ALBERT

Description: Simulations of total and polarized cloud reflectance angular signatures such as the ones measured by the multi-angular and polarized radiometer POLDER3/PARASOL are used to evaluate cloud heterogeneity effects on cloud parameter retrievals. Effects on optical thickness, albedo, effective radius and variance of the cloud droplet size distribution and aerosol parameters above cloud are analyzed. Three different clouds that have the same mean optical thicknesses were generated: the first with a flat top, the second with a bumpy top and the last with a fractional cloud cover. At small scale (50 m), for oblique solar incidence, the illumination effects lead to higher total but also polarized reflectances. The polarized reflectances even reach values that cannot be predicted by the 1-D homogeneous cloud assumption. At the POLDER scale (7 km × 7 km), the angular signature is modified by a combination of the plane–parallel bias and the shadowing and illumination effects. In order to quantify effects of cloud heterogeneity on operational products, we ran the POLDER operational algorithms on the simulated reflectances to retrieve the cloud optical thickness and albedo. Results show that the cloud optical thickness is greatly affected: biases can reach up to −70, −50 or +40 % for backward, nadir and forward viewing directions, respectively. Concerning the albedo of the cloudy scenes, the errors are smaller, between −4.7 % for solar incidence angle of 20∘ and up to about +8 % for solar incidence angle of 60∘. We also tested the heterogeneity effects on new algorithms that allow retrieving cloud droplet size distribution and cloud top pressures and also aerosol above clouds. Contrary to the bi-spectral method, the retrieved cloud droplet size parameters are not significantly affected by the cloud heterogeneity, which proves to be a great advantage of using polarized measurements. However, the cloud top pressure obtained from molecular scattering in the forward direction can be biased up to about 60 hPa (around 550 m). Concerning the aerosol optical thickness (AOT) above cloud, the results are different depending on the available angular information. Above the fractional cloud, when only side scattering angles between 100 and 130∘ are available, the AOT is underestimated because of the plane–parallel bias. However, for solar zenith angle of 60∘ it is overestimated because the polarized reflectances are increased in forward directions.

Description: This study presents a comparison between the retrieval of optical properties of aerosol above clouds (AAC) from different techniques developed for the A-Train sensors CALIOP/CALIPSO and POLDER/PARASOL. The main objective is to analyse the consistency between the results derived from the active and the passive measurements. We compare the aerosol optical thickness (AOT) above optically thick clouds (cloud optical thickness (COT) larger than 3) and their Ångström exponent (AE). These parameters are retrieved with the CALIOP operational method, the POLDER operational polarization method and the CALIOP-based depolarization ratio method (DRM) – for which we also propose a calibrated version (denominated DRMSODA, where SODA is the Synergized Optical Depth of Aerosols). We analyse 6 months of data over three distinctive regions characterized by different types of aerosols and clouds. Additionally, for these regions, we select three case studies: a biomass-burning event over the South Atlantic Ocean, a Saharan dust case over the North Atlantic Ocean and a Siberian biomass-burning event over the North Pacific Ocean. Four and a half years of data are studied over the entire globe for distinct situations where aerosol and cloud layers are in contact or vertically separated. Overall, the regional analysis shows a good correlation between the POLDER and the DRMSODA AOTs when the microphysics of aerosols is dominated by fine-mode particles of biomass-burning aerosols from southern Africa (correlation coefficient (R2) of 0.83) or coarse-mode aerosols of Saharan dust (R2 of 0.82). A good correlation between these methods (R2 of 0.68) is also observed in the global treatment, when the aerosol and cloud layers are separated well. The analysis of detached layers also shows a mean difference in AOT of 0.07 at 532 nm between POLDER and DRMSODA at a global scale. The correlation between the retrievals decreases when a complex mixture of aerosols is expected (R2 of 0.37) – as in the East Asia region – and when the aerosol–cloud layers are in contact (R2 of 0.36). The correlation coefficient between the CALIOP operational method and POLDER is found to be low, as the CALIOP method largely underestimates the aerosol loading above clouds by a factor that ranges from 2 to 4. Potential biases on the retrieved AOT as a function of cloud properties are also investigated. For different types of scenes, the retrieval of above-cloud AOT from POLDER and from DRM are compared for different underlying cloud properties (droplet effective radius (reff) and COT retrieved with MODIS). The results reveal that DRM AOT vary with reff. When accounting for reff in the DRM algorithm, the consistency between the methods increases. The sensitivity study shows that an additional polarized signal coming from aerosols located within the cloud could affect the polarization method, which leads to an overestimation of the AOT retrieved with POLDER algorithm. In addition, the aerosols attached to or within the cloud can potentially impact the DRM retrievals through the modification of the cloud droplet chemical composition and its ability to backscatter light. The next step of this work is to combine POLDER and CALIOP to investigate the impacts of aerosols on clouds and climate when these particles are transported above or within clouds.

Description: The Polarization and Anisotropy of Reflectances for Atmospheric Sciences Coupled with Observations from a Lidar (PARASOL) and Aqua are two satellites on sun-synchronous orbits in the A-Train constellation. Aboard these two platforms, the Polarization and Directionality of Earth Reflectances (POLDER) and Moderate Resolution Imaging Spectroradiometer (MODIS) provide quasi simultaneous and coincident observations of cloud properties. The similar orbits but different detecting characteristics of these two sensors call for a comparison between the derived datasets to identify and quantify potential uncertainties in retrieved cloud properties. To focus on the differences due to different sensor spatial resolution and coverage, while minimizing sampling and weighting issues, the authors have recomputed monthly statistics directly from the respective official level-2 products. The authors have developed a joint dataset that contains both POLDER and MODIS level-2 cloud products collocated on a common sinusoidal grid. The authors have then computed and analyzed monthly statistics of cloud fractions corresponding either to the total cloud cover or to the “retrieved” cloud fraction for which cloud optical properties are derived. These simple yet crucial cloud statistics need to be clearly understood to allow further comparison work of the other cloud parameters. From this study, it is demonstrated that on average POLDER and MODIS datasets capture correctly the main characteristics of global cloud cover and provide similar spatial distributions and temporal variations. However, each sensor has its own advantages and weaknesses in discriminating between clear and cloudy skies in particular situations. Also it is shown that significant differences exist between the MODIS total cloud fraction (day mean) and the “retrieved” cloud fraction (combined mean). This study found a global negative difference of about 10% between POLDER and MODIS day-mean cloud fraction. On the contrary, a global positive difference of about 10% exists between POLDER and MODIS combined-mean cloud fraction. These statistical biases show both global and regional distributions that can be driven by sensors characteristics, environmental factors, and also carry potential information on cloud cover structure. These results provide information on the quality of cloud cover derived from POLDER and MODIS and should be taken into account for the use of other cloud products.

Description: Insufficient knowledge of the habit distribution and the degree of surface roughness of ice crystals within ice clouds is a source of uncertainty in the forward light scattering and radiative transfer simulations of ice clouds used in downstream applications. The Moderate Resolution Imaging Spectroradiometer (MODIS) collection-5 ice microphysical model presumes a mixture of various ice crystal shapes with smooth facets, except for the compact aggregate of columns for which a severely rough condition is assumed. When compared with Polarization and Anisotropy of Reflectances for Atmospheric Sciences coupled with Observations from a Lidar (PARASOL) polarized reflection data, simulations of polarized reflectance using smooth particles show a poor fit to the measurements, whereas very rough-faceted particles provide an improved fit to the polarized reflectance. In this study a new microphysical model based on a mixture of nine different ice crystal habits with severely roughened facets is developed. Simulated polarized reflectance using the new ice habit distribution is calculated using a vector adding–doubling radiative transfer model, and the simulations closely agree with the polarized reflectance observed by PARASOL. The new general habit mixture is also tested using a spherical albedo differences analysis, and surface roughening is found to improve the consistency of multiangular observations. These results are consistent with previous studies that have used polarized reflection data. It is suggested that an ice model incorporating an ensemble of different habits with severely roughened surfaces would potentially be an adequate choice for global ice cloud retrievals.

Description: New evidence from collocated measurements, with support from theory and numerical simulations, that multidirectional measurements in the oxygen A band from the third Polarization and Directionality of the Earth’s Reflectances (POLDER-3) instrument on the Polarization and Anisotropy of Reflectances for Atmospheric Sciences coupled with Observations from a Lidar (PARASOL) satellite platform within the “A-Train” can help to characterize the vertical structure of clouds is presented. In the case of monolayered clouds, the standard POLDER cloud oxygen pressure product PO2 is shown to be sensitive to the cloud geometrical thickness H in two complementary ways: 1) PO2 is, on average, close to the pressure at the geometrical middle of the cloud layer (MCP) and methods are proposed for reducing the pressure difference PO2 − MCP and 2) the angular standard deviation of PO2 and the cloud geometrical thickness H are tightly correlated for liquid clouds. Accounting for cloud phase, there is thus the potential to obtain a statistically reasonable estimate of H. Such derivation from passive measurements, as compared with or supplementing other observations, is expected to be of interest in a broad range of applications for which it is important to define better the macrophysical cloud parameters in a practical way.

Description: Aerosols have a direct effect on the Earth's radiative budget and can also affect cloud development and lifetime, and the aerosols above clouds (AAC) are particularly associated with high uncertainties in global climate models. Therefore, it is a prerequisite to improve the description and understanding of these situations. During the austral winter, large loadings of biomass burning aerosols originating from fires in the southern African subcontinent are lifted and transported westwards, across the southeastern Atlantic Ocean. The negligible wet scavenging of these absorbing aerosols leads to a near-persistent smoke layer above one of the largest stratocumulus cloud decks on the planet. Therefore, the southeastern Atlantic region is a very important area for studying the impact of above-cloud absorbing aerosols, their radiative forcing and their possible effects on clouds. In this study we aim to analyse and quantify the effect of smoke loadings on cloud properties using a synergy of different remote sensing techniques from A-Train retrievals (methods based on the passive instruments POLDER and MODIS and the operational method of the spaceborne lidar CALIOP), collocated with ERA-Interim re-analysis meteorological profiles. To analyse the possible mechanisms of AAC effects on cloud properties, we developed a high and low aerosol loading approach, which consists in evaluating the change in radiative quantities (i.e. cloud-top cooling, heating rate vertical profiles) and cloud properties with the smoke loading. During this analysis, we account for the variation in the meteorological conditions over our sample area by selecting the months associated with one meteorological regime (June–August). The results show that the region we focus on is primarily under the energetic influence of absorbing aerosols, leading to a significant positive shortwave direct effect at the top of the atmosphere. For larger loads of AACs, clouds are optically thicker, with an increase in liquid water path of 20 g m−2 and lower cloud-top altitudes by 100 m. These results do not contradict the semi-direct effect of above-cloud aerosols, explored in previous studies. Furthermore, we observe a strong covariance between the aerosol and the water vapour loadings, which has to be accounted for. A detailed analysis of the heating rate profiles shows that within the smoke layer, the absorbing aerosols are 90 % responsible for warming the ambient air by approximately 5.7 K d−1. The accompanying water vapour, however, has a longwave effect at distance on the cloud top, reducing its cooling by approximately 4.7 K d−1 (equivalent to 7 %). We infer that this decreased cloud-top cooling in particular, in addition with the higher humidity above the clouds, might modify the cloud-top entrainment rate and its effect, leading to thicker clouds. Therefore, smoke (the combination of aerosol and water vapour) events would have the potential to modify and probably reinforce the underlaying cloud cover.

Description: The 2014–15 Holuhraun lava-flood eruption of Bárdarbunga volcano (Iceland) has emitted prodigious amounts of sulfur dioxide into the atmosphere. This eruption caused a large-scale episode of air pollution throughout Western Europe in September 2014, the first event of this magnitude recorded in the modern era. We gathered a wealth of complementary observations from satellite sensors (OMI, IASI), ground-based remote sensing (lidar, sunphotometry, differential optical absorption spectroscopy) and ground-level air quality monitoring networks to characterize both the spatial-temporal distributions of volcanic SO2 and sulfate aerosols as well as the dynamics of the planetary boundary layer. Time variations of dynamical and microphysical properties of sulfate aerosols in the aged low-tropospheric volcanic cloud, including loading, vertical distribution, size distribution and single scattering albedo, are provided. Retrospective chemistry-transport simulations capture the correct temporal dynamics of this far-range air pollution event but fail to reproduce the magnitude of SO2 concentration at ground-level. Improving forecasts of large-scale volcanogenic air pollution will require refined emission parameters and adapted model grid resolution to accurately describe both long-range transport and local boundary layer dynamics.

Description: Aerosols have a direct effect on the Earth's radiative budget and can also affect the cloud development and lifetime. The aerosols above clouds (AAC) are particularly associated with high uncertainties in global climate models. Therefore, it is prerequisite to improve the description and understanding of these situations. During the austral winter, large loadings of biomass burning aerosols originating from fires in the southern African subcontinent are lifted and transported long distances westwards, across the Southeast Atlantic Ocean. The negligible wet scavenging of these absorbing aerosols leads to a near-persistent smoke layer above one of the largest stratocumulus cloud deck on the planet. Therefore, the Southeast Atlantic region is a very important area for studying the impact of above cloud absorbing aerosols, their radiative forcing and their possible effects on clouds. In this study we aim to analyse and quantify the effect of smoke loadings on cloud properties using a synergy of different remote sensing technics from A-Train retrievals (methods based on the passive instruments POLDER and MODIS and the operational method of the spaceborne lidar CALIOP), collocated with ERA-Interim re-analysis meteorological profiles. To analyse the possible mechanisms of AACs effects on cloud properties, we developed a high and low aerosol loading approach, that consists in evaluating the change in radiative quantities (i.e. cloud top cooling, heating rate vertical profiles) and cloud properties with the smoke loading. During this analysis, we account for the variation in the meteorological conditions over our sample area. The results show that the region we focus on is primarily under the energetic influence of absorbing aerosols, leading to a significant positive shortwave direct effect at the top of the atmosphere. For larger loads of AACs, clouds are optically thicker, with an increase in liquid water path of 20 g m−2 and lower cloud top altitudes by 100 m. These results do not contradict the semi-direct effect of above cloud aerosols, explored in previous studies. Furthermore, we observe a strong correlation between the aerosol and the water vapor loadings, which has to be accounted for. A detailed analysis of the heating rates shows that the absorbing aerosols are 90 % responsible for warming the ambient air where they reside, with approximately + 5.7 K/day, while the accompanying water vapour above clouds has a longwave effect of + 4.7 K/day (equivalent to 7 % decrease) on the cloud top cooling. We infer that this decreased cloud top cooling in particular, in addition with the higher humidity above the clouds, might modify the cloud top entrainment rate and its effect, leading to thicker clouds. Therefore, smoke (the combination of aerosol and water vapor) events would have the potential to modify and probably reinforce the underlaying cloud cover.

Description: Simulations of total and polarized cloud reflectance angular signatures such as the ones measured by the multi-angular and polarized radiometer POLDER3/PARASOL are used to evaluate cloud heterogeneity effects on cloud parameter retrievals. Effects on optical thickness, cloud albedo, effective radius and variance of the cloud droplet size distribution and aerosol above cloud optical thickness are analyzed. Three different clouds having the same mean optical thicknesses were generated: the first one with a flat top, the second one with a bumpy top and the last one with a fractional cloud cover. At small scale (50 m), for oblique solar incidence, the illumination effects lead to higher total but also polarized reflectances. The polarized reflectances even reach values that cannot be predicted by the 1D homogeneous cloud assumption. At the POLDER scale (7 km × 7 km), the angular signature is modified by a combination of the plane-parallel bias and the shadowing and illumination effects. In order to quantify effects of cloud heterogeneity on operational products, we ran the POLDER operational algorithms on the simulated reflectances to retrieve the cloud optical thickness and albedo. Results show that the cloud optical thickness is greatly affected: biases can reach up to −70 %, −50 % or +40 % for backward, nadir and forward viewing directions respectively. Concerning the cloud albedo, the errors are smaller, between −4.7 % for solar incidence angle of 20° and up to about 8 % for solar incidence angle of 60°. We also tested the heterogeneity effects on new algorithms that allow retrieving cloud droplet size distribution and cloud top pressures and also aerosol above clouds. Contrarily to the bi-spectral method, the retrieved cloud droplet size parameters are not significantly affected by the cloud heterogeneity, which proves to be a great advantage of using polarized measurements. However the cloud top pressure obtained from molecular scattering in the forward direction can be biased up to 120 hPa (around 1 km). Concerning the aerosol optical thickness (AOT) above cloud, the results are different depending on the available angular information. Above the fractional cloud, when only side scattering angles are available, the AOT can be underestimated because of the plane-parallel bias. For solar zenith angle of 60°, on contrary, it is overestimated because the polarized reflectances are increased in forward directions.