ALBERT

Description: This study underlines the important role of the transported black carbon (BC) mass concentration in the West African monsoon (WAM) area. BC was measured with a micro-aethalometer integrated in the payload bay of the unmanned research aircraft ALADINA (Application of Light-weight Aircraft for Detecting IN situ Aerosol). As part of the DACCIWA (Dynamics–Aerosol–Chemistry–Cloud Interactions in West Africa) project, 53 measurement flights were carried out at Savè, Benin, on 2–16 July 2016. A high variability of BC (1.79 to 2.42±0.31 µg m−3) was calculated along 155 vertical profiles that were performed below cloud base in the atmospheric boundary layer (ABL). In contrast to initial expectations of primary emissions, the vertical distribution of BC was mainly influenced by the stratification of the ABL during the WAM season. The article focuses on an event (14 and 15 July 2016) which showed distinct layers of BC in the lowermost 900 m above ground level (a.g.l.). Low concentrations of NOx and CO were sampled at the Savè supersite near the aircraft measurements and suggested a marginal impact of local sources during the case study. The lack of primary BC emissions was verified by a comparison of the measured BC with the model COSMO-ART (Consortium for Small-scale Modelling–Aerosols and Reactive Trace gases) that was applied for the field campaign period. The modelled vertical profiles of BC led to the assumption that the measured BC was already altered, as the size was mainly dominated by the accumulation mode. Further, calculated vertical transects of wind speed and BC presume that the observed BC layer was transported from the south with maritime inflow but was mixed vertically after the onset of a nocturnal low-level jet at the measurement site. This report contributes to the scope of DACCIWA by linking airborne BC data with ground observations and a model, and it illustrates the importance of a more profound understanding of the interaction between BC and the ABL in the WAM region.

Description: The relative contribution of the synoptic-scale circulations to local and mesoscale processes was quantified in terms of the variability of midlatitude temperature anomalies from 2003 to 2013 using meteorological variables collected from three French observatories and reanalyses. Four weather regimes were defined from sea level pressure anomalies using National Centers for Environmental Prediction reanalyses with a K-means algorithm. No correlation was found between daily temperature anomalies and weather regimes, and the variability of temperature anomalies within each regime was large. It was therefore not possible to evaluate the effect of large scales on temperature anomalies by this method. An alternative approach was found with the use of the analogs method: the principle being that for each day of the considered time series, a set of days that had a similar large-scale 500-hPa geopotential height field within a fixed domain was considered. The observed temperature anomalies were then compared with those observed during the analog days: the closer the two types of series are to each other, the greater is the influence of the large scale. This method highlights a widely predominant influence of the large-scale atmospheric circulation on the temperature anomalies. It showed a potentially larger influence of the Mediterranean Sea and orographic flow on the two southern observatories. Low-level cloud radiative effects substantially modulated the variability of the daily temperature anomalies.

Description: Water in the atmosphere can exist in the solid, liquid or gas phase. At high humidities, if the aerosol population remains constant, more water vapour will condense onto the particles and cause them to swell, sometimes up to several times their original size. This significant change in size and chemical composition is termed hygroscopic growth and alters a particle's optical properties. Even in unsaturated conditions, this can change the aerosol direct effect, for example by increasing the extinction of incoming sunlight. This can have an impact on a region's energy balance and affect visibility. Here, aerosol and relative humidity measurements collected from aircraft and radiosondes during the Dynamics–Aerosol–Chemistry–Cloud Interactions in West Africa (DACCIWA) campaign were used to estimate the effect of highly humid layers of air on aerosol optical properties during the monsoon season in southern West Africa. The effects of hygroscopic growth in this region are of particular interest due to the regular occurrence of high humidity and the high levels of pollution in the region. The Zdanovskii, Stokes and Robinson (ZSR) mixing rule is used to estimate the hygroscopic growth of particles under different conditions based on chemical composition. These results are used to estimate the aerosol optical depth (AOD) at λ=525 nm for 63 relative humidity profiles. The median AOD in the region from these calculations was 0.36, the same as that measured by sun photometers at the ground site. The spread in the calculated AODs was less than the spread from the sun photometer measurements. In both cases, values above 0.5 were seen predominantly in the mornings and corresponded with high humidities. Observations of modest variations in aerosol load and composition are unable to explain the high and variable AODs observed using sun photometers, which can only be recreated by accounting for the very elevated and variable relative humidities (RHs) in the boundary layer. Most importantly, the highest AODs present in the mornings are not possible without the presence of high RH in excess of 95 %. Humid layers are found to have the most significant impact on AOD when they reach RH greater than 98 %, which can result in a wet AOD more than 1.8 times the dry AOD. Unsaturated humid layers were found to reach these high levels of RH in 37 % of observed cases. It can therefore be concluded that the high AODs present across the region are driven by the high humidities and are then moderated by changes in aerosol abundance. Aerosol concentrations in southern West Africa are projected to increase substantially in the coming years; results presented here show that the presence of highly humid layers in the region is likely to enhance the consequent effect on AOD significantly.

Description: A ground-based field campaign was conducted in southern West Africa from mid-June to the end of July 2016 within the framework of the Dynamics–Aerosol–Chemistry–Cloud Interactions in West Africa (DACCIWA) project. It aimed to provide a high-quality comprehensive data set for process studies, in particular of interactions between low-level clouds (LLCs) and boundary-layer conditions. In this region missing observations are still a major issue. During the campaign, extensive remote sensing and in situ measurements were conducted at three supersites: Kumasi (Ghana), Savè (Benin) and Ile-Ife (Nigeria). Daily radiosoundings were performed at 06:00 UTC, and 15 intensive observation periods (IOPs) were performed during which additional radiosondes were launched, and remotely piloted aerial systems were operated. Extended stratiform LLCs form frequently in southern West Africa during the nighttime and persist long into the following day. They affect the radiation budget and hence the evolution of the atmospheric boundary layer and regional climate. The relevant parameters and processes governing the formation and dissolution of the LLCs are still not fully understood. This paper gives an overview of the diurnal cycles of the energy-balance components, near-surface temperature, humidity, wind speed and direction as well as of the conditions (LLCs, low-level jet) in the boundary layer at the supersites and relates them to synoptic-scale conditions (monsoon layer, harmattan layer, African easterly jet, tropospheric stratification) in the DACCIWA operational area. The characteristics of LLCs vary considerably from day to day, including a few almost cloud-free nights. During cloudy nights we found large differences in the LLCs' formation and dissolution times as well as in the cloud-base height. The differences exist at individual sites and also between the sites. The synoptic conditions are characterized by a monsoon layer with south-westerly winds, on average about 1.9 km deep, and easterly winds above; the depth and strength of the monsoon flow show great day-to-day variability. Within the monsoon layer, a nocturnal low-level jet forms in approximately the same layer as the LLC. Its strength and duration is highly variable from night to night. This unique data set will allow us to test some new hypotheses about the processes involved in the development of LLCs and their interaction with the boundary layer and can also be used for model evaluation.

Description: This study presents the first detailed observational analysis of the complete diurnal cycle of stratiform low-level clouds (LLC) and involved atmospheric processes over southern West Africa (SWA). The data used here were collected during the comprehensive DACCIWA (Dynamics-Aerosol-Chemistry-Cloud-Interactions in West Africa) ground-based campaign, which aimed at monitoring LLC characteristics and capturing the wide range of atmospheric conditions related to the West African monsoon flow. In this study, in situ and remote sensing measurements from the supersite near Savè (Benin) collected during a typical day, which is characterized by the onset of a nocturnal low-level jet (NLLJ) and the formation of LLC, are analyzed. The associated dynamic and thermodynamic conditions allow the identification of five different phases related to the LLC diurnal cycle: the stable, jet, stratus I, stratus II, and convective phases. The analysis of relative humidity tendency shows that cooling is a dominant process for LLC formation, which leads to a continuous increase in relative humidity at a maximum rate of 6 % h−1, until finally saturation is reached and LLC form with a cloud-base height near the height of NLLJ maximum. Results of heat budget analysis illustrate that horizontal cold-air advection, related to the maritime inflow, which brings the cool maritime air mass and a prominent NLLJ wind profile, has the dominant role in the observed strong cooling of −1.2 K h−1 during the jet phase. The contribution from horizontal cold advection is quantified to be up to 68 %, while radiative cooling and sensible heat flux divergence both contribute 16 % to the observed heat budget below the NLLJ maximum. After the LLC form (stratus phases I and II), turbulent mixing is an important factor leading to the cooling below the cloud base, while strong radiative cooling at the cloud top helps to maintain thick stratus.

Description: During the West African summer monsoon season, extended nocturnal stratiform low-level clouds (LLCs) frequently form in the atmospheric boundary layer over southern West Africa and persist long into the following day affecting the regional climate. A unique data set was gathered within the framework of the Dynamics–Aerosol–Chemistry–Cloud Interactions in West Africa (DACCIWA) project, which allows, for the first time, for an observational analysis of the processes and parameters crucial for LLC formation. In this study, in situ and remote sensing measurements from radiosondes, ceilometer, cloud radar and energy balance stations from a measurement site near Savè in Benin are analyzed amongst others for 11 nights. The aim is to study LLC characteristics, the intranight variability of boundary layer conditions and physical processes relevant for LLC formation, as well as to assess the importance of these processes. Based on the dynamic and thermodynamic conditions in the atmospheric boundary layer we distinguish typical nocturnal phases and calculate mean profiles for the individual phases. A stable surface inversion, which forms after sunset, is eroded by differential horizontal cold air advection with the Gulf of Guinea maritime inflow, a cool air mass propagating northwards from the coast in the late afternoon and the evening, and shear-generated turbulence related to a nocturnal low-level jet. The analysis of the contributions to the relative humidity changes before the LLC formation reveals that cooling in the atmospheric boundary layer is crucial to reach saturation, while specific humidity changes play a minor role. We quantify the heat budget terms and find that about 50 % of the cooling prior to LLC formation is caused by horizontal cold air advection, roughly 20 % by radiative flux divergence and about 22 % by sensible heat flux divergence in the presence of a low-level jet. The outcomes of this study contribute to the development of a conceptual model on LLC formation, maintenance and dissolution over southern West Africa.

Description: Nocturnal low-level stratus clouds (LLCs) are frequently observed in the atmospheric boundary layer (ABL) over southern West Africa (SWA) during the summer monsoon season. Considering the effect these clouds have on the surface energy and radiation budgets as well as on the diurnal cycle of the ABL, they are undoubtedly important for the regional climate. However, an adequate representation of LLCs in the state-of-the-art weather and climate models is still a challenge, which is largely due to the lack of high-quality observations in this region and gaps in understanding of underlying processes. In several recent studies, a unique and comprehensive data set collected in summer 2016 during the DACCIWA (Dynamics-aerosol-chemistry-cloud interactions in West Africa) ground-based field campaign was used for the first observational analyses of the parameters and physical processes relevant for the LLC formation over SWA. However, occasionally stratus-free nights occur during the monsoon season as well. Using observations and ERA5 reanalysis, we investigate differences in the boundary-layer conditions during 6 stratus-free and 20 stratus nights observed during the DACCIWA campaign. Our results suggest that the interplay between three major mechanisms is crucial for the formation of LLCs during the monsoon season: (i) the onset time and strength of the nocturnal low-level jet (NLLJ), (ii) horizontal cold-air advection, and (iii) background moisture level. Namely, weaker or later onset of NLLJ leads to a reduced contribution from horizontal cold-air advection. This in turn results in weaker cooling, and thus saturation is not reached. Such deviation in the dynamics of the NLLJ is related to the arrival of a cold air mass propagating northwards from the coast, called Gulf of Guinea maritime inflow. Additionally, stratus-free nights occur when the intrusions of dry air masses, originating from, for example, central or south Africa, reduce the background moisture over large parts of SWA. Backward-trajectory analysis suggests that another possible reason for clear nights is descending air, which originated from drier levels above the marine boundary layer.

Description: This study presents the first detailed observational analysis of the complete diurnal cycle of stratiform low-level clouds (LLC) and involved atmospheric processes over southern West Africa. The data used here were collected during the comprehensive DACCIWA (Dynamics-Aerosol-Chemistry-Cloud-Interactions in West Africa) ground-based campaign, which aimed at monitoring LLC characteristics and capturing the wide range of atmospheric conditions related to the West African monsoon flow. In this study, in-situ and remote sensing measurements from the supersite near Savè (Benin) collected during a typical day, which is characterized by the onset of a nocturnal low-level jet (NLLJ) and the formation of LLC, are analyzed. The associated dynamic and thermodynamic conditions allow the identification of five different phases of the LLC diurnal cycle: the Stable, Jet, Stratus I, Stratus II and Convective phase. The analysis of relative humidity tendency shows that cooling is a dominant process for LLC formation, which leads to a continuous increase of relative humidity at a maximum rate of 6% per hour, until finally saturation is reached and LLC form with a cloud-base height near the height of NLLJ maximum. Results of heat budget analysis illustrate that horizontal cold air advection, related to the maritime inflow, which brings the cool maritime air mass and a prominent NLLJ wind profile, has the dominant role on the observed strong cooling of −1.2K per hour during the Jet phase. The contribution from horizontal cold advection is quantified to be up to 72%, while radiative cooling and sensible heat flux divergence contribute with 16 and 12%, respectively, to the observed heat budget below the NLLJ maximum. After the LLC form (Stratus phase I and II), turbulent mixing is an important factor leading to the cooling below the cloud base, while strong radiative cooling at the cloud top helps to maintain thick stratus.

Description: The misrepresentation of the diurnal cycle of boundary-layer clouds by large scale models strongly impacts the modeled regional energy balance in southern West Africa. In particular, recognizing the processes involved in the maintenance and transition of the nighttime stratocumulus to diurnal shallow cumulus over land remains a challenge. This is due to the fact that over vegetation, surface fluxes exhibit a much larger magnitude and variability than on the more researched marine stratocumulus transitions. An improved understanding of the interactions between surface and atmosphere is thus necessary to improve its representation. To this end, the DACCIWA measurement campaign gathered a unique dataset of observations of the frequent stratocumulus to cumulus transition in southern West Africa. Inspired and constrained by these observations, we perform a series of numerical experiments using Large Eddy Simulation. The experiments include interactive radiation and surface schemes where we explicitly resolve, quantify and describe the physical processes driving such transition. Focusing on the local processes, we quantify the transition in terms of dynamics, radiation, cloud properties, surface processes and the evolution of dynamically relevant layers such as subcloud layer, cloud layer and inversion layer. We further quantify the processes driving the stratocumulus thinning and the subsequent transition initiation by using a liquid water path budget. Finally, we study the impact of mean wind and wind shear at cloud top through two additional numerical experiments. We find that the sequence starts with a nighttime well-mixed layer from surface to cloud top, in terms of temperature and humidity, and transitions to a prototypical convective boundary layer by the afternoon. We identify radiative cooling as the largest factor for the maintenance leading to a net thickening of the cloud layer of about 18 g m−2 h−1 before sunrise. Four hours after sunrise, the cloud layer decouples from the surface through a growing negative buoyancy flux at cloud base. After sunrise, the increasing impact of entrainment leads to a progressive thinning of the cloud layer. While the effect of wind on the stratocumulus layer during nighttime is limited, after sunrise we find shear at cloud top to have the largest impact: the local turbulence generated by shear enhances the boundary layer growth and entrainment aided by the increased surface fluxes. As a consequence wind shear at cloud top accelerates the breakup and transition by about 2 hours. The quantification of the transition and its driving factors presented here sets the path for an improved representation by larger scale models.

Description: The vertical variability of the black carbon (BC) mass concentration in the atmospheric boundary layer (ABL) is analysed during the West-African Monsoon (WAM) season. BC was measured with a micro aethalometer (model AE51, AethLabs) integrated in the payload bay of the unmanned research aircraft ALADINA (Application of Light-weight Aircraft for Detecting IN situ Aerosol) as part of the field experiment of the DACCIWA (Dynamics-Aerosol-Chemistry-Cloud Interactions in West Africa) project. In total, 53 measurement flights were performed at the local airfield of Save, Benin, in the period of 2–16 July 2016. The mean results show a high variability of BC (1.79 to 2.42 ± 0.31 μg/m3) influenced by the stratification of the ABL during the WAM. The model COSMO-ART (Consortium for Small-scale Modelling–Aerosols and Reactive Trace gases) was applied for the field campaign period and used in order to investigate possible sources of the measured BC. The model output was compared with the BC data on two selected measurement days (14 and 15 July 2016). The modeled vertical profiles of BC show that the observed BC was already altered, as the size was mainly dominated by the accumulation mode. Further, the calculated vertical transects of wind speed and BC showed that the measured BC layer was transported from the south with maritime inflow, but was mixed vertically after to the onset of the nocturnal low-level jet (NLLJ) at the measurement site. The validations and the ground observations of gas concentrations NOx and CO confirm that primary emission could be excluded during the case study, in contrast to initially expected. The case underlines the important role of BC transport processes in the WAM area.