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  • 2005-2009  (5)
  • 2006  (5)
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  • 2005-2009  (5)
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  • 1
    Publication Date: 2006-08-15
    Description: A global chemical transport model of the atmosphere [the Model for Ozone and Related Tracers, version 2 (MOZART-2)] driven by prescribed surface emissions and by meteorological fields provided by the ECHAM5/Max Planck Institute Ocean Model (MPI-OM-1) coupled atmosphere–ocean model is used to assess how expected climate changes (2100 versus 2000 periods) should affect the chemical composition of the troposphere. Calculations suggest that ozone changes resulting from climate change only are negative in a large fraction of the troposphere because of enhanced photochemical destruction by water vapor. In the Tropics, increased lightning activity should lead to larger ozone concentrations. The magnitude of the climate-induced ozone changes in the troposphere remains smaller than the changes produced by enhanced anthropogenic emissions when the Special Report on Emission Scenarios (SRES) A2P is adopted to describe the future evolution of these emissions. Predictions depend strongly on future trends in atmospheric methane levels, which are not well established. Changes in the emissions of NOx by bacteria in soils and of nonmethane hydrocarbons by vegetation associated with climate change could have a significant impact on future ozone levels.
    Print ISSN: 0894-8755
    Electronic ISSN: 1520-0442
    Topics: Geography , Geosciences , Physics
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  • 2
    Publication Date: 2019-07-18
    Description: The approach to create a comprehensive emission inventory for the time period 1980 to 2000 is described in this paper. We have recently compiled an emission database, which we will use for a 21 year simulation of tropospheric aerosols with the GOCART model. Particular attention was paid to the time-dependent SO2, black carbon and organic carbon aerosol emissions. For the emission of SO2 from sporadically erupting volcanoes, we assembled emission data from the Global Volcanism Program of the Smithsonian Institution, using the VEI to derive the volcanic cloud height and the SO2 amount, and amended this dataset by the SO2 emission data from the TOMS instrument when available. 3-dimensional aircraft emission data was obtained for a number of years from the AEAP project, converted from burned fuel to SO2 and interpolated to each year, taking the sparsity of the flight patterns into account. Other anthropogenic SO2 emissions are based on gridded emissions from the EDGAR 2000 database (excluding sources from aircraft, biomass burning and international ship traffic), which were scaled to individual years with country/regional based emission inventories. Gridded SO2 emissions from international ship traffic for 2000 and the scaling factors for other years are from [Eyring et al., 2005]. We used gridded anthropogenic black and organic carbon emissions for 1996 [Bond et al., 2005], again excluding aircraft, biomass burning and ship sources. These emissions were scaled with regional based emission inventories from 1980 to 2000 to derive gridded emissions for each year. The biomass burning emissions are based on a climatology, which is scaled with regional scaling factors derived from the TOMS aerosol index and the AVHRR/ASTR fire counts to each year [Duncan et al., 2003]. Details on the integration of the information from the various sources will be provided and the distribution patterns and total emissions in the final product will be discussed.
    Keywords: Meteorology and Climatology
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  • 3
    Publication Date: 2019-07-19
    Description: Western Africa is one of the most important aerosol source regions in the world. Major aerosol sources include dust from the world's largest desert Sahara, biomass burning from the Sahel, pollution aerosols from local sources and long-range transport from Europe, and biogenic sources from vegetation. Because these sources have large seasonal variations, the aerosol composition over the western Africa changes significantly with time. These aerosols exert large influences on local air quality and regional climate. In this study, we use the Goddard Chemistry Aerosol Radiation and Transport (GOCART) model to analyze satellite lidar data from the GLAS instrument on the ICESat and the sunphotometer data from the ground-based network AERONET taken in both the wet (September - October 2003) and dry (February - March 2004) seasons over western Africa. We will quantify the seasonal variations of aerosol sources and compositions and aerosol spatial (horizontal and vertical) distributions over western Africa. We will also assess the climate impact of western African aerosols. Such studies will be applied to support the international project, Africa Monsoon Multidisciplinary Analysis (AMMA) and to analyze the AMMA data.
    Keywords: Meteorology and Climatology
    Type: Joint CACGP/IGAC/WMO Symposium: Atmospheric Chemistry at the Interfaces 2006; Sep 09, 2006 - Sep 24, 2006; Cape Town; South Africa
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  • 4
    Publication Date: 2019-07-19
    Description: Dust originating from Asian deserts and desertification areas can be transported regionally and globally to affect surface air quality, visibility, and radiation budget not only at immediate downwind locations (e.g., eastern Asia) but also regions far away from the sources (e.g., North America). Deposition of Asian dust to the North Pacific Ocean basin influences the ocean productivity. In this study, we will use the Goddard Chemistry Aerosol Radiation and Transport (GOCART) model, remote sensing data form satellite and from the ground-based network, and in-situ data from aircraft and surface observations to address the following questions: - What are the effects of Asian dust on the surface air quality and visibility over Asia and North America? - What are the seasonal and spatial variations of dust deposition to the North Pacific Ocean? How does the Asian dust affect surface radiation budget?
    Keywords: Earth Resources and Remote Sensing
    Type: Western Pacific Geophysics Meeting; Jul 22, 2006 - Jul 28, 2006; Beijing; China
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  • 5
    Publication Date: 2019-07-19
    Description: Aerosol particles, also known as PM2.5 (particle diameter less than 2.5 microns) and PM10 (particle diameter less than 10 microns), is one of the key atmospheric components that determine ambient air quality. Current US air quality standards for PM10 (particles with diameter 〈 10 microns) and PM2.5 (particles with diameter 2.5 microns) are 50 pg/cu m and 15 pg/cu m, respectively. While local and regional emission sources are the main cause of air pollution problems, aerosols can be transported on a hemispheric or global scale. In this study, we use the Goddard Chemistry Aerosol Radiation and Transport (GOCART) model to quantify contributions of long-range transport vs. local/regional pollution sources and from natural vs. anthropogenic sources to PM concentrations different regions. In particular, we estimate the hemispheric impact of anthropogenic sulfate aerosols and dust from major source areas on other regions in the world. The GOCART model results are compared with satellite remote sensing and ground-based network measurements of aerosol optical depth and concentrations.
    Keywords: Meteorology and Climatology
    Type: Joint CACGP/IGAC/WMO Symposium: Atmospheric Chemistry at the Interfaces 2006; Sep 09, 2006 - Sep 24, 2006; Cape Town; South Africa
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