Publication Date:
2019-07-12
Description:
Cyclic temporal variations of pH and ionic concentration in sampled clouds which traversed the Mt. Mitchell State Park (North Carolina) site during the summers of 1986, 1987, and 1988 are reported. These clouds typically had a measured pH minimum during their initial and final stages. The cause of this basic cylic pattern is attributed to sampling at different vertical levels of the cloud. This is substantiated by visual observations made while sampling. The results also suggest that the measured pH patterns do not always exhibit minima during the formative and dissipative stages of the cloud, apparently in response to the underlying dynamical processes. The relationship between temporal pH measurements made at a stationary site to vertical cloud levels provides insights into the physical processes (e.g., nucleation scavenging near cloud base, dry air entrainment near cloud top) influencing the observed cloud-water chemistry on a real-time basis and would improve cloud chemistry models.
Keywords:
METEOROLOGY AND CLIMATOLOGY
Type:
Journal of the Atmospheric Sciences (ISSN 0022-4928); 47; 1117-112
Format:
text
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