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  • 1
    Publication Date: 2012-10-03
    Description: Author(s): J. Shan, W. Shi, L. Y. Liu, Y. R. Shen, and L. Xu Gold nanoparticles deposited on the windows of a liquid crystal (LC) cell were found to be able to reduce the surface anchoring energy of the LC, and hence the threshold for its reorientation phase transition, by 1 to 2 orders of magnitude when a cw pump light was used to excite the local plasmon re... [Phys. Rev. Lett. 109, 147801] Published Tue Oct 02, 2012
    Keywords: Soft Matter, Biological, and Interdisciplinary Physics
    Print ISSN: 0031-9007
    Electronic ISSN: 1079-7114
    Topics: Physics
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  • 2
    Publication Date: 2009-06-12
    Description: The electronic bandgap is an intrinsic property of semiconductors and insulators that largely determines their transport and optical properties. As such, it has a central role in modern device physics and technology and governs the operation of semiconductor devices such as p-n junctions, transistors, photodiodes and lasers. A tunable bandgap would be highly desirable because it would allow great flexibility in design and optimization of such devices, in particular if it could be tuned by applying a variable external electric field. However, in conventional materials, the bandgap is fixed by their crystalline structure, preventing such bandgap control. Here we demonstrate the realization of a widely tunable electronic bandgap in electrically gated bilayer graphene. Using a dual-gate bilayer graphene field-effect transistor (FET) and infrared microspectroscopy, we demonstrate a gate-controlled, continuously tunable bandgap of up to 250 meV. Our technique avoids uncontrolled chemical doping and provides direct evidence of a widely tunable bandgap-spanning a spectral range from zero to mid-infrared-that has eluded previous attempts. Combined with the remarkable electrical transport properties of such systems, this electrostatic bandgap control suggests novel nanoelectronic and nanophotonic device applications based on graphene.〈br /〉〈span class="detail_caption"〉Notes: 〈/span〉Zhang, Yuanbo -- Tang, Tsung-Ta -- Girit, Caglar -- Hao, Zhao -- Martin, Michael C -- Zettl, Alex -- Crommie, Michael F -- Shen, Y Ron -- Wang, Feng -- England -- Nature. 2009 Jun 11;459(7248):820-3. doi: 10.1038/nature08105.〈br /〉〈span class="detail_caption"〉Author address: 〈/span〉Department of Physics, University of California at Berkeley, USA.〈br /〉〈span class="detail_caption"〉Record origin:〈/span〉 〈a href="http://www.ncbi.nlm.nih.gov/pubmed/19516337" target="_blank"〉PubMed〈/a〉
    Print ISSN: 0028-0836
    Electronic ISSN: 1476-4687
    Topics: Biology , Chemistry and Pharmacology , Medicine , Natural Sciences in General , Physics
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  • 3
    Publication Date: 1994-05-06
    Description: Surface vibrational spectroscopy by sum-frequency generation was used to study hydrophobicity at the molecular level at various interfaces: water-surfactant-coated quartz, water-hexane, and water-air. In all cases, hydrophobicity was characterized by the appearance of dangling hydroxyl bonds on 25 percent of the surface water molecules. At the water-quartz interface, packing restrictions force the water surface layer to have a more ordered, ice-like structure. A partly wettable water-quartz interface was also studied.〈br /〉〈span class="detail_caption"〉Notes: 〈/span〉Du, Q -- Freysz, E -- Shen, Y R -- New York, N.Y. -- Science. 1994 May 6;264(5160):826-8.〈br /〉〈span class="detail_caption"〉Record origin:〈/span〉 〈a href="http://www.ncbi.nlm.nih.gov/pubmed/17794723" target="_blank"〉PubMed〈/a〉
    Print ISSN: 0036-8075
    Electronic ISSN: 1095-9203
    Topics: Biology , Chemistry and Pharmacology , Computer Science , Medicine , Natural Sciences in General , Physics
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  • 4
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    American Association for the Advancement of Science (AAAS)
    Publication Date: 2006-09-30
    Description: Time-resolved sum-frequency vibrational spectroscopy permits the study of hitherto neglected ultrafast vibrational dynamics of neat water interfaces. Measurements on interfacial bonded OH stretch modes revealed relaxation behavior on sub-picosecond time scales in close resemblance to that of bulk water. Vibrational excitation is followed by spectral diffusion, vibrational relaxation, and thermalization in the hydrogen-bonding network. Dephasing of the excitation occurs in 〈/=100 femtoseconds. Population relaxation of the dangling OH stretch was found to have a time constant of 1.3 picoseconds, the same as that for excitation transfer between hydrogen-bonded and unbonded OH stretches of water molecules surrounded by acetone.〈br /〉〈span class="detail_caption"〉Notes: 〈/span〉McGuire, John A -- Shen, Y Ron -- New York, N.Y. -- Science. 2006 Sep 29;313(5795):1945-8.〈br /〉〈span class="detail_caption"〉Author address: 〈/span〉Department of Physics, University of California, Berkeley, CA 94720, USA.〈br /〉〈span class="detail_caption"〉Record origin:〈/span〉 〈a href="http://www.ncbi.nlm.nih.gov/pubmed/17008527" target="_blank"〉PubMed〈/a〉
    Print ISSN: 0036-8075
    Electronic ISSN: 1095-9203
    Topics: Biology , Chemistry and Pharmacology , Computer Science , Medicine , Natural Sciences in General , Physics
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  • 5
    Publication Date: 2008-03-15
    Description: Two-dimensional graphene monolayers and bilayers exhibit fascinating electrical transport behaviors. Using infrared spectroscopy, we find that they also have strong interband transitions and that their optical transitions can be substantially modified through electrical gating, much like electrical transport in field-effect transistors. This gate dependence of interband transitions adds a valuable dimension for optically probing graphene band structure. For a graphene monolayer, it yields directly the linear band dispersion of Dirac fermions, whereas in a bilayer, it reveals a dominating van Hove singularity arising from interlayer coupling. The strong and layer-dependent optical transitions of graphene and the tunability by simple electrical gating hold promise for new applications in infrared optics and optoelectronics.〈br /〉〈span class="detail_caption"〉Notes: 〈/span〉Wang, Feng -- Zhang, Yuanbo -- Tian, Chuanshan -- Girit, Caglar -- Zettl, Alex -- Crommie, Michael -- Shen, Y Ron -- New York, N.Y. -- Science. 2008 Apr 11;320(5873):206-9. doi: 10.1126/science.1152793. Epub 2008 Mar 13.〈br /〉〈span class="detail_caption"〉Author address: 〈/span〉Department of Physics, University of California at Berkeley, Berkeley, CA 94720, USA. fengwang76@berkeley.edu〈br /〉〈span class="detail_caption"〉Record origin:〈/span〉 〈a href="http://www.ncbi.nlm.nih.gov/pubmed/18339901" target="_blank"〉PubMed〈/a〉
    Print ISSN: 0036-8075
    Electronic ISSN: 1095-9203
    Topics: Biology , Chemistry and Pharmacology , Computer Science , Medicine , Natural Sciences in General , Physics
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  • 6
    Publication Date: 2016-11-29
    Description: Author(s): Hui Shi, Yu Zhang, Mengyu Yao, Fuhao Ji, Dong Qian, Shan Qiao, Y. R. Shen, and Wei-Tao Liu Second harmonic generation (SHG) from three-dimensional topological insulators originates from both surface and bulk, which does not allow probing of surface states unless the measurement can separate the two contributions. In this paper, we used combined measurements of transmitted and reflected SH… [Phys. Rev. B 94, 205307] Published Mon Nov 28, 2016
    Keywords: Semiconductors II: surfaces, interfaces, microstructures, and related topics
    Print ISSN: 1098-0121
    Electronic ISSN: 1095-3795
    Topics: Physics
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  • 7
    Electronic Resource
    Electronic Resource
    s.l. : American Chemical Society
    The @journal of physical chemistry 〈Washington, DC〉 85 (1981), S. 3327-3333 
    Source: ACS Legacy Archives
    Topics: Chemistry and Pharmacology , Physics
    Type of Medium: Electronic Resource
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  • 8
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 71 (1992), S. 2655-2662 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: We demonstrate that optical second-harmonic generation (SHG) can be successfully used for in situ study of metal/polymer interfaces. With this SHG technique, Cu cluster formation on polyimide by surface diffusion and Cu diffusion into polyimide have been investigated. The diffusion coefficients of Cu clusters into polyimide at various temperatures have been determined from the measured decay of SHG signal with time. The effects of temperature, cluster size, and surface modification on diffusion have also been examined. For T 〈 Tg, the surface diffusion of Cu on polyimide to form clusters dominates over the diffusion into the bulk. The latter process becomes competitive with increasing temperature. When T (approximately-greater-than) Tg, few large-size Cu clusters can be formed on the polyimide surface. Cu diffusion into polyimide bulk can be greatly impeded by either a monolayer of Ti or by Cu clusters implanted in polyimide beforehand. In this case, Cu can wet the modified surface and form an interface between Cu and polyimide with good adhesion.
    Type of Medium: Electronic Resource
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  • 9
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 95 (1991), S. 4620-4625 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: Optical second harmonic generation is employed to investigate the adsorption of soluble naphthalene sulfonates from the bulk solution to the air/water interface in the presence of excess counter ions. Both the surface density of surfactant molecules and the surface pressure were measured as functions of surfactant concentration in solution to yield the adsorption isotherm and the surface pressure/area isotherm. The system investigated shows nonideal gas behavior. The ratio of the activity coefficients at the surface and in the bulk is not unity; however both appear to be constant over the concentration range probed.
    Type of Medium: Electronic Resource
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  • 10
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 88 (1988), S. 4621-4636 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: We used rotational cooling of molecules to ∼5 K by supersonic expansion and state-selective, multilevel saturation spectroscopy to obtain high-resolution spectra of the fundamental and first and second overtone transitions of C–H stretching modes in ground-electronic-state benzene and its dimer. Greatly reduced linewidths (〈3 cm−1 FWHM) in the rich spectra show that previously reported spectra have suffered from inhomogeneous congestion. Our observed spectral widths indicate that the vibrational lifetimes of the C–H stretches are at least a few ps, even at the energy of the second overtone (8800 cm−1). The "local mode'' picture appears to apply when at least three quanta of C–H stretching motion are present. Spectra of the dimer are similar to those of the monomer but show a red shift of a few cm−1, the appearance of combination bands involving van der Waals vibrational modes, some intensity changes, and a broadening of spectral features that increases with the vibrational energy. The dimer's predissociation lifetime at ∼3000 cm−1 vibrational energy exceeds ∼3 ps.
    Type of Medium: Electronic Resource
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