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  • Articles  (2)
  • Atmospheric Chemistry and Physics. 2018; 18(3): 2307-2328. Published 2018 Feb 15. doi: 10.5194/acp-18-2307-2018.  (1)
  • Atmospheric Chemistry and Physics. 2019; 19(15): 10379-10390. Published 2019 Aug 15. doi: 10.5194/acp-19-10379-2019.  (1)
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  • Articles  (2)
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  • 1
    Publication Date: 2018-02-15
    Description: The eruption of Mt. Tambora in 1815 was the largest volcanic eruption of the past 500 years. The eruption had significant climatic impacts, leading to the 1816 year without a summer, and remains a valuable event from which to understand the climatic effects of large stratospheric volcanic sulfur dioxide injections. The eruption also resulted in one of the strongest and most easily identifiable volcanic sulfate signals in polar ice cores, which are widely used to reconstruct the timing and atmospheric sulfate loading of past eruptions. As part of the Model Intercomparison Project on the climatic response to Volcanic forcing (VolMIP), five state-of-the-art global aerosol models simulated this eruption. We analyse both simulated background (no Tambora) and volcanic (with Tambora) sulfate deposition to polar regions and compare to ice core records. The models simulate overall similar patterns of background sulfate deposition, although there are differences in regional details and magnitude. However, the volcanic sulfate deposition varies considerably between the models with differences in timing, spatial pattern and magnitude. Mean simulated deposited sulfate on Antarctica ranges from 19 to 264 kg km−2 and on Greenland from 31 to 194 kg km−2, as compared to the mean ice-core-derived estimates of roughly 50 kg km−2 for both Greenland and Antarctica. The ratio of the hemispheric atmospheric sulfate aerosol burden after the eruption to the average ice sheet deposited sulfate varies between models by up to a factor of 15. Sources of this inter-model variability include differences in both the formation and the transport of sulfate aerosol. Our results suggest that deriving relationships between sulfate deposited on ice sheets and atmospheric sulfate burdens from model simulations may be associated with greater uncertainties than previously thought.
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 2
    Publication Date: 2019-08-15
    Description: In 1963 a series of eruptions of Mt. Agung, Indonesia, resulted in the third largest eruption of the 20th century and claimed about 1900 lives. Two eruptions of this series injected SO2 into the stratosphere, which can create a long-lasting stratospheric sulfate layer. The estimated mass flux of the first eruption was about twice as large as the mass flux of the second eruption. We followed the estimated emission profiles and assumed for the first eruption on 17 March an injection rate of 4.7 Tg SO2 and 2.3 Tg SO2 for the second eruption on 16 May. The injected sulfur forms a sulfate layer in the stratosphere. The evolution of sulfur is nonlinear and depends on the injection rate and aerosol background conditions. We performed ensembles of two model experiments, one with a single eruption and a second one with two eruptions. The two smaller eruptions result in a lower sulfur burden, smaller aerosol particles, and 0.1 to 0.3 Wm−2 (10 %–20 %) lower radiative forcing in monthly mean global average compared to the individual eruption experiment. The differences are the consequence of slightly stronger meridional transport due to different seasons of the eruptions, lower injection height of the second eruption, and the resulting different aerosol evolution. Overall, the evolution of the volcanic clouds is different in case of two eruptions than with a single eruption only. The differences between the two experiments are significant. We conclude that there is no justification to use one eruption only and both climatic eruptions should be taken into account in future emission datasets.
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
    Location Call Number Expected Availability
    BibTip Others were also interested in ...
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