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  • 1
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    Coupled evolution of temperature and carbonate chemistry during the Paleocene–Eocene; new trace element records from the low latitude Indian Ocean (2020)
    In:  Earth and Planetary Science Letters
    Details
    Publication Date: 2020-12-08
    Description: The early Paleogene represents the most recent interval in Earth's history characterized by global greenhouse warmth on multi-million year timescales, yet our understanding of long-term climate and carbon cycle evolution in the low latitudes, and in particular the Indian Ocean, remains very poorly constrained. Here we present the first long-term sub-eccentricity-resolution stable isotope ( and ) and trace element (Mg/Ca and B/Ca) records spanning the late Paleocene–early Eocene (∼58–53 Ma) across a surface–deep hydrographic reconstruction of the northern Indian Ocean, resolving late Paleocene 405-kyr paced cyclicity and a portion of the PETM recovery. Our new records reveal a long-term warming of ∼4–5 °C at all depths in the water column, with absolute surface ocean temperatures and magnitudes of warming comparable to the low latitude Pacific. As a result of warming, we observe a long-term increase in of the mixed layer, implying an increase in net evaporation. We also observe a collapse in the temperature gradient between mixed layer- and thermocline-dwelling species from ∼57–54 Ma, potentially due to either the development of a more homogeneous water column with a thicker mixed layer, or depth migration of the Morozovella in response to warming. Synchronous warming at both low and high latitudes, along with decreasing B/Ca ratios in planktic foraminifera indicating a decrease in ocean pH and/or increasing dissolved inorganic carbon, suggest that global climate was forced by rising atmospheric CO2 concentrations during this time.
    Type: info:eu-repo/semantics/article
    Format: application/pdf
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  • 2
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    Toward a Cenozoic history of atmospheric CO2 (2023)
    In:  Science
    Details
    Publication Date: 2024-02-12
    Description: The geological record encodes the relationship between climate and atmospheric carbon dioxide (CO2) over long and short timescales, as well as potential drivers of evolutionary transitions. However, reconstructing CO2 beyond direct measurements requires the use of paleoproxies and herein lies the challenge, as proxies differ in their assumptions, degree of understanding, and even reconstructed values. In this study, we critically evaluated, categorized, and integrated available proxies to create a high-fidelity and transparently constructed atmospheric CO2 record spanning the past 66 million years. This newly constructed record provides clearer evidence for higher Earth system sensitivity in the past and for the role of CO2 thresholds in biological and cryosphere evolution.
    Type: info:eu-repo/semantics/article
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  • 3
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    Neogene Mass Accumulation Rate of Carbonate Sediment Across Northern Zealandia, Tasman Sea, Southwest Pacific (2022)
    In:  Paleoceanography and Paleoclimatology
    Details
    Publication Date: 2024-03-28
    Description: Sediment mass accumulation rate (MAR) is a proxy for paleoceanographic conditions, especially if biological productivity generated most of the sediment. We determine MAR records from pelagic calcareous sediments in Tasman Sea based on analysis of 11 boreholes and 〉3 million seismic reflection horizon picks. Seismic data from regions of 10,000–30,000 km2 around each borehole were analyzed using data from International Ocean Discovery Program Expedition 371 and other boreholes. Local MAR was affected by deepwater currents that winnowed, eroded, or deposited seafloor sediment. Therefore, it is necessary to average MARs across regions to test paleoceanographic and productivity models. MARs during the Miocene Climate optimum (18–14 Ma) were slightly lower than Quaternary values but increased on southern Lord Howe Rise at 14–13 Ma, when global climate became colder. Intensification of the Indian and East Asian monsoons at ∼8 Ma and ∼3.6 Ma approximately corresponds to the start and end, respectively, of the Biogenic Bloom, which had MARs at least double Quaternary values. On northern Lord Howe Rise, we recognize peak MARs at∼7 Ma and ∼5 Ma. There is no correlation between Neogene MAR and ocean pH or atmospheric CO2 concentration. Neogene MARs are on average higher than Quaternary values. We posit that future long-term productivity in the southwest Pacific could be higher than Quaternary values, but new computer models that can fit our observations are required to test this hypothesis.
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  • 4
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    Timing of Eocene compressional plate failure during subduction initiation, northern Zealandia, southwestern Pacific (2022)
    In:  Geophysical Journal International
    Details
    Publication Date: 2024-03-28
    Description: Rapid onset of subduction tectonics across the western Pacific convergent margins in the early Eocene was followed by a slower phase of margin growth of the proto Tonga-Kermadec subduction system north of Zealandia during a middle Eocene phase of tectonic adjustment. We present new age constraints from International Ocean Discovery Program Expedition 371 borehole data on deformation events in northern Zealandian sediments that document the formation of the convergent margin boundary northwest of New Zealand. The deformation shows a shortening event that lasted up to 20 myr and acted over distances of ∼1000 km inboard of the evolving plate margin, just northwest of New Zealand. Multichannel seismic profiles tied to our new borehole sites show shortening occurred predominantly between 45 and 35 Ma with some deformation related to slope failure continuing into the Oligocene. The termination of shortening is linked to opening of the backarc basins of the southwest Pacific and the migration of the Tonga-Kermadec Trench to the east which may have removed the structural evidence of the Eocene plate margin. Palaeogene deformation observed inboard of the evolving proto Tonga-Kermadec subduction system indicates that the lithosphere of northern Zealandia, a region of thin continental crust, was strong enough to act as a stress guide. Compressive stresses that caused intraplate folding and faulting developed behind the initiating subduction system with the finite period of deformation indicating the time frame over which an active convergent margin lay along the northern margin of Zealandia.
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  • 5
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    Continental-scale geographic change across Zealandia during Paleogene subduction initiation (2020)
    In:  Geology
    Details
    Publication Date: 2024-03-28
    Description: Data from International Ocean Discovery Program (IODP) Expedition 371 reveal vertical movements of 1–3 km in northern Zealandia during early Cenozoic subduction initiation in the western Pacific Ocean. Lord Howe Rise rose from deep (∼1 km) water to sea level and subsided back, with peak uplift at 50 Ma in the north and between 41 and 32 Ma in the south. The New Caledonia Trough subsided 2–3 km between 55 and 45 Ma. We suggest these elevation changes resulted from crust delamination and mantle flow that led to slab formation. We propose a “subduction resurrection” model in which (1) a subduction rupture event activated lithospheric-scale faults across a broad region during less than ∼5 m.y., and (2) tectonic forces evolved over a further 4–8 m.y. as subducted slabs grew in size and drove plate-motion change. Such a subduction rupture event may have involved nucleation and lateral propagation of slip-weakening rupture along an interconnected set of preexisting weaknesses adjacent to density anomalies.
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  • 6
    Electronic Resource
    Electronic Resource
    Heats of Combustion. VII. The Heats of Combustion of Some Amino Acids (1958)
    s.l. : American Chemical Society
    The @journal of physical chemistry 〈Washington, DC〉 62 (1958), S. 1594-1594 
    Details
    Source: ACS Legacy Archives
    Topics: Chemistry and Pharmacology , Physics
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1021/j150570a032
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  • 7
    Electronic Resource
    Electronic Resource
    Bubble and Foam Fractionation Combined (1965)
    s.l. : American Chemical Society
    Industrial and engineering chemistry 4 (1965), S. 13-16 
    Details
    Source: ACS Legacy Archives
    Topics: Chemistry and Pharmacology , Process Engineering, Biotechnology, Nutrition Technology
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1021/i260013a004
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  • 8
    Electronic Resource
    Electronic Resource
    Acid-Dependent Electrophilicity of Cyclopropylpyrroloindoles. Nature's Masking Strategy for a Potent DNA Alkylator (1994)
    s.l. : American Chemical Society
    Journal of the American Chemical Society 116 (1994), S. 7573-7580 
    Details
    ISSN: 1520-5126
    Source: ACS Legacy Archives
    Topics: Chemistry and Pharmacology
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1021/ja00096a014
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  • 9
    Electronic Resource
    Electronic Resource
    Mechanism of paraquat tolerance in perennial ryegrass (1978)
    Oxford, UK : Blackwell Publishing Ltd
    Plant, cell & environment 1 (1978), S. 0 
    Details
    ISSN: 1365-3040
    Source: Blackwell Publishing Journal Backfiles 1879-2005
    Topics: Biology
    Notes: Abstract The mechanism of paraquat tolerance was investigated in lines of perennial ryegrass (Lolium perenne L.) which had been selected for resistance to the herbicide. Uptake, metabolism and translocation of paraquat were studied. Susceptible cultivars and a tolerant line were not found to differ in uptake of radioactive paraquat applied to the leaf surface or supplied to the cut ends of excised leaves. Distribution of herbicide within leaf tissue was similar in tolerant and susceptible plants and no metabolites of 14C-paraquat were detected in tolerant or susceptible plants treated with sub-lethal concentrations of the herbicide. Autoradiography and quantitative determinations showed much variation in translocation of 14C-paraquat out of treated leaves of intact plants, but the variation was not related to the degree of susceptibility to the herbicide. It is concluded that paraquat tolerance in perennial ryegrass is unlikely to depend upon reduced uptake, enhanced metabolism or altered translocation of the herbicide.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1111/j.1365-3040.1978.tb00762.x
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  • 10
    Electronic Resource
    Electronic Resource
    Mechanism of paraquat tolerance in perennial ryegrass (1978)
    Oxford, UK : Blackwell Publishing Ltd
    Plant, cell & environment 1 (1978), S. 0 
    Details
    ISSN: 1365-3040
    Source: Blackwell Publishing Journal Backfiles 1879-2005
    Topics: Biology
    Notes: Abstract Relative activities of superoxide dismutase, catalase and peroxidase have been determined in crude extracts of 4 paraquat-tolerant lines and 11 paraquat-susceptible cultivars of perennial ryegrass (Lolium perenne L.) grown under controlled conditions. Paraquat-tolerant lines showed significantly higher activities of both catalase and superoxide dismutase than susceptible cultivars and some resistant lines exhibited in addition elevated peroxidase activity. Differences in superoxide dismutase levels in isolated chloroplasts appeared to parallel those in crude extracts. It is tentatively proposed that paraquat tolerance is due to destruction of O2−by elevated concentrations of superoxide dismutase and detoxification of the resulting hydrogen peroxide by increased levels of catalase and peroxidase.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1111/j.1365-3040.1978.tb00763.x
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