Sr0.3MnO3 heterostructure for the transport perpendicular to the layer planes and applied magnetic field in the film plane. The observed MR features do not show any obvious correlation with the hysteresis behavior of the ferromagnetic bilayers. A possible explanation of these results is given in terms of the relative differences in the majority and minority spin bands of the two ferromagnetic layers and the field induced modifications of domain structures therein. © 1998 American Institute of Physics.
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