ALBERT

Description: Aerosol particles are essential constituents of the Earth's atmosphere, impacting the earth radiation balance directly by scattering and absorbing solar radiation, and indirectly by acting as cloud condensation nuclei. In contrast to most greenhouse gases, aerosol particles have short atmospheric residence times, resulting in a highly heterogeneous distribution in space and time. There is a clear need to document this variability at regional scale through observations involving, in particular, the in situ near-surface segment of the atmospheric observation system. This paper will provide the widest effort so far to document variability of climate-relevant in situ aerosol properties (namely wavelength dependent particle light scattering and absorption coefficients, particle number concentration and particle number size distribution) from all sites connected to the Global Atmosphere Watch network. High-quality data from almost 90 stations worldwide have been collected and controlled for quality and are reported for a reference year in 2017, providing a very extended and robust view of the variability of these variables worldwide. The range of variability observed worldwide for light scattering and absorption coefficients, single-scattering albedo, and particle number concentration are presented together with preliminary information on their long-term trends and comparison with model simulation for the different stations. The scope of the present paper is also to provide the necessary suite of information, including data provision procedures, quality control and analysis, data policy, and usage of the ground-based aerosol measurement network. It delivers to users of the World Data Centre on Aerosol, the required confidence in data products in the form of a fully characterized value chain, including uncertainty estimation and requirements for contributing to the global climate monitoring system.

Description: This work presents a new bias-correction method for precipitation over complex terrain that explicitly considers orographic characteristics. This consideration offers a good alternative to the standard empirical quantile mapping (EQM) method during colder climate states in which the orography strongly deviates from the present-day state, e.g. during glacial conditions such as the Last Glacial Maximum (LGM). Such a method is needed in the event that absolute precipitation fields are used, e.g. as input for glacier modelling or to assess potential human occupation and according migration routes in past climate states. The new bias correction and its performance are presented for Switzerland using regional climate model simulations at 2 km resolution driven by global climate model outputs obtained under perpetual 1990 and LGM conditions. Comparing the present-day regional climate model simulation with observations, we find a strong seasonality and, especially during colder months, a height dependence of the bias in precipitation. Thus, we suggest a three-step correction method consisting of (i) a separation into different orographic characteristics, (ii) correction of very low intensity precipitation, and (iii) the application of an EQM, which is applied to each month separately. We find that separating the orography into 400 m height intervals provides the overall most reasonable correction of the biases in precipitation. The new method is able to fully correct the seasonal precipitation bias induced by the global climate model. At the same time, some regional biases remain, in particular positive biases over high elevated areas in winter and negative biases in deep valleys and Ticino in winter and summer. A rigorous temporal and spatial cross-validation with independent data exhibits robust results. The new bias-correction method certainly leaves some drawbacks under present-day conditions. However, the application to the LGM demonstrates that it is a more appropriate correction compared to the standard EQM under highly different climate conditions as the latter imprints present-day orographic features into the LGM climate.

Description: High altitude stations are often emphasized as free tropospheric measuring sites but they remain influenced by atmospheric boundary layer (ABL) air masses due to convective transport processes. The local and meso-scale topographical features around the station are involved in the convective boundary layer development and in the formation of thermally induced winds leading to ABL air lifting. The station altitude alone is not a sufficient parameter to characterize the ABL influence. In this study, a topography analysis is performed allowing calculation of a newly defined index called ABL-TopoIndex. The ABL-TopoIndex is constructed in order to correlate with the ABL influence at the high altitude stations and long-term aerosol time series are used to assess its validity. Topography data from the global digital elevation model GTopo30 were used to calculate five parameters for 43 high and 3 middle altitude stations situated on five continents. The geometric mean of these five parameters determines a topography based index called ABL-TopoIndex, which can be used to rank the high altitude stations as a function of the ABL influence. To construct the ABL-TopoIndex, we rely on the criteria that the ABL influence will be low if the station is one of the highest points in the mountainous massif, if there is a large altitude difference between the station and the valleys or high plains, if the slopes around the station are steep, and finally if the inverse drainage basin potentially reflecting the source area for thermally lifted pollutants to reach the site is small. All stations on volcanic islands exhibit a low ABL-TopoIndex, whereas stations in the Himalayas and the Tibetan Plateau have high ABL-TopoIndex values. Spearman's rank correlation between aerosol optical properties and number concentration from 28 stations and the ABL-TopoIndex, the altitude and the latitude are used to validate this topographical approach. Statistically significant (SS) correlations are found between the 5th and 50th percentiles of all aerosol parameters and the ABL-TopoIndex, whereas no SS correlation is found with the station altitude. The diurnal cycles of aerosol parameters seem to be best explained by the station latitude although a SS correlation is found between the amplitude of the diurnal cycles of the absorption coefficient and the ABL-TopoIndex.

Description: High altitude stations are often emphasized as free tropospheric measuring sites but they remain influenced by atmospheric boundary layer (ABL) air masses due to convective transport processes. The local and meso-scale topographical features around the station are involved in the convective boundary layer development and in the formation of thermally induced winds leading to ABL air lifting. The station altitude is not a sufficient parameter to characterize the ABL influence. Topography data from the global digital elevation model GTopo30 were used to calculate 5 parameters for 46 high altitude stations situated in five continents. The geometric mean of these 5 parameters determines a topography based index called ABL-TopoIndex which can be used to rank the high altitude stations as a function of the ABL influence. To construct the ABL-TopoIndex, we rely on the criteria that the ABL influence will be low if the station is one of the highest points in the mountainous massif, if there is a large altitude difference between the station and the valleys or plateaus, if the slopes around the station are steep, and finally if the drainage basin for air convection is small. All stations on volcanic islands exhibit a low ABL-TopoIndex whereas stations in the Himalaya and the Tibetan Plateau have high ABL-TopoIndex values. Spearman's rank correlation between aerosol optical properties and number concentration from 28 stations and the ABL-TopoIndex, the altitude and the latitude are used to validate this topographical approach. Statistically significant (s.s.) correlations are found between the 5 and 50 percentiles of all aerosol parameters and the ABL-TopoIndex whereas no s.s. correlation is found with the station altitude. The diurnal cycles of aerosol parameters seem to be best explained by the station latitude although a s.s. correlation is found between the amplitude of the diurnal cycles of the absorption coefficient and the ABL-TopoIndex. Finally, the main flow paths for air convection were calculated for various ABL heights.

Description: This work presents a new bias-correction method for precipitation that considers orographic characteristics, which makes it flexible to be used under highly different climate conditions, e.g., glacial conditions. The new bias-correction and its performance are presented for Switzerland using a regional climate simulation under perpetual 1990 conditions at 2-km resolution driven by a simulation performed with a global climate model. Comparing the regional simulations with observations, we find a strong seasonal and height dependence of the bias in precipitation commonly observed in regional climate modelling over complex terrain. Thus, we suggest a 3-step correction method consisting of (i) a separation into different orographic characteristics, (ii) correction of low intensity precipitation, and finally (iii) the application of empirical quantile mapping, which is applied to each month separately. Testing different orographic characteristics shows that separating in 400-m height-intervals provides the overall most reasonable correction of the biases in precipitation and additionally at the lowest computational costs. The seasonal precipitation bias induced by the global climate model is fully corrected, whereas some regional biases remain, in particular positive biases in winter over mountains and negative biases in winter and summer in deep valleys and Ticino. The biases over mountains are difficult to judge, as observations over complex terrain are afflicted with uncertainties, which may be more than 30 % above 1500 m a.s.l. A rigorous cross validation, which trains the correction method with independent observations from Germany, Austria and France, exhibits a similar performance compared to just using Switzerland as training and verification region. This illustrates the robustness of the new method. Thus, the new bias-correction provides a flexible tool which is suitable in studies where orography strongly changes, e.g., during glacial times.

Description: Ozone (O3) soundings have been performed on Easter Island or Rapa Nui (27 8S, 109 8W, 51 m a.s.l.) since 1994 as part of the Global Atmospheric Watch Programme of the World Meteorological Organization. In this work, we analyze 260 soundings compiled over the period 19942014, and make the data available for the international community. We characterize O3 profiles over this remote area of the Pacific by means of statistical analyses that consider, on the one hand, a traditional climatology that describes the data in terms of seasonal cycles based on monthly averages and, on the other hand, a process-oriented analysis based on self-organizing maps. Our analyses show the influence of both tropical and subtropical/mid-latitude air masses at Rapa Nui. The former occurs in summer and fall when convective conditions prevail, and the latter in late winter and spring when subsiding conditions are recurrent. The occurrence of stratospheric intrusions in late winter and spring in connection with deep troughs and the presence of the subtropical jet stream is also apparent in the data set. The tropospheric ozone column is in good agreement with the corresponding data derived from satellites but with a systematic overestimate of summer and fall values. There is evidence of an upward trend in ozone near the surface, which suggests the impact of local pollution. We look forward to an enhancement of the Rapa Nui observing site, given its location that offers a privileged position to observe climate change over the sparsely sampled and vast South Pacific Ocean.

Description: 〈jats:p〉Abstract. Aerosol particles are essential constituents of the Earth's atmosphere, impacting the earth radiation balance directly by scattering and absorbing solar radiation, and indirectly by acting as cloud condensation nuclei. In contrast to most greenhouse gases, aerosol particles have short atmospheric residence times, resulting in a highly heterogeneous distribution in space and time. There is a clear need to document this variability at regional scale through observations involving, in particular, the in situ near-surface segment of the atmospheric observation system. This paper will provide the widest effort so far to document variability of climate-relevant in situ aerosol properties (namely wavelength dependent particle light scattering and absorption coefficients, particle number concentration and particle number size distribution) from all sites connected to the Global Atmosphere Watch network. High-quality data from almost 90 stations worldwide have been collected and controlled for quality and are reported for a reference year in 2017, providing a very extended and robust view of the variability of these variables worldwide. The range of variability observed worldwide for light scattering and absorption coefficients, single-scattering albedo, and particle number concentration are presented together with preliminary information on their long-term trends and comparison with model simulation for the different stations. The scope of the present paper is also to provide the necessary suite of information, including data provision procedures, quality control and analysis, data policy, and usage of the ground-based aerosol measurement network. It delivers to users of the World Data Centre on Aerosol, the required confidence in data products in the form of a fully characterized value chain, including uncertainty estimation and requirements for contributing to the global climate monitoring system. 〈/jats:p〉