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  • 1
    Publikationsdatum: 2014-01-01
    Beschreibung: This present study shows a comprehensive 2D numerical model for removal of CO2in a polypropylene (PP) hollow fiber membrane contactor (HFMC) using the computational fluid dynamics (CFD) method. Monoethanolamine (MEA) solution was used as the liquid absorbent in a nonwetting mode. The simulation results represented that higher liquid velocity and concentration and lower gas velocity and concentration led to higher percent of CO2removal. The most proper parameters for CO2removal were less than 1 mol m−3gas concentration and 0.2 m s−1gas flow rate, and for MEA the values were above 8 mol m−3concentration and approximately 1 m s−1liquid velocity. Furthermore, the model was validated with the experiment results. Therefore, the modeling results provided references to the selection of absorbents and operation parameters in the experimental study and pilot-scale applications.
    Print ISSN: 1687-806X
    Digitale ISSN: 1687-8078
    Thema: Chemie und Pharmazie , Werkstoffwissenschaften, Fertigungsverfahren, Fertigung
    Publiziert von Hindawi
    Standort Signatur Erwartet Verfügbarkeit
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  • 2
    Publikationsdatum: 2016-01-01
    Beschreibung: Hollow fiber membrane contactor is a new, highly efficient, and the most promising technology for CO2absorption in flue gas. There is still SO2that exists in the flue gas after desulfurization tower of power plant. This paper studied the influence of SO2on CO2absorption characteristic in flue gas by hollow fiber membrane contactor with absorbent of EDA, EDA + MEA (0.6 : 0.4), and EDA + MEA + PZ (0.4 : 0.4 : 0.2). The influences of SO2concentration, cycle absorption and desorption characteristic of absorbent, absorbent concentration, and liquid-gas flow rate ratio are studied to analyze the influence of SO2on CO2absorption characteristic. The appropriate absorbent composition ratio and appropriate parameter range that can inhibit the influence of SO2are proposed by studying the hybrid sorbent with activating agent, appropriate absorbent concentration, and ratio of liquid-gas flow rate. Among the three kinds of absorbents, EDA + MEA + PZ (0.4 : 0.4 : 0.2) had the best tolerance ability to SO2and the highest efficiency. With comprehensive consideration of CO2removal efficiency and operating cost, under the condition of 1000 ppm SO2, the appropriate concentration and liquid-gas flow rate ratio of EDA, EDA + MEA, and EDA + MEA + PZ are proposed.
    Print ISSN: 2090-9063
    Digitale ISSN: 2090-9071
    Thema: Chemie und Pharmazie
    Publiziert von Hindawi
    Standort Signatur Erwartet Verfügbarkeit
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